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A detailed study of the structural and magnetic properties of a spin-$5/2$ triangular lattice antiferromagnet RbFe(HPO$_{3}$)$_{2}$ is presented using x-ray diffraction, magnetization, heat capacity, and $^{31}$P nuclear magnetic resonance…

Materials Science · Physics 2025-11-24 V. Nagpal , Sebin J. Sebastian , Surya P. Patra , S. Shibash , Q. -P. Ding , Y. Furukawa , R. Nath

The spiral magnetic structure and underlying spin lattice of BiMnFe2O6 are investigated by low-temperature neutron powder diffraction and density functional theory band structure calculations. In spite of the random distribution of the Mn3+…

New frustrated antiferromagnetic compounds CuRE2Ge2O8 (RE=Pr, Nd, Sm, Eu) have been investigated using high-resolution x-ray diffraction, magnetic and heat capacity measurements. These systems show different magnetic lattices depending on…

Strongly Correlated Electrons · Physics 2017-12-27 Hwanbeom Cho , Marie Kratochvilova , Nahyun Lee , Hasung Sim , Je-Geun Park

In the context of magnetism, frustration arises when a group of spins cannot find a configuration that minimizes all of their pairwise interactions simultaneously. We consider the effects of the geometric frustration that arises in a…

Statistical Mechanics · Physics 2015-05-19 A. Jagannathan , B. Motz , E. Vedmedenko

Neutron scattering experiment on NiS2 single crystal revealed a honeycomb pattern of the intensity distribution in reciprocal lattice space (continuous-line structure along the fcc zone boundary) providing the first direct evidence for…

Strongly Correlated Electrons · Physics 2007-05-23 M. Matsuura , Y. Endoh , H. Hiraka , K. Yamada , K. Hirota , A. S. Mishchenko , N. Nagaosa , I. V. Solovyev

A new crystal chemical method was used to calculate the sign and strength not only of the nearest-neighbor (NN)interactions, but also of the next-nearest-neighbor (NNN) ones in tetragonal compounds Zn2(VO)(PO4)2 (I),(VO)(H2PO4)2 (II),…

Materials Science · Physics 2007-05-23 L. M. Volkova , S. A. Polyshchuk

Magnetic frustration, which is well-defined in insulating systems with localized magnetic moments, yields exotic ground states like spin ices, spin glasses, or spin liquids. In metals magnetic frustration is less well defined because of the…

A new type of magnetically frustrated lattice is found in the layered fluoride NaBa2Mn3F11. A kagome-type array of regular triangles composed of Mn2+ ions (spin 5/2) deforms so as to generate the next-nearest-neighbor interaction J2 between…

Materials Science · Physics 2014-03-11 Hajime Ishikawa , Tsuyoshi Okubo , Yoshihiko Okamoto , Zenji Hiroi

We report magnetization and specific heat measurements on polycrystalline samples of BaCdVO(PO_4)_2 and show that this compound is a S=1/2 frustrated square lattice with ferromagnetic nearest-neighbor (J_1) and antiferromagnetic…

Strongly Correlated Electrons · Physics 2008-08-26 R. Nath , A. A. Tsirlin , H. Rosner , C. Geibel

Spin-frustrated systems are one avenue for inducing macroscopic quantum states in materials. However, experimental realization of this goal has been difficult because of the lack of simple materials and, if available, the separation of the…

Strongly Correlated Electrons · Physics 2010-04-07 S. Chu , T. M. McQueen , R. Chisnell , D. E. Freedman , P. Müller , Y. S. Lee , D. G. Nocera

Magnetic frustration is a route that can lead to the emergence of novel ground states, including spin liquids and spin ices. Such frustration can be introduced through either the geometry of lattice structures or by incompatible exchange…

Motivated by the recent discoveries of some compounds such as the $\mathrm{Bi}_{2}\mathrm{Fe}_{4}\mathrm{O}_{9}$ which crystallizes in an orthorhombic crystal structure with the $\mathrm{Fe}^{3+}$ ions, and iron-based oxyfluoride ${\rm…

Strongly Correlated Electrons · Physics 2017-03-03 F. C. Rodrigues , S. M. de Souza , Onofre Rojas

The layered compound with distorted Kagome nets, Dy3Ru4Al12, was previously reported to undergo antiferromagnetic ordering below (TN=) 7 K, based on investigations on single crystals. Here, we report the results of our investigation of ac…

Strongly Correlated Electrons · Physics 2016-05-05 Venkatesh Chandragiri , Kartik K Iyer , E. V. Sampathkumaran

The spinels CoB$_2$O$_4$ with magnetic Co$^{2+}$ ions on the diamond lattice A site can be frustrated because of competing near-neighbor ($J_1$) and next-near neighbor ($J_2$) interactions. Here we describe attempts to tune the relative…

Kondo metals with geometric frustration offer fertile ground for exploring exotic states of matter with a field-induced fractional magnetization platform and nonsaturating magnetoresistance. Herein, a Ce3ScBi5 single crystal with…

Strongly Correlated Electrons · Physics 2025-11-14 Zhongchen Xu , Yaxian Wang , Cuiwei Zhang , Hongxiong Liu , Xin Han , Liusuo Wu , Xianmin Zhang , Quansheng Wu , Youguo Shi

Incommensurate magnetic order in the spin-3/2 antiferromagnet Na$_3$RuO$_4$ is uncovered by neutron diffraction combined with ab initio calculations. The crystal structure of Na$_3$RuO$_4$ contains two triangular motifs on different length…

Strongly Correlated Electrons · Physics 2023-10-23 Vera P. Bader , Clemens Ritter , Elias Papke , Philipp Gegenwart , Alexander A. Tsirlin

We have identified TbOF as a unique frustrated and mixed-anion lattice, hosting unconventional magnetism. By means of magnetization, specific heat and neutron diffraction measurements down to 90 mK, as well as DFT calculations, we present a…

We synthesized a quasi-two-dimensional distorted triangular lattice antiferromagnet Ca$_3$CoNb$_2$O$_9$, in which the effective spin of Co$^{2+}$ is 1/2 at low temperatures, whose magnetic properties were studied by dc susceptibility and…

Strongly Correlated Electrons · Physics 2015-12-25 J. Dai , P. Zhou , P. S. Wang , F. Pang , T J. Munsie , G. M. Luke , J. S. Zhang , Weiqiang Yu

The phenomenon of frustration, which gives rise to many fascinating phenomena, is conventionally associated with the topology of non-bipartite lattices, where nearest-neighbor (nn) interactions and global connectivity compete in the…

Strongly Correlated Electrons · Physics 2009-11-11 J. Kunes , W. E. Pickett

Structural and magnetic properties of a two-dimensional spin-$\frac{5}{2}$ frustrated triangular lattice antiferromagnet NH$_{4}$Fe(PO$_{3}$F)$_2$ are explored via x-ray diffraction, magnetic susceptibility, high-field magnetization, heat…

Materials Science · Physics 2025-02-11 S. Mohanty , K. M. Ranjith , C. S. Saramgi , Y. Skourski , B. Büchner , H. -J. Grafe , R. Nath