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Luminescence of surface and free bulk excitons is detected in xenon for the first time for substrate-free rare-gas clusters. Xenon clusters were produced by the method of gas condensation in a supersonic jet emitted into vacuum. Optical…

Atomic and Molecular Clusters · Physics 2015-06-26 O. G. Danylchenko , Yu. S. Doronin , S. I. Kovalenko , M. Yu. Libin , V. N. Samovarov , V. L. Vakula

Cathodoluminescence spectra of free xenon clusters produced by condensation of xenon-argon gas mixtures in supersonic jets expanding into vacuum were studied. By varying initial experimental parameters, including xenon concentration, we…

Atomic and Molecular Clusters · Physics 2011-07-27 O. G. Danylchenko , Yu. S. Doronin , S. I. Kovalenko , M. Yu. Libin , V. N. Samovarov , V. L. Vakula

In this paper, electron diffraction and optical methods are used together for the first time to study the problem of phase equilibrium in binary clusters of heavy rare gases. For the argon-xenon system, a new effect of its decay into pure…

Atomic and Molecular Clusters · Physics 2007-05-23 O. G. Danylchenko , Yu. S. Doronin , S. I. Kovalenko , V. N. Samovarov

We propose a new approach to analysis of cathodoluminescence spectra of substrate-free nanoclusters of argon produced in a supersonic jet expanding into a vacuum. It is employed to analyze intensities of the luminescence bands of neutral…

Atomic and Molecular Clusters · Physics 2016-01-28 Yu. S. Doronin , V. L. Vakula , G. V. Kamarchuk , A. A. Tkachenko , V. N. Samovarov

The strong excitonic emission at 5.75 eV of hexagonal boron nitride (h-BN) makes this material one of the most promising candidate for light emitting devices in the far ultraviolet (UV). However, single excitons occur only in perfect…

The absorption and emission spectra of silicon nanocrystals up to 1 nm diameter including geometry optimization and the many-body effects induced by the creation of an electron-hole pair have been calculated within a first-principles…

The near- and far-field photoluminescence spectra of a gated two-dimensional electron gas have been measured. Spatial fluctuations in the electron density are found to be manifested as spatial fluctuations in the emission amplitude of the…

Condensed Matter · Physics 2009-10-31 Y. Yayon , M. Rappaport , V. Umansky , I. Bar-Joseph

Electron--impact excitation of Xe atoms in pure Xe gas and in a Xe(10 %)--Ar(90 %) mixture has led to the discovery of infrared (IR) luminescence of Xe$_{2}$ excimers. The investigation of the emission spectrum at low gas density has…

Atomic Physics · Physics 2009-11-13 A. F. Borghesani , G. Carugno , I. Mogentale

We demonstrate spontaneous formation of a nonlinear vortex cluster state in a microcavity exciton-polariton condensate with time-periodic sign flipping of its topological charges at the GHz scale. When optically pumped with a ring-shaped…

Mesoscale and Nanoscale Physics · Physics 2022-06-22 Kirill A. Sitnik , Sergey Alyatkin , Julian D. Töpfer , Ivan Gnusov , Tamsin Cookson , Helgi Sigurdsson , Pavlos G. Lagoudakis

Any distortion of a chemical structure causes new features to appear in the absorption spectrum of the structure, especially in the visible and near UV (see Paper I). Chemical modeling, using molecular orbital theory, showed that the…

Astrophysics of Galaxies · Physics 2020-01-09 Renaud Papoular

Optical excitations in hexagonal nanonetwork materials, for example, Boron-Nitride (BN) sheets and nanotubes, are investigated theoretically. A permanent electric dipole moment, whose direction is from the B site to the N site, is…

Optics · Physics 2016-09-08 Kikuo Harigaya

Light emission from higher-order correlated excitonic states has been recently reported in hBN-encapsulated monolayer WSe2 and WS2 upon optical excitation. These exciton complexes are found to be bound states of excitons residing in…

Mesoscale and Nanoscale Physics · Physics 2019-04-19 Matthias Paur , Aday J. Molina-Mendoza , Rudolf Bratschitsch , Kenji Watanabe , Takashi Taniguchi , Thomas Mueller

The optical properties of particularly the tungsten-based transition-metal dichalcogenides are strongly influenced by the presence of dark excitons. Recently, theoretical predictions as well as indirect experimental insights have shown that…

Mesoscale and Nanoscale Physics · Physics 2019-12-25 Lorenz Maximilian Schneider , Shanece Esdaille , Daniel Rhodes , Katayun Barmak , James Hone , Arash Rahimi-Iman

The signature of defects in the optical spectra of hexagonal boron nitride (BN) is investigated using many body perturbation theory. A single BN-sheet serves as a model for different layered BN- nanostructures and crystals. In the sheet we…

Mesoscale and Nanoscale Physics · Physics 2011-05-03 C. Attaccalite , M. Bockstedte , A. Marini , A. Rubio , L. Wirtz

We theoretically study nonlinear optics of excitons under intense THz irradiation. In particular, the linear near infrared absorption and resonantly enhanced nonlinear sideband generation are described. We predict a rich structure in the…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Kristinn Johnsen , Antti-Pekka Jauho

A spectroscopic study of liquid argon from the vacuum ultraviolet at 110 nm to 1000 nm is presented. Excitation was performed using continuous and pulsed 12 keV electron beams. The emission is dominated by the analogue of the so called 2nd…

Instrumentation and Detectors · Physics 2015-11-25 T. Heindl , T. Dandl , M. Hofmann , R. Krücken , L. Oberauer , W. Potzel , J. Wieser , A. Ulrich

We consider a bilayer system of two-dimensional Bose-Einstein-condensed dipolar dark excitons (upper layer) and bright ones (bottom layer). We demonstrate that the interlayer interaction leads to a mixing between excitations from different…

Quantum Gases · Physics 2019-02-12 N. A. Asriyan , I. L. Kurbakov , A. K. Fedorov , Yu. E. Lozovik

The various decay mechanisms of excitons in cuprous oxide (Cu2O) are highly sensitive to defects which can relax selection rules. Here we report cryogenic hyperspectral imaging of exciton luminescence from cuprous oxide crystals grown via…

Noble gases provide tracers of cosmic provenance that are accessible to a future Uranus Atmospheric Probe. Argon and krypton are expected to be well-mixed on Uranus with respect to H$_2$ and He, although condensation at the winter pole may…

Earth and Planetary Astrophysics · Physics 2024-02-15 Kevin J Zahnle

Low-dimensional materials differ from their bulk counterpart in many respects. In particular, the screening of the Coulomb interaction is strongly reduced, which can have important consequences such as the significant increase of exciton…

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