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The power conversion efficiency of organic solar cells based on donor--acceptor blends is governed by an interplay of polaron pair dissociation and bimolecular polaron recombination. Both processes are strongly dependent on the charge…

Materials Science · Physics 2010-05-26 C. Deibel , A. Wagenpfahl , V. Dyakonov

Surface recombination has a major impact on the open-circuit voltage ($V_\text{oc}$) of organic photovoltaics. Here, we study how this loss mechanism is influenced by imbalanced charge transport in the photoactive layer. As a model system,…

Radiative and non-radiative charge carrier recombination in thin-film diodes plays a key role in determining the efficiency of electronic devices made of next generation semiconductors such as organic, perovskite and nanocrystals. In this…

Applied Physics · Physics 2019-08-06 Oskar J. Sandberg , Ardalan Armin

Solar energy is the most convenient and reliable energy source among all renewable energy resources and an efficient photovoltaic device is required to convert this energy into utilizable energy. Different types of solar cells (SC) are…

Applied Physics · Physics 2019-08-02 Ali Imran , Deborah Eric , Muhammad Noaman Zahid , Muhammad Yousaf

Recombination losses contribute to reduce $J_{SC}$, $V_{OC}$ and the fill factor of organic solar cells. Recent advances in non-fullerene organic photovoltaics have shown, nonetheless, that efficient charge generation can occur under small…

Materials Science · Physics 2022-11-24 Artur M. Andermann , Luis G. C. Rego

State of the art organic solar cells exhibit power conversion efficiencies of 18 % and above. These devices benefit from the suppression of free charge recombination with regard to the Langevin-limit of charge encounter in a homogeneous…

Applied Physics · Physics 2021-12-24 Guangzheng Zuo , Safa Shoaee , Martijn Kemerink , Dieter Neher

Recombination of photogenerated charge carriers in polymer bulk heterojunction (BHJ) solar cells reduces the short circuit current (Jsc) and the fill factor (FF). Identifying the mechanism of recombination is, therefore, fundamentally…

Materials Science · Physics 2015-05-20 Sarah R. Cowan , Anshuman Roy , Alan J. Heeger

In a recent paper, Street et al. [Phys. Rev. B 81, 205307 (2010)] propose first order recombination due to interface states to be the dominant loss mechanism in organic bulk heterojunction solar cells, based on steady-state current--voltage…

Materials Science · Physics 2010-11-15 C. Deibel , A. Wagenpfahl

Fundamental electronic processes such as charge-carrier transport and recombination play a critical role in determining the efficiency of hybrid perovskite solar cells. The presence of mobile ions complicates the development of a clear…

Materials Science · Physics 2020-12-17 Sebastian Reichert , Katelyn Goetz , Christopher Wöpke , Yana Vaynzof , Carsten Deibel

The radiative recombination, Shokley-Read recombination, frontal-surface and rear-surface recombination and the recombination at the heterojunction boundaries and the recombination in the space charge region are considered in the…

Materials Science · Physics 2013-07-04 A. V. Sachenko , V. P. Kostylyov , N. P. Kulish , I. O. Sokolovskyi , A. I. Shkrebtii

A modified detailed balance model is built to understand and quantify efficiency loss of perovskite solar cells. The modified model captures the light-absorption dependent short-circuit current, contact and transport-layer modified carrier…

The power conversion efficiency of organic solar cells has recently improved beyond 20%. The active layers of these devices comprise of at least two organic semiconductors, forming a type II heterojunction. Hereby, the device performance is…

Materials Science · Physics 2026-01-22 Jonathan L. Langentepe-Kong , Manasi Pranav , Safa Shoaee , Dieter Neher

Apparent recombination orders exceeding the value of two expected for bimolecular recombination have been reported for organic solar cells in various publications. Two prominent explanations are bimolecular losses with a carrier…

Soft Condensed Matter · Physics 2012-08-23 D. Rauh , C. Deibel , V. Dyakonov

Modeling the charge-generation process is highly important to understand device physics and optimize power conversion efficiency of bulk-heterojunction (BHJ) organic solar cells (OSCs). Free carriers are generated by both ultrafast exciton…

Mesoscale and Nanoscale Physics · Physics 2016-12-06 Zi Shuai Wang , Wei E. I. Sha , Wallace C. H. Choy

The physics of organic bulk heterojunction solar cells is studied within a six state model, which is used to analyze the factors that affect current-voltage characteristics, power-voltage properties and efficiency, and their dependence on…

Materials Science · Physics 2015-06-18 Mario Einax , Marcel Dierl , Philip R. Schiff , Abraham Nitzan

We investigate nongeminate recombination in organic solar cells based on copper phthalocyanine (CuPc) and C$_{60}$. Two device architectures, the planar heterojunction (PHJ) and the bulk heterojunction (BHJ), are directly compared in view…

Applied Physics · Physics 2021-06-21 A. Foertig , A. Wagenpfahl , T. Gerbich , D. Cheyns , V. Dyakonov , C. Deibel

The theoretical effects of phase separation on encounter-limited charge carrier recombination in organic semiconductor blends are investigated using kinetic Monte Carlo (KMC) simulations of pump-probe experiments. Using model bulk…

Materials Science · Physics 2015-04-06 Michael C. Heiber , Christoph Baumbach , Vladimir Dyakonov , Carsten Deibel

We studied the recombination dynamics of charge carriers in organic bulk heterojunction solar cells made of the blend system poly(2,5-bis(3-dodecyl thiophen-2-yl) thieno[2,3-b]thiophene) (pBTCT-C12):[6,6]-phenyl-C61-butyric acid methyl…

Organic heterojunction solar cells are analyzed within a minimal model that includes the essential physical features of such systems. The dynamical properties of this model, calculated using a master equation approach, account for the…

Materials Science · Physics 2011-11-11 Mario Einax , Marcel Dierl , Abraham Nitzan

The fill factor (FF) is a critical parameter for solar cell efficiency, but its analytical description is challenging due to the interplay between recombination and charge extraction processes. An often overlooked yet significant factor…

Materials Science · Physics 2025-02-18 Maria Saladina , Carsten Deibel
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