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Tracking the coupled motion of electrons and nuclei on their intrinsic timescales is essential to understanding and controlling photochemical transformations. While attosecond techniques have provided unprecedented insight into electronic…

In classical mechanics and electromagnetism, interference occurs when two or more waves overlap at the same point in spacetime. However, the advent of quantum electrodynamics (QED) and its remarkable success in describing light-matter…

Quantum Physics · Physics 2025-08-15 Alan C. Santos , Celso J. Villas-Boas

Coherent electron displacement is a conventional strategy for processing quantum information, as it enables to interconnect distinct sites in a network of atoms. The efficiency of the processing relies on the precise control of the…

Quantum Physics · Physics 2020-12-02 Hicham Agueny

Atom interferometers provide a powerful tool for measuring physical constants and testifying fundamental physics with unprecedented precision. Conventional atom interferometry focuses on the phase difference between two paths and utilizes…

Quantum Gases · Physics 2024-06-25 Peng Peng , Dekai Mao , Yi Liang , Guoling Yin , Hongmian Shui , Bo Song , Xiaoji Zhou

The time-dependent Schr\"{o}dinger equation for the hydrogen atom and its interaction with coherent intense high-frequency short laser pulses is solved numerically exactly by propagating the single-electron wave packets. Thereby, the…

Atomic Physics · Physics 2013-09-11 Philipp V. Demekhin , David Hochstuhl , Lorenz S. Cederbaum

The theory of resonant Auger decay of atoms in a high intensity coherent X-ray pulse is presented. The theory includes the coupling between the ground state and the resonance due to an intense X-ray pulse, taking into account the decay of…

Atomic Physics · Physics 2011-05-27 Philipp V Demekhin , Lorenz S. Cederbaum

Ultrashort pulses can excite or ionize molecules and populate coherent electronic wavepackets, inducing complex dynamics. In this work, we simulate the coupled electron-nuclear dynamics upon ionization to different electronic wavepackets of…

Based on numerical solutions of the time-dependent Schr\"odinger equation for either one or two active electrons, we propose a method for observing instantaneous level shifts in an oscillating strong infrared (IR) field in time, using a…

Atomic Physics · Physics 2015-05-28 Feng He , Camilo Ruiz , Andreas Becker , Uwe Thumm

We report the experimental observation of quantum interference in the nuclear wave-packet dynamics driving ultrafast excitation-energy transfer in argon dimers below the threshold of interatomic Coulombic decay (ICD). Using time-resolved…

Atomic and Molecular Clusters · Physics 2023-07-05 Meng Han , Jacqueline Fedyk , Jia-Bao Ji , Victor Despré , Alexander I. Kuleff , Hans Jakob Wörner

Shaping electron beams with the cycles of light provides femtosecond and attosecond time resolution in electron microscopy and enables fundamental quantum-coherent measurements. However, efficient light-electron control requires a prolonged…

We propose an experiment to observe interference of a single electron as it is transported along two parallel quasi-one-dimensional channels trapped in a single minimum of a travelling periodic electric field. The experimental device is a…

Attosecond physics enables the study of ultrafast coherent electron dynamics in matter upon photoexcitation and photoionization, revealing spectacular effects such as hole migration and coherent Auger dynamics in molecules. In the…

Atomic Physics · Physics 2024-01-15 Marco Ruberti , Vitali Averbukh , Florian Mintert

We study resonance contrast by a two-step pulse observation method to enhance the frequency stability of coherent population trapping (CPT) atomic clocks. The proposed method is a two-step Raman--Ramsey scheme with low intensity during…

Atomic Physics · Physics 2017-03-08 Yuichiro Yano , Shigeyoshi Goka , Masatoshi Kajita

In a multi-electron atom, an excited electron can decay by emitting a photon. Typically, the leftover electrons are in their ground state. In a radiative Auger process, the leftover electrons are in an excited state and a redshifted photon…

Complementarity lies at the heart of conceptual foundation of orthodox quantum mechanics. The wave-particle duality makes it impossible to tell which slit each particle passes through and still observe an interference pattern in a Young's…

Quantum Physics · Physics 2007-05-23 Zhi-Yuan Li

We introduce a novel technique for enhancing the robustness of light-pulse atom interferometers against the pulse infidelities that typically limit their sensitivities. The technique uses quantum optimal control to favorably harness the…

We explore the possibility of retrieving Auger spectra with FEL radiation. Using a laser pulse of 260 eV photon energy, we study the interplay of photo-ionization and Auger processes following the initial formation of a 2p inner-shell hole…

Atomic Physics · Physics 2015-06-19 Alisdair O. G. Wallis , L. Lodi , A. Emmanouilidou

The Zeeman-split spin states of a single quantum dot can be used together with its optical trion transitions to form a spin-photon interface between a stationary (the spin) and a flying (the photon) quantum bit. Besides long coherence times…

Mesoscale and Nanoscale Physics · Physics 2021-10-26 Hendrik Mannel , Jens Kerski , Pia Lochner , Marcel Zöllner , Andreas D. Wieck , Arne Ludwig , Axel Lorke , Martin Geller

A technique complementary to those for spectral lines is proposed for the observation of continuum radiation. As, quantum mechanically, the radiation is a mixture of pure states, it should be possible to measure the temporal coherence of…

Quantum Physics · Physics 2015-10-08 Richard Fong

We report on the design and performance of a double-sided coincidence velocity map imaging spectrometer optimized for electron-ion and ion-ion coincidence experiments studying inner-shell photoionization of gas-phase molecules with soft…