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Using a valence force field model based on that introduced by Martin, we present three related methods through which we analytically determine valence force field parameters. The methods introduced allow easy derivation of valence force…

Materials Science · Physics 2019-10-09 Daniel S. P. Tanner , Miguel A. Caro , Stefan Schulz , Eoin P. O'Reilly

In the present work we have proposed the method that allows one to easily estimate hardness and bulk modulus of known or hypothetical solid phases from the data on Gibbs energy of atomization of the elements and corresponding covalent…

Materials Science · Physics 2011-02-08 Vladimir A. Mukhanov , Oleksandr O. Kurakevych , Vladimir L. Solozhenko

We demonstrate the possibility in quantifying the Raman intensities for both specimen and substrate layers in a common stacked experimental configuration and, consequently, propose a general and rapid thickness identification technique for…

Mesoscale and Nanoscale Physics · Physics 2013-08-20 Song-Lin Li , Hisao Miyazaki , Haisheng Song , Hiromi Kuramochi , Shu Nakaharai , Kazuhito Tsukagoshi

Two-dimensional (2D) layered materials have been extensively studied owing to their fascinating and technologically relevant properties. Their functionalities can be often tailored by the interlayer stacking pattern. Low-frequency (LF)…

Mesoscale and Nanoscale Physics · Physics 2017-10-06 Liangbo Liang , Alexander A. Puretzky , Bobby G. Sumpter , Vincent Meunier

Fracture toughness $K_{IC}$ plays an important role in materials design. Along with numerous experimental methods to measure fracture toughness of materials, its understanding and theoretical prediction is very important. However,…

Materials Science · Physics 2019-03-27 Haiyang Niu , Shiwei Niu , Artem R. Oganov

In chemical processing and bioprocessing, conventional online sensors are limited to measure only basic process variables like pressure and temperature, pH, dissolved O and CO$_2$ and viable cell density (VCD). The concentration of other…

Quantitative Methods · Quantitative Biology 2020-05-07 Semion Rozov

Raman spectroscopy is a widely used, powerful, and nondestructive tool for studying the vibrational properties of bulk and low-dimensional materials. Raman spectra can be simulated using first-principles methods, but due to the high…

Materials Science · Physics 2019-03-06 Arsalan Hashemi , Arkady V. Krasheninnikov , Martti Puska , Hannu-Pekka Komsa

For many materials, Raman spectra are intricately structured and provide valuable information about compositional stoichiometry and crystal quality. Here we use density-functional theory calculations, mass approximation, and the Raman…

Materials Science · Physics 2024-09-04 Nima Ghafari Cherati , I. Abdolhosseini Sarsari , Arsalan Hashemi , Tapio Ala-Nissila

Recently, two unusual features were theoretically predicted for the Raman response of out-of-plane phonons in magnetic two-dimensional materials hosting massive Dirac fermions. First, the phase difference between certain Raman tensor…

Materials Science · Physics 2026-03-17 Selçuk Parlak , Abhishek Kumar , Runhan Li , Maia G. Vergniory , Ion Garate

Transient absorption and Raman scattering measurements on noble metal nanoparticles offer complimentary information on their vibrational modes and mechanical interactions with their surroundings. We have developed a comprehensive modeling…

Mesoscale and Nanoscale Physics · Physics 2024-10-29 Rachel Gelfand , Matthew Pelton

The way atoms attach to each other defines the function(s), e.g., mechanical, optical, electronic, of a given material. The nature of the chemical bond is, therefore, one of the most fundamental issues in materials. Both ionic interactions,…

Materials Science · Physics 2019-07-10 Yevgeny Rakita , Thomas Kirchartz , Gary Hodes , David Cahen

By performing density functional theory-based ab-initio calculations, Raman active phonon modes of novel single-layer two-dimensional (2D) materials and the effect of in-plane biaxial strain on the peak frequencies and corresponding…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 M. Yagmurcukardes , C. Bacaksiz , E. Unsal , B. Akbali , R. T. Senger , H. Sahin

The bremsstrahlung cross section for relativistic electrons in a crystal is split into the sum of coherent and incoherent parts (the last is due to a thermal motion of atoms in the crystal). Although the spectrum of incoherent radiation in…

Accelerator Physics · Physics 2010-06-04 N. F. Shul'ga , V. V. Syshchenko , A. I. Tarnovsky

A consistent calculation of resonant inelastic (Raman) scattering amplitudes for relatively large quantum dots, which takes account of valence-band mixing, discrete character of the spectrum in intermediate and final states, and…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Alain Delgado , Augusto Gonzalez

We introduce a computational approach to estimate the hardness and stiffness of diamond surfaces and nanoparticles by studying their elastic response to atomic nanoindentation. Results of our ab initio density functional calculations…

Mesoscale and Nanoscale Physics · Physics 2020-02-28 Alexander Quandt , Igor Popov , David Tománek

Lattice vibration frequencies are related to many important materials properties such as thermal and electrical conductivity as well as superconductivity. However, computational calculation of vibration frequencies using density functional…

Materials Science · Physics 2021-11-12 Nghia Nguyen , Steph-Yves Louis , Lai Wei , Kamal Choudhary , Ming Hu , Jianjun Hu

Low-frequency Raman and inelastic neutron scattering of amorphous bis-phenol A polycarbonate is measured at low temperature, and compared. The vibrational density of states and light-vibration coupling coefficient are determined. The…

Disordered Systems and Neural Networks · Physics 2009-10-31 L. Saviot , E. Duval , J. F. Jal , A. J. Dianoux

The vibrational properties of ErTe$_3$ were investigated using Raman spectroscopy and analyzed on the basis of peculiarities of the RTe$_3$ crystal structure. Four Raman active modes for the undistorted structure, predicted by factor-group…

Strongly Correlated Electrons · Physics 2011-01-31 N. Lazarević , Z. V. Popović , Rongwei Hu , C. Petrovic

Coherent Raman scattering provides highly sensitive vibrational analysis through nonlinear light-matter interactions. However, its application to metal interfaces has remained challenging because the intrinsically large non-resonant…

Lattice structure and symmetry of two-dimensional (2D) layered materials are of key importance to their fundamental mechanical, thermal, electronic and optical properties. Raman spectroscopy, as a convenient and nondestructive tool, however…

Mesoscale and Nanoscale Physics · Physics 2015-08-28 Yanqing Feng , Wei Zhou , Yaojia Wang , Jian Zhou , Erfu Liu , Yajun Fu , Zhenhua Ni , Xinglong Wu , Hongtao Yuan , Feng Miao , Baigeng Wang , Xiangang Wan , Dingyu Xing
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