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We performed high-resolution powder neutron diffraction experiments and discovered an elliptic helical incommensurate magnetic structure in the semiconducting rare-earth magnet YbCuS2, featuring effective spin-1/2 Yb$^{3+}$ ions that form a…

Strongly Correlated Electrons · Physics 2025-01-09 T. Onimaru , Y. Ohmagari , S. Mizutani , R. Yamamoto , H. Kaneshima , C. Moriyoshi , D. T. Adroja , D. Khyalyavin , P. Manuel , H. Saito , C. Hotta

We report $^{75}$As Nuclear Magnetic Resonance data in a single crystal of CaFe$_2$As$_2$. The Knight shift, electric field gradient, and spin-lattice relaxation rate are strongly temperature dependent in the paramagnetic state, and change…

Strongly Correlated Electrons · Physics 2009-02-11 S. -H. Baek , N. J. Curro , T. Klimczuk , E. D. Bauer , F. Ronning , J. D. Thompson

The manganese tellurate Li2MnTeO6 consists of trigonal spin lattices made up of Mn4+ (d3, S = 3/2) ions. The magnetic properties of this compound were characterized by several experimental techniques, which include magnetic susceptibility,…

In this Letter we report high-resolution synchrotron X-ray powder diffraction and transmission electron microscope analysis of Mn-substituted LaFeAsO samples, demonstrating that a static incommensurate modulated structure develops across…

Superconductivity · Physics 2017-02-08 A. Martinelli , P. Manfrinetti , A. Provino , A. Genovese , F. Caglieris , G. Lamura , C. Ritter , M. Putti

Macroscopic magnetic properties and microscopic magnetic structure of Rb$_2$Mn$_3$(MoO$_4$)$_3$(OH)$_2$ (space group $Pnma$) are investigated by magnetization, heat capacity and single-crystal neutron diffraction measurements. The…

The new quaternary iron arsenide-fluoride SrFeAsF with the tetragonal ZrCuSiAs-type structure was synthesized and the crystal structure was determined by X-ray powder diffraction (P4/nmm, a = 399.30(1), c = 895.46(1) pm). SrFeAsF undergoes…

Superconductivity · Physics 2009-01-06 M. Tegel , S. Johansson , V. Weiss , I. Schellenberg , W. Hermes , R. Poettgen , Dirk Johrendt

The complex metal oxide Mn3TeO6 exhibits a corundum related structure and has been prepared both in forms of single crystals by chemical transport reactions and of polycrystalline powders by a solid state reaction route. The crystal…

Materials Science · Physics 2011-09-15 S. A. Ivanov , P. Nordblad , R. Mathieu , R. Tellgren , C. Ritter , N. Golubko , E. D. Politova , M. Weil

We present the results of the first neutron powder and single crystal diffraction studies of the coupled spin tetrahedra systems ${\CuTeX}$ (X=Cl, Br). Incommensurate antiferromagnetic order with the propagation vectors…

Strongly Correlated Electrons · Physics 2009-11-10 O. Zaharko , A. Daoud-Aladine , S. Streule , J. Mesot , P. -J. Brown , H. Berger

A complex magnetic order of the multiferroic compound Co3TeO6 has been revealed by neutron powder diffraction studies on ceramics and crushed single crystals. The compound adopts a monoclinic structure (s.g. C2/c) in the studied temperature…

Materials Science · Physics 2011-11-28 S. A. Ivanov , R. Tellgren , C. Ritter , P. Nordblad , R. Mathieu , G. Andre , N. V. Golubko , E. D. Politova , M. Weil

The iron arsenide Sr2CrO3FeAs with the tetragonal Sr2GaO3CuS-type structure was synthesized and its crystal structure re-determined by neutron powder diffraction. In contrast to previous X-ray crystallographic studies, a mixed occupancy of…

Superconductivity · Physics 2010-02-24 Marcus Tegel , Franziska Hummel , Yixi Su , Tapan Chatterji , Michela Brunelli , Dirk Johrendt

Magnetic susceptibility, specific heat, and neutron powder diffraction measurements have been performed on polycrystalline Li2Co(WO4)2 samples. Under zero magnetic field, two successive magnetic transitions at TN1 ~ 9.4 K and TN2 ~ 7.4 K…

The magnetic phase transitions reported below 230 K in cupric oxide are analyzed theoretically at the macroscopic and microscopic levels. The incommensurate multiferroic and lock-in commensurate phases are shown to realize an inverted…

We report a neutron diffraction study of the magnetic phase transitions in the charge-density-wave (CDW) TbTe$_3$ compound. We discover that in the paramagnetic phase there are strong 2D-like magnetic correlations, consistent with the…

Strongly Correlated Electrons · Physics 2012-01-10 F. S. Pfuner , S. N. Gvasaliya , O. Zaharko , L. Keller , J. Mesot , V. Pomjakushin , J. -H. Chu , I. R. Fisher , L. Degiorgi

We performed elastic neutron scattering and magnetization measurements on Fe(1.07)Te(0.75)Se(0.25) and FeTe(0.7)Se(0.3). Short-range incommensurate magnetic order is observed in both samples. In the former sample with higher Fe content, a…

Superconductivity · Physics 2009-09-11 Jinsheng Wen , Guangyong Xu , Zhijun Xu , Zhi Wei Lin , Qiang Li , W. Ratcliff , Genda Gu , J. M. Tranquada

Magnetic excitations and magnetic structure of EuRbFe$_4$As$_4$ were investigated by inelastic neutron scattering (INS), neutron diffraction, and random phase approximation (RPA) calculations. Below the superconducting transition…

Neutron scattering and muon spin rotation ($\mu$SR) measurements on single-crystal SmAu$_3$Al$_7$ reveal magnetically ordered states associated with successive transitions at $T_{\rm N}$ = 2.8 K and $T^*$ = 0.9 K. Magnetic Bragg peaks…

Temperature dependent $^{57}$Fe M\"ossbauer spectroscopy and specific heat measurements for CaK(Fe$_{1-x}$Ni$_x$)$_4$As$_4$ with $x$ = 0, 0.017, 0.033, and 0.049 are presented. No magnetic hyperfine field (e.g. no static magnetic order)…

The newly discovered Ising-type ferromagnet CeRu$_2$Al$_2$B exhibits an additional phase transition at $T_\textrm{N}$ = 14.2 K before entering the ferromagnetic ground state at $T_\textrm{C}$ = 12.8 K. We clarify the nature of this…

Strongly Correlated Electrons · Physics 2016-03-09 A. Bhattacharyya , D. D. Khalyavin , F. Krüger , D. T. Adroja , A. M. Strydom , W. A. Kockelmann , A. D . Hillier

Neutron diffraction measurements of a high quality single crystal of CaFe2As2 are reported. A sharp transition was observed between the high temperature tetragonal and low temperature orthorhombic structures at TS = 172.5K (on cooling) and…

hrough neutron diffraction experiments, including spin-polarized measurements, we find a collinear incommensurate spin-density wave with propagation vector $ \mathbf k = $ ($0.4481(4) \, \,0 \, \, \frac1 2$) at base temperature in the…