Related papers: On the "viscosity maximum" during the uniaxial ext…
Nonlinear extensional flows are common in polymer processing but remain challenging theoretically because dramatic stretching of chains deforms the entanglement network far from equilibrium. Here, we present coarse-grained simulations of…
Simulations of undulatory swimming in viscoelastic fluids with large amplitude gaits show concentration of polymer elastic stress at the tips of the swimmers.We use a series of related theoretical investigations to probe the origin of these…
In Part I of this paper [Haward et al. submitted (2023)], we presented a new three-dimensional microfluidic device (the optimized uniaxial and biaxial extensional rheometer, OUBER) for generating near-homogeneous uniaxial and biaxial…
Viscosity overshoot of entangled polymer melts has been observed under shear flow and uniaxial elongational flow, but has never been observed under biaxial elongational flow. We confirmed the presence of viscosity overshoot under biaxial…
Here we present an experimentally practical and robust method to compute the transient extensional viscosity from exponential shear on a wide variety of viscoelastic complex fluids. To achieve this, we derive an analytical, frame-invariant…
An experimental investigation of the impact of sample inhomogeneity on measurements of the linear elongational viscosity of two low-density polyethelenes is presented. A novel method of in-situ measurements of the diameter of samples under…
The viscoelastic behavior of liquid polymers changes depending on the microstructure of the polymer chains. To investigate the unsteady structural changes induced by polymer chain morphology under stress, we develop a simple rheo-optical…
We investigate freely expanding liquid sheets made of either simple Newtonian fluids or solutions of high molecular water-soluble polymer chains. A sheet is produced by the impact of a drop on a quartz plate covered with a thin layer of…
Building off recent advances on how to practically use exponential shear in a torsional rheometer to compute transient planar extensional viscosity (Kroo et al. 2025a), we extend the technique to cyclic tensile measurements in complex…
We investigate previously unclarified effects of fluid elasticity on shear-thickening in dilute suspensions in an Oldroyd-B viscoelastic fluid using a novel direct numerical simulation based on the smoothed profile method. Fluid elasticity…
The measurement of interfacial mechanical or rheological properties in polymer blends is a challenging task, as well as providing a quantitative link between these properties and the interfacial nanostructure. Here, we perform a systematic…
This study presents an experimental framework for large amplitude oscillatory extension (LAOE) to investigate nonlinear material properties of complex fluids. Using a microfluidic optimized shape cross-slot extensional rheometer, we…
We give the first correction to the suspension viscosity due to fluid elasticity for a dilute suspension of spheres in a viscoelastic medium. Our perturbation theory is valid to $O(\phi\mathrm{Wi}^2)$ in the Weissenberg number…
This paper investigates the relationship between extensional and shear viscosity of low-viscosity power-law fluids. We show the first experimental evidence of the conditions satisfying the same power exponents for extensional and shear…
The extensional rheology of dilute suspensions of spheres in viscoelastic or polymeric liquids is studied computationally. At low polymer concentration (c) and Deborah number (De), a wake of highly stretched polymers forms downstream of the…
We model within the framework of finite elasticity two inherent instabilities observed in liquid crystal elastomers under uniaxial tension. First is necking which occurs when a material sample suddenly elongates more in a small region where…
We investigate the wrinkling dynamics of an elastic filament immersed in a viscous fluid submitted to compression at a finite rate with experiments and by combining geometric nonlinearities, elasticity, and slender body theory. The drag…
The present study proposes a novel full-field extensional rheo-optical technique to investigate the relationship between the rheological properties and internal structural deformation of complex fluids under uniaxial extensional flow.…
Minimally invasive experimental methods that can measure local rate dependent mechanical properties are essential in understanding the behaviour of soft and biological materials in a wide range of applications. Needle based measurement…
The dewetting dynamics of ultrathin polymer films, e.g. in the model system of polystyrene on a polydimethylsiloxane-covered substrate, exhibits interesting behavior like a fast decay of the dewetting velocity and a maximum in the width of…