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We consider the optical properties of a single magnetic impurity in a self-assembled quantum dot. We show that using the resonant pumping one can address and manipulate selectively individual spin states of a magnetic impurity. The…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 A. O. Govorov , A. V. Kalameitsev

The optical orientation of Mn$^{2+}$ spins in the first excited state $^4$T$_1$ was experimentally observed in bulk (Zn, Mn)Se ($x_\mathrm{Mn}=0.01$) in the an external magnetic field of up to $6\,$T in Faraday geometry. This occurred…

Mesoscale and Nanoscale Physics · Physics 2024-10-15 N. V. Kozyrev , K. A. Baryshnikov , B. R. Namozov , I. I. Kozlov , M. E. Boiko , N. S. Averkiev , Yu. G. Kusrayev

The efficient single photon emission capabilities of quantum dot molecules position them as promising platforms for quantum information processing. Furthermore, quantum dot molecules feature a "decoherence-free" subspace that enables spin…

Quantum Physics · Physics 2021-03-31 D. Farfurnik , R. M. Pettit , Z. Luo , E. Waks

We investigated optical spin orientation and dynamic nuclear polarization (DNP) in individual self-assembled InGaAs/GaAs quantum dots (QDs) doped by a single Mn atom, a magnetic impurity providing a neutral acceptor A$^0$ with an effective…

Mesoscale and Nanoscale Physics · Physics 2016-11-15 O. Krebs , E. Baudin , A. Lemaître

The spin of an electron in a self-assembled InAs/GaAs quantum dot molecule is optically prepared and measured through the trion triplet states. A longitudinal magnetic field is used to tune two of the trion states into resonance, forming a…

We present the results of a comprehensive magneto-optical characterization of single CdTe quantum dots containing a few Mn2+ ions. We find that some quantum dots exhibit an unexpected evolution of excitonic photoluminescence spectrum with…

Mesoscale and Nanoscale Physics · Physics 2017-01-04 Maciej Koperski , Tomasz Smoleński , Mateusz Goryca , Piotr Wojnar , Marek Potemski , Piotr Kossacki

To understand and optimize optical spin initialization in room temperature CdSe nanocrystal quantum dots (NCQDs) we studied the dependence of the time-resolved Faraday rotation signal on pump energy $E_p$ in a series of NCQD samples with…

Mesoscale and Nanoscale Physics · Physics 2014-07-22 A. Khastehdel Fumani , J. Berezovsky

We present a comprehensive examination of optical pumping of spins in individual GaAs quantum dots as we change the charge from positive to neutral to negative using a Schottky diode. We observe that photoluminescence polarization memory…

Initializing a set of qubits to a given quantum state is a basic prerequisite for the physical implementation of quantum-information protocols. Here, we discuss the polarization of the electronic and nuclear spin in a single nitrogen…

Quantum Physics · Physics 2017-07-26 Tanmoy Chakraborty , Jingfu Zhang , Dieter Suter

We have performed all-optical measurements of spin relaxation in single self-assembled InAs/GaAs quantum dots (QD) as a function of static external electric and magnetic fields. To study QD spin dynamics we measure the degree of resonant…

Mesoscale and Nanoscale Physics · Physics 2009-09-29 Jan Dreiser , Mete Atature , Christophe Galland , Tina Muller , Antonio Badolato , Atac Imamoglu

We investigate the optical properties of (Cd,Mn)Te quantum dots (QDs) by looking at the excitons as a function of the Mn impurities positions and their magnetic alignments. When doped with two Mn impurities, the Mn spins, aligned initially…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 C. Echeverría-Arrondo , J. Pérez-Conde , A. Ayuela

We review spin properties of semiconductor quantum dots and their effect on optical spectra. Photoluminescence and other types of spectroscopy are used to probe neutral and charged excitons in individual quantum dots with high spectral and…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Allan S. Bracker , Daniel Gammon , Vladimir L. Korenev

The optical manipulation of electron spins is of great benefit to solid-state quantum information processing. In this letter, we provide a comparative study on the ultrafast optical manipulation of single electron spin in the doped and…

Other Condensed Matter · Physics 2009-11-11 Jinshuang Jin , Xin-Qi Li , YiJing Yan

We investigate spin and charge current through a quantum dot pumped by a time-varying magnetic field. Using the density matrix method, quantum rate equations for the electronic occupation numbers in the quantum dot are obtained and solved…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Zhao Yang Zeng , Hong Li , Baowen Li

The use of single electron spins in quantum dots as qubits requires detailed knowledge about the processes involved in their initialization and operation as well as their relaxation and decoherence. In optical schemes for such spin qubits,…

Mesoscale and Nanoscale Physics · Physics 2024-02-19 Eric Kleinherbers , Hendrik Mannel , Jens Kerski , Martin Geller , Axel Lorke , Jürgen König

We present a direct observation of a coherent spin precession of an individual Mn$^{2+}$ ion, having both electronic and nuclear spins equal to 5/2, embedded in a CdTe quantum dot and placed in magnetic field. The spin state evolution is…

Mesoscale and Nanoscale Physics · Physics 2014-11-27 M. Goryca , M. Koperski , P. Wojnar , T. Smoleński , T. Kazimierczuk , A. Golnik , P. Kossacki

We report optical pumping of neutral quantum dots leading to nuclear spin alignment with direction insensitive to polarization and wavelength of light. Measurements of photoluminescence of both "dark" and "bright" excitons in single dots…

Mesoscale and Nanoscale Physics · Physics 2011-04-05 E. A. Chekhovich , A. B. Krysa , M. S. Skolnick , A. I. Tartakovskii

We use femtosecond optical pulses to induce, control and monitor magnetization precession in ferromagnetic Ga0.965Mn0.035As. At temperatures below ~40 K we observe coherent oscillations of the local Mn spins, triggered by an ultrafast…

Materials Science · Physics 2009-11-13 J. Qi , Y. Xu , N. Tolk , X. Liu , J. K. Furdyna , I. E. Perakis

A common impediment to qubit performance is imperfect state initialization. In the case of the diamond nitrogen-vacancy (NV) center, the initialization fidelity is limited by fluctuations in the defect's charge state during optical pumping.…

Quantum Physics · Physics 2021-12-13 David A. Hopper , Joseph D. Lauigan , Tzu-Yung Huang , Lee C. Bassett

We study theoretically the recently proposed hole spin initialization scheme for $p$-doped quantum well or dot systems via coupling to trion states with sub-picosecond circularly polarized laser pulses. We analyze the efficiency of spin…

Mesoscale and Nanoscale Physics · Physics 2018-01-11 Michał Gawełczyk , Paweł Machnikowski