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Neutron scattering studies on powder and single crystals have provided new evidences for unconventional magnetism in Cu2Te2O5Cl2. The compound is built from tetrahedral clusters of S=1/2 Cu2+ spins located on a tetragonal lattice. Magnetic…

Strongly Correlated Electrons · Physics 2009-11-11 O. Zaharko , H. M. Ronnow , A. Daoud-Aladine , S. Streule , F. Juranyi , J. Mesot , H. Berger , P. J. Brown

The magnetic structure of honeycomb iridate Na$_2$IrO$_3$ is of paramount importance to its exotic properties. The magnetic order is established experimentally to be zigzag antiferromagnetic. However, the previous assignment of ordered…

Materials Science · Physics 2015-10-20 Kaige Hu , Fa Wang , Ji Feng

We report a neutron scattering study of the metallic triangular lattice antiferromagnet PdCrO$_2$. Powder neutron diffraction measurements confirm that the crystalline space group symmetry remains $R\bar{3}m$ below $T_N$. This implies that…

The tetragonal copper oxide Bi$_2$CuO$_4$ has an unusual crystal structure with a three-dimensional network of well separated CuO$_4$ plaquettes. This material was recently predicted to host electronic excitations with an unconventional…

Strongly Correlated Electrons · Physics 2017-08-23 L. Zhao , H. Guo , W. Schmidt , K. Nemkovski , M. Mostovoy , A. C. Komarek

Magnetic properties of a quasi one-dimensional magnet CuV_2O_6 have been studied by means of susceptibility measurement, NMR and powder neutron diffraction. Cu^{2+} spins (S=1/2) order antiferromagnetically below 22.6 K, and the saturation…

Strongly Correlated Electrons · Physics 2009-10-31 Jun Kikuchi , Kazuhiro Ishiguchi , Kiyoichiro Motoya , Masayuki Itoh , Kazunori Inari , Naotoshi Eguchi , Jun Akimitsu

Dynamic spin correlation function of the $S=1/2$ antiferromagnetic spin chain with alternating nearest neighbor and competing next nearest neighbor interactions is studied using the numerical diagonalization method. We find characteristics…

Condensed Matter · Physics 2009-10-31 Shigeyoshi Mori , Isao Harada , Takashi Tonegawa

We report magnetic susceptibility, specific heat and muon spin relaxation (muSR) experiments on the triangular antiferromagnet La2Ca2MnO7 which develops a genuine two-dimensional, three-sublattice \sqrt{3} \times \sqrt{3} magnetic order…

Strongly Correlated Electrons · Physics 2015-07-08 P. Dalmas de Réotier , C. Marin , A. Yaouanc , T. Douce , A. Sikora , A. Amato , C. Baines

The spin dynamics and magnetic excitations of the slightly distorted triangular s = 3/2 system alpha-CaCr2O4 are investigated by means of Raman spectroscopy and electron spin resonance (ESR) to elucidate its peculiar magnetic properties.…

We study the spin dynamics of classical Heisenberg antiferromagnet with nearest neighbor interactions on a quasi-two-dimensional kagome bilayer. This geometrically frustrated lattice consists of two kagome layers connected by a…

Strongly Correlated Electrons · Physics 2021-06-09 Preetha Saha , Depei Zhang , Seung-Hun Lee , Gia-Wei Chern

We report a neutron scattering study of the spin correlations for the spin 5/2, two-dimensional antiferromagnet Rb_2MnF_4 in an external magnetic field. Choosing fields near the system's bicritical point, we tune the effective anisotropy in…

Strongly Correlated Electrons · Physics 2009-10-31 R. L. Leheny , R. J. Christianson , R. J. Birgeneau , R. W. Erwin

The entire magnetic phase diagram of the quasi two dimensional (2D) magnet on a distorted triangular lattice KFe(MoO4)2 is outlined by means of magnetization, specific heat, and neutron diffraction measurements. It is found that the spin…

Investigation of dynamical excitations is difficult but crucial to the understanding of many exotic quantum phenomena discovered in quantum materials. This is particularly true for highly frustrated quantum antiferromagnets whose dynamical…

Strongly Correlated Electrons · Physics 2022-11-24 Run-Ze Chi , Yang Liu , Yuan Wan , Hai-Jun Liao , T. Xiang

Accurate ab initio calculations on embedded Cu_4O_{12} square clusters, fragments of the La_2CuO_4 lattice, confirm a value of the nearest neighbor antiferromagnetic coupling (J=124 meV) previously obtained from ab initio calculations on…

Strongly Correlated Electrons · Physics 2009-10-31 Carmen J. Calzado , Jean-Paul Malrieu

Neutron scattering studies and measurements of the dielectric susceptibility and ferroelectric polarization P have been carried out in various magnetic fields H for single-crystal samples of the multiferroic system LiVCuO4 with quasi…

Strongly Correlated Electrons · Physics 2015-05-13 Yukio Yasui , Yutaka Naito , Kenji Sato , Taketo Moyoshi , Masatoshi Sato* , Kazuhisa Kakurai

Inelastic neutron scattering measurements on the itinerant antiferromagnet (AFM) CaCo$_{\mathrm{2}-y}$As$_{2}$ at a temperature of 8 K reveal two orthogonal planes of scattering perpendicular to the Co square lattice in reciprocal space,…

The $A$MnO$_{2}$ delafossites ($A$=Na, Cu), are model frustrated antiferromagnets, with triangular layers of Mn$^{3+}$~spins. At low temperatures ($T_{N}$=65 K), a $C2/m \rightarrow P\overline{1}$ transition is found in CuMnO$_2$, which…

Here we report a study of the spin dynamics in the ferromagnetic chain compound $Li_{2}CuO_{2}$. Inelastic neutron scattering measurements allow for the spin Hamiltonian to be determined using a $J_{1}-J_{2}$ $XXZ$-Heisenberg spin chain…

Strongly Correlated Electrons · Physics 2023-08-10 Eli Zoghlin , Matthew B. Stone , Stephen D. Wilson

Spin-driven multiferroics exhibit strong magnetoelectric coupling, with notable polarization changes under a magnetic field, but these effects are usually limited to high-Z magnetic insulators with low electronic polarization. In this work,…

Materials Science · Physics 2024-12-31 Ranquan Cao , Ruizhi Dong , Ruixiang Fei , Yugui Yao

The minerals A2Cu3O(SO4)3 (A2=Na2, NaK, K2) constitute quantum spin systems with copper hexamers as basic structural units. Strong intra-hexamer spin couplings give rise to an effective triplet ground-state. Weak inter-hexamer spin…

Strongly Correlated Electrons · Physics 2021-12-06 A. Furrer , A. Podlesnyak , E. Pomjakushina , V. Pomjakushin

We report a comprehensive neutron scattering study of low energy magnetic excitations in the breathing pyrochlore helimagnetic $\text{Cu}_2\text{OSeO}_3$. Fully documenting the four lowest energy magnetic modes that leave the ferrimagnetic…