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Screening due to surrounding dielectric medium reshapes the electron-hole interaction potential and plays a pivotal role in deciding the binding energies of strongly bound exciton complexes in quantum confined monolayers of transition metal…

Mesoscale and Nanoscale Physics · Physics 2017-08-16 Garima Gupta , Sangeeth Kallatt , Kausik Majumdar

We report on the charge dynamics of Ta$_2$Pd$_3$Te$_5$ using temperature-dependent optical spectroscopy with polarized light. We observe a metal-insulator transition characterized by the collapse of Drude response and the emergence of sharp…

1T-TiSe2 is one of the most studied charge density wave (CDW) systems, not only because of its peculiar properties related to the CDW transition, but also due to its status as a promising candidate of exciton insulator signaled by the…

A new state of matter, an excitonic insulator (EI) state, was predicted to emerge from Bose-Einstein condensation of electron-hole pairs. Some candidate materials were suggested but it has been elusive to confirm its existence. Recent works…

Strongly Correlated Electrons · Physics 2021-05-12 Jin Mo Bok , Jungseek Hwang , Han-Yong Choi

With decreasing density $n_s$ the thermopower $S$ of a low-disorder 2D electron system in silicon is found to exhibit a sharp increase by more than an order of magnitude, tending to a divergence at a finite, disorder-independent density…

Strongly Correlated Electrons · Physics 2015-06-03 A. Mokashi , S. Li , Bo Wen , S. V. Kravchenko , A. A. Shashkin , V. T. Dolgopolov , M. P. Sarachik

We study theoretically the effect of the fermion and boson densities on the superconductivity transition critical temperature $(T_c)$ of a two dimensional electron gas (2DEG), where superconductivity is mediated by a Bose-Einstein…

Superconductivity · Physics 2014-10-15 E. D. Cherotchenko , T. Espinosa-Ortega , A. V. Nalitov , I. A. Shelykh , A. V. Kavokin

The spontaneous condensation of excitons in the excitonic insulating phase has been reported in Ta$_2$NiSe$_5$ below 325 K. In this context, we present the temperature-dependent optical pump optical probe spectroscopy of Ta$_2$NiSe$_5$,…

Materials Science · Physics 2024-12-02 Vikas Arora , Sukanya Pal , Luminita Harnagea , D. V. S. Muthu , A K Sood

The ultrafast electronic structures of the charge density wave material 1T-TiSe$_2$ were investigated by high-resolution time- and angle-resolved photoemission spectroscopy. We found that the quasiparticle populations drove ultrafast…

Strongly Correlated Electrons · Physics 2023-06-02 Shaofeng Duan , Wei Xia , Chaozhi Huang , Shichong Wang , Lingxiao Gu , Haoran Liu , Dao Xiang , Dong Qian , Yanfeng Guo , Wentao Zhang

Using a high-resolution differential technique we have determined the electronic specific heat coefficient gamma(T) of Ba1-xKxFe2As2 with x=0 to 1.0, at temperatures (T) from 2K to 380K and in magnetic fields H=0 to 13T. In the normal state…

Superconductivity · Physics 2013-10-15 J. G. Storey , J. W. Loram , J. R. Cooper , Z. Bukowski , J. Karpinski

The controversy regarding the precise nature of the high-temperature phase of 1T-TiSe2 lasts for decades. It has intensified in recent times when new evidence for the excitonic origin of the low-temperature charge-density wave state started…

The strong electron-electron interaction in transition metal dichalcogenides (TMDs) gives rise to phenomena such as strong exciton and trion binding and excitonic condensation, as well as large negative exchange and correlation…

Femtosecond time-resolved core-level photoemission spectroscopy with a free-electron laser is used to measure the atomic-site specific charge-order dynamics in the charge-density-wave/Mott insulator 1T-TaS2. After strong photoexcitation, a…

Measuring terahertz (THz) conductivity on an ultrafast time scale is an excellent way to observe charge-carrier dynamics in semiconductors as a function of time after photoexcitation. However, a conductivity measurement alone cannot…

Utilizing the unbiased time-dependent density-matrix renormalization group technique, we examine the photoemission spectra in the extended Falicov-Kimball model at zero and finite temperatures, particularly with regard to the excitonic…

Strongly Correlated Electrons · Physics 2021-03-31 Satoshi Ejima , Florian Lange , Holger Fehske

The energy spectrum of the conduction band in HgTe/Cd$_x$Hg$_{1-x}$Te quantum wells of a width $d=(4.6-20.2)$ nm has been experimentally studied in a wide range of electron density. For this purpose, the electron density dependence of the…

The excitonic insulator is an intriguing correlated electron phase formed of condensed excitons. A promising candidate is the small band gap semiconductor Ta2NiSe5. Here we investigate the quasiparticle and coherent phonon dynamics in…

Strongly Correlated Electrons · Physics 2018-08-01 Daniel Werdehausen , Tomohiro Takayama , Gelon Albrecht , Yangfan Lu , Hidenori Takagi , Stefan Kaiser

Using first-principles simulations combined with many-body calculations, we show that two-dimensional free-standing quintuple-layer Bi2Se2Te is an inversion symmetric monolayer expected to achieve spatially indirect exciton with large…

Materials Science · Physics 2024-07-18 Yuanyuan Wang , Ying Dai , Baibiao Huang , Yee Sin Ang , Wei Wei

We report high-resolution inelastic x-ray measurements of the soft phonon mode in the charge-density-wave compound TiSe$_2$. We observe a complete softening of a transverse optic phonon at the L point, i.e. q = (0.5, 0, 0.5), at T ~…

Strongly Correlated Electrons · Physics 2015-05-28 F. Weber , S. Rosenkranz , J. -P. Castellan , R. Osborn , G. Karapetrov , R. Hott , R. Heid , K. -P. Bohnen , A. Alatas

At low temperature TiSe2 undergoes a charge density wave instability. Superconductivity is stabilized either by pressure or by Cu intercalation. We show that the pressure phase diagram of TiSe2 is well described by first-principles…

Materials Science · Physics 2015-05-27 Matteo Calandra , Francesco Mauri

Excitons are bosonic quasiparticles with a variety of applications in optoelectronics, photosyn thesis, and dissipationless informatics, and their lifetime can become sufficiently long to form a quantum condensate. While exciton…

Strongly Correlated Electrons · Physics 2025-07-23 Siwon Lee , Kyung-Hwan Jin , SeongJin Kwon , Hyunjin Jung , Choongjae Won , Sang-Wook Cheong , Gil Young Cho , Jaeyoung Kim , Han Woong Yeom