Related papers: Decoherence in Weakly Coupled Excitonic Complexes
We show that the biomolecular exciton dynamics under the influence of slow polarization fluctuations in the solvent cannot be described by approaches which are perturbative in the system-bath coupling. For this, we compare results for the…
We compare four different types of equations of motion for reduced density matrix of a system of molecular excitons interacting with thermodynamic bath. All four equations are of second order in the linear system-bath interaction…
The prospect of coherent dynamics and excitonic delocalization across several light-harvesting structures in photosynthetic membranes is of considerable interest, but challenging to explore experimentally. Here we demonstrate theoretically…
Decoherence is a major obstacle to any practical implementation of quantum information processing. One of the leading strategies to reduce decoherence is dynamical decoupling --- the use of an external field to average out the effect of the…
Realising scalable quantum networks requires a meticulous level of understanding and mitigating the deleterious effects of decoherence. Many quantum device platforms feature multiple decoherence mechanisms, often with a dominant mechanism…
We present a rigorous theoretical description of excitonic dynamics in molecular light-harvesting aggregates photoexcited by weak-intensity radiation of arbitrary properties. While the interaction with light is included up to the second…
Properties of weak spatio-spectral twin beams in paraxial approximation are analyzed using the decomposition into appropriate paired modes. Numbers of paired modes as well as numbers of modes in the signal (or idler) field in the transverse…
Phonon interactions in solid-state photonics systems cause intrinsic quantum decoherence and often present the limiting factor in emerging quantum technology. Due to recent developments in nanophotonics, exciton-cavity structures with very…
We derive a non-Markovian master equation for a charged particle in a magnetic field coupled to a bath and study decoherence by analysing the temporal decay of the off-diagonal elements of the reduced density matrix in the position basis.…
The idea that excitonic state (electronic) coherences are of fundamental importance to natural photosynthesis gained popularity when, a decade ago, slowly dephasing quantum beats were observed in the two-dimensional electronic spectra of…
A popular model of decoherence based on the linear coupling to harmonic oscillator heat baths is analized and shown to be inappropriate in the regime where decoherence dominates over energy dissipation, called pure decoherence regime. The…
We demonstrate in a very general fashion, considerable slowing down of decoherence and relaxation by fast frequency modulation of the system heat bath coupling. The slowing occurs as the decoherence rates are now determined by the spectral…
A theoretical description of local absorption is proposed in order to investigate spectral variations on a length scale comparable with the extension of the relevant quantum states. A general formulation is derived within the density-matrix…
We present an approach that allows quantifying decoherence processes in an open quantum system subject to external time-dependent control. Interactions with the environment are modeled by a standard bosonic heat bath. We develop two…
Recent ultrafast optical experiments show that excitons in large biological light-harvesting complexes are coupled to molecular vibration modes. These high-frequency vibrations will not only affect the optical response, but also drive the…
Weak measurement is a new technique which allows one to describe the evolution of postselected quantum systems. It appears to be useful for resolving a variety of thorny quantum paradoxes, particularly when used to study properties of pairs…
Long-lived beatings in two-dimensional electronic spectroscopy (2DES) remain difficult to interpret within standard excitonic open-system models, which typically assume factorized initialization and predict rapid coherence decay. We show…
The dynamics of excitonic energy transfer in molecular complexes triggered by interaction with laser pulses offers a unique window into the underlying physical processes. The absorbed energy moves through the network of interlinked pigments…
Coupling to phonon modes is a primary mechanism of excitonic dephasing and energy loss in semiconductors. However, low-energy phonons in colloidal quantum dots and their coupling to excitons are poorly understood, since their experimental…
We report an anomalous decoherence phenomenon of a quantum dissipative system in the framework of a stochastic decoupling scheme along with a hierarchical equations-of-motion formalism without the usual Born-Markov or weak coupling…