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We study high-order harmonic generation (HHG) from aligned molecules in strong elliptically polarized laser fields numerically and analytically. Our simulations show that the spectra and polarization of HHG depend strongly on the molecular…

Atomic Physics · Physics 2021-05-19 F. J. Sun , C. Chen , W. Y. Li , X. Liu , W. Li , Y. J. Chen

We study the ellipticity of high-order harmonics emitted from CO$_2$ molecule driven by linearly polarized laser fields using numerical simulations within the time-dependent density functional theory. We find that the overall ellipticity of…

Atomic and Molecular Clusters · Physics 2024-09-17 Andres Mora , Lauren Bauerle , Yuqing Xia , Agnieszka Jaron

The present work reports on the generation of short-pulse coherent extreme ultraviolet radiation of controlled polarization. The proposed strategy is based on high-order harmonics generated in pre-aligned molecules. Field-free molecular…

A recent paper reported elliptically polarized high-order harmonics from aligned N$_2$ using a linearly polarized driving field [X. Zhou \emph{et al.}, Phys. Rev. Lett. \textbf{102}, 073902 (2009)]. This observation cannot be explained in…

Atomic Physics · Physics 2010-03-29 Adam Etches , Christian Bruun Madsen , Lars Bojer Madsen

We carried out a joint theoretical and experimental study of the polarization of high-order harmonics generated from ZnO by intense infrared laser pulses. Experimentally we found that the dependence of parallel and perpendicular…

We investigate the polarization properties of high harmonic generation from polar molecules with a linearly polarized field. It is found that elliptically polarized harmonics are observed in a wide spectral range from the plateau to the…

Optics · Physics 2011-12-06 Meiyan Qin , Xiaosong Zhu , Qingbin Zhang , Weiyi Hong , Peixiang Lu

We investigate the influence of intense, elliptically polarized driving fields on high-order harmonic spectra from aligned diatomic molecules. We derive a generalized two-center interference condition for elliptically polarized fields,…

Atomic Physics · Physics 2015-06-16 T. Das , B. B. Augstein , C. Figueira de Morisson Faria

We show that high-order harmonics generated from molecules by intense laser pulses can be expressed as the product of a returning electron wave packet and the photo-recombination cross section (PRCS) where the electron wave packet can be…

Atomic Physics · Physics 2008-04-04 Anh-Thu Le , R. Della Picca , P. D. Fainstein , D. A. Telnov , M. Lein , C. D. Lin

We investigate the process of circularly polarized high harmonic generation in molecules using a bicircular laser field. In this context, we show that molecules offer a very robust framework for the production of circularly polarized…

Atomic Physics · Physics 2016-06-22 F Mauger , A. D. Bandrauk , T Uzer

The present work introduces a robust way to generate attosecond pulses with tunable ellipticity via high-order harmonic generation by co-rotating $\omega - 2\omega$ bicircular laser fields. The total electric field of the laser fields…

Optics · Physics 2023-05-02 Rambabu Rajpoot , Amol R. Holkundkar , Navdeep Rana , Gopal Dixit

The below-threshold harmonic generation in the multiphoton ionization regime for a helium atom driven by the elliptically polarized laser field is studied numerically within the framework of two-dimensional (2D) and three-dimensional (3D)…

Optics · Physics 2024-12-11 Mikhail Yu. Emelin , Mikhail Yu. Ryabikin

Spectra of circularly polarized harmonics is calculated by numerically solving the Time-Dependent Schr\"{o}dinger Equation for a 2D model of Ne atom using circularly polarized fundamental with counter-rotating second harmonic laser fields.…

Atomic Physics · Physics 2015-10-28 Lukas Medišauskas , Jack Wragg , Hugo van der Haart , Misha Yu. Ivanov

An investigation of field-free molecular alignment produced by elliptically polarized laser pulses is reported. Experiments are conducted in CO$_2$ at room temperature. A non invasive all-optical technique, based on the cross defocusing of…

Quantum Physics · Physics 2008-12-18 E. Hertz , D. Daems , S. Guérin , H. R. Jauslin , B. Lavorel , O. Faucher

This paper describes a method for the explicit reconstruction and visualization of various polarization ellipses from the intensities measured after a rotating polarizer. The state of polarization of a light beam is represented by the…

Optics · Physics 2022-11-29 Ramonika Sengupta , Brijesh Tripathi , Asha Adhiya

We present a numerical study of the resonant high harmonic generation by tin ions in an elliptically-polarised laser field along with a simple analytical model revealing the mechanism and main features of this process. We show that the…

Optics · Physics 2021-04-22 M. A. Khokhlova , M. Yu. Emelin , M. Yu. Ryabikin , V. V. Strelkov

We studied the high-order harmonic generation (HHG) from 2D solid materials in circularly and bichromatic circularly polarized laser fields numerically by simulating the dynamics of single-active-electron processes in 2D periodic…

Photoelectron angular distributions (PADs) of oriented polar molecules in response to different polarized lasers are systematically investigated. It is found that the PADs of polar CO molecules show three distinct styles excited by…

Chemical Physics · Physics 2013-03-05 Xiaosong Zhu , Qingbin Zhang , Weiyi Hong , Peixiang Lu , Zhizhan Xu

We investigate the polarization properties of high harmonics generated with the bichromatic counterrotating circularly polarized (BCCP) laser fields by numerically solving time-dependent Schr\"odinger equation (TDSE). It is found that, the…

Atomic Physics · Physics 2016-12-21 Xiaofan Zhang , Liang Li , Xiaosong Zhu , Xi Liu , Qingbin Zhang , Pengfei Lan , Peixiang Lu

We observe the generation of high harmonics in the plane perpendicular to the driving laser polarization and show that these are driven by the spin-orbit interaction. Using R-Matrix with time-dependence theory, we demonstrate that for…

Quantum-mechanical investigation is presented to study single attosecond pulse generation by gating high-order harmonic emission from H$_2^+$ molecule in intense laser pulses with time-dependent ellipticity. The high-order harmonic…

Atomic Physics · Physics 2018-01-17 Nehzat Safaei
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