English
Related papers

Related papers: Dimerization-assisted energy transport in light-ha…

200 papers

Fluctuations in the energy gap and coupling constants in and between chromophores can play important role in the absorption and energy transfer across a collection of two level systems. In a noisy environment, fluctuations can control…

Chemical Physics · Physics 2024-04-17 Rajesh Dutta , Biman Bagchi

As a minimal model to study charge transfer effects in a transition metal (TM) and Oxygen (OX) chain, we consider a one-dimensional chain with spinless fermion with an alternating motif of site-pairs with nearest neighbor (NN) repulsion $U$…

Strongly Correlated Electrons · Physics 2023-10-05 Prabhakar , Anamitra Mukherjee

The most recent crystal structure of the Fenna-Matthews-Olson (FMO) protein complex indicates that each subunit contains an additional eighth chromophore. It has been proposed that this extra site functions as a link between the chlorosome…

Biological Physics · Physics 2011-09-16 Jeremy Moix , Jianlan Wu , Pengfei Huo , David Coker , Jianshu Cao

We investigate entanglement dynamics in bipartite systems governed by inhomogeneous Hamiltonians of the form $H = H_L + H_R$, where $H_{L/R}$ acts only on the left or right region and is homogeneous within each region. Focusing on the XX…

Statistical Mechanics · Physics 2026-05-05 Andrea Di Pasquale , Federico Rottoli , Vincenzo Alba

Decoupling charge and heat transport is essential for optimizing thermoelectric materials. Strategies to inhibit lattice-driven heat transport, however, also compromise carrier mobility, limiting the performance of most thermoelectrics,…

We present a systematic analysis and classification of several models of quantum batteries involving different combinations of two level systems and quantum harmonic oscillators. In particular, we study energy transfer processes from a…

In an organic blend the vibrational normal mode excited by exciton splitting is the same as the one coupled to charge hopping. Excess driving force for exciton splitting can therefore aid charge transfer, if vibrational relaxation is slow…

Mesoscale and Nanoscale Physics · Physics 2010-04-05 James Kirkpatrick

Dual fluorescence in 4-(dimethylamino)benzonitrile (DMABN) and its derivatives in polar solvents has been studied extensively for the past several decades. An intramolecular charge transfer (ICT) minimum on the excited state potential…

Chemical Physics · Physics 2025-03-26 Avdhoot Datar , Saisrinivas Gudivada , Devin A. Matthews

For more than 50 years we have known that photosynthetic systems harvest solar energy with almost unit {\it quantum efficiency}. However, recent experimental evidence of {\it quantum coherence} during the excitonic energy transport in…

Biological Physics · Physics 2012-05-25 Tobias Zech , Roberto Mulet , Thomas Wellens , Andreas Buchleitner

2D transition metal dichalcogenides (TMDCs) exhibit an electron-hole liquid phase transition at unusually high temperatures. Because these materials are atomically thin, optical excitation leads to material expansion. As a result, during…

Mesoscale and Nanoscale Physics · Physics 2021-02-17 R. L. Wilmington , H. Ardekani , A. Rustagi , A. Bataller , A. F. Kemper , R. A. Younts , K. Gundogdu

We investigate the time an electronic excitation travels in a supermolecular setup using a measurement process in an open quantum-system framework. The approach is based on the stochastic Schr\"odinger equation and uses a Hamiltonian from…

Materials Science · Physics 2013-12-09 Dirk Hofmann , Heiko Appel , Massimiliano Di Ventra , Stephan Kümmel

Donor-acceptor (D-A) type copolymers show great potential for the application in the active layer of organic solar cells. Nevertheless the nature of the excited states, the coupling mechanism and the relaxation pathways following…

We review recent theoretical calculations of quantum entanglement in photosynthetic light harvesting complexes. These works establish, for the first time, a manifestation of this characteristically quantum mechanical phenomenon in…

Quantum Physics · Physics 2010-12-21 K. Birgitta Whaley , Mohan Sarovar , Akihito Ishizaki

The electroosmotic transfer (ratio of velocity of liquid to electric current density) and conductivity of disperse system were calculated as functions of volume fraction of disperse particles. The considered model of electric double layer…

Soft Condensed Matter · Physics 2007-05-23 V. N. Shilov , N. I. Zharkikh

Nanometer-thick quantum-well structures are quantum model systems offering a few discrete unoccupied energy states that can be impulsively filled and that relax back to equilibrium predominantly via spontaneous emission of light. Here we…

Materials Science · Physics 2024-01-03 Michele Perlangeli , Francesco Proietto , Fulvio Parmigiani , Federico Cilento

In two-dimensional (2D) electron systems, an off-resonant high-frequency circularly polarized electromagnetic field can induce the quasi-stationary bound electron states of repulsive scatterers. As a consequence, the resonant scattering of…

Mesoscale and Nanoscale Physics · Physics 2020-08-07 O. V. Kibis , M. V. Boev , V. M. Kovalev

Confinement-deconfinement transition in quarter-filled two-coupled chains comprising dimerization, repulsive interactions and interchain hopping has been demonstrated by applying the renormalization group method to the bosonized…

Strongly Correlated Electrons · Physics 2009-10-31 Y. Suzumura , M. Tsuchiizu

The initial energy transfer in photosynthesis occurs between the light-harvesting pigments and on ultrafast timescales. We analyze the carotenoid to bacteriochlorophyll energy transfer in LH2 Marichromatium purpuratum as well as in an…

Photosystem I is a protein-pigment complex that performs photosynthesis in plants, green algae, and cyanobacteria. It contains an aggregate of chlorophylls that absorbs light and delivers the resulting electronic excitation to the special…

Biological Physics · Physics 2007-05-23 Sanghyun Park , Melih K. Sener , Deyu Lu , Klaus Schulten

Photoinduced charge-transfer processes play a key role for novel photovoltaic phenomena and devices. Thus, the development of ab initio methods that allow for an accurate and computationally inexpensive treatment of charge-transfer…

Chemical Physics · Physics 2014-04-25 Iris Theophilou , M. Tassi , S. Thanos