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Equations of motion for weakly coupled excitonic complexes are derived. The description allows to treat the system in the basis of electronic states localized on individual chromophores, while at the same time accounting for experimentally…

Chemical Physics · Physics 2012-01-30 Tomas Mancal , Vytautas Balevicius , Leonas Valkunas

We show that the quantum coherent transfer of excitations between biomolecular chromophores is strongly influenced by spatial correlations of the environmental fluctuations. The latter are due either to propagating environmental modes or to…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 P. Nalbach , J. Eckel , M. Thorwart

We study the nature of the energy transfer process within a pair of coupled two-level systems (donor and acceptor) subject to interactions with the surrounding environment. Going beyond a standard weak-coupling approach, we derive a master…

Quantum Physics · Physics 2011-04-05 Dara P. S. McCutcheon , Ahsan Nazir

We investigate the weak-strong coupling transition of two linearly coupled systems under the influence of a phase fluctuating coupling. In the weak coupling regime the exponential decay of quantum properties is well known. A different…

Quantum Physics · Physics 2013-11-13 Dagoberto S. Freitas , M. C. Nemes

Recent observations of beating signals in the excitation energy transfer dynamics of photosynthetic complexes have been interpreted as evidence for sustained coherences that are sufficiently long-lived for energy transport and coherence to…

Quantum Physics · Physics 2013-03-05 A. W. Chin , J. Prior , R. Rosenbach , F. Caycedo-Soler , S. F. Huelga , M. B. Plenio

Fluctuations in the energy gap and coupling constants in and between chromophores can play important role in the absorption and energy transfer across a collection of two level systems. In a noisy environment, fluctuations can control…

Chemical Physics · Physics 2024-04-17 Rajesh Dutta , Biman Bagchi

Strong coupling between excitons and confined modes of light presents a promising pathway to tunable and enhanced energy transport in organic materials. By forming hybrid light-matter quasiparticles, exciton-polaritons, electronic…

Chemical Physics · Physics 2024-11-01 Niclas Krupp , Gerrit Groenhof , Oriol Vendrell

The theory of full counting statistics allows complete characterization of charge transport processes through nanoscale systems. The majority of existing theoretical treatments used to obtain the current cumulants rely on perturbative…

Mesoscale and Nanoscale Physics · Physics 2017-07-12 Richard Stones , Alexandra Olaya-Castro

Recent ultrafast optical experiments show that excitons in large biological light-harvesting complexes are coupled to molecular vibration modes. These high-frequency vibrations will not only affect the optical response, but also drive the…

Quantum Physics · Physics 2015-02-12 Arend G. Dijkstra , Chen Wang , Jianshu Cao , Graham R. Fleming

We give a theoretical treatment of the interaction of electronic excitations (excitons) in biomolecules and quantum dots with the surrounding polar solvent. Significant quantum decoherence occurs due to the interaction of the electric…

Soft Condensed Matter · Physics 2009-11-10 Joel Gilmore , Ross H. McKenzie

The interplay between an open quantum system and its environment can lead to both coherent and incoherent behaviour. We explore the extent to which strong coupling to a single bosonic mode can alter the coherence properties of a two-level…

Quantum Physics · Physics 2016-04-20 E. K. Levi , E. K. Irish , B. W. Lovett

Transfer and decay dynamics of an exciton coupled to a polarization vibration in a dimer is investigated in a mixed quantum-classical picture with the exciton decay incorporated by a sink site. Using a separation of time scales, it is…

Condensed Matter · Physics 2009-10-28 Holger Schanz , Ivan Barvik , Bernd Esser

Engineering and harnessing coherent excitonic transport in organic nanostructures has recently been suggested as a promising way towards improving man-made light harvesting materials. However, realising and testing the dissipative…

Quantum Physics · Physics 2018-06-19 A. W. Chin , E. Mangaud , O. Atabek , M. Desouter-Lecomte

We analyze the transport properties of a semiconductor based bilayer system under non-equilibrium conditions with special emphasis on the charge transfer statistics in the regime dominated by the exciton transport. We consider two different…

Mesoscale and Nanoscale Physics · Physics 2013-08-06 H. Soller , A. Komnik

We study the decoherence of a qubit weakly coupled to frustrated spin baths. We focus on spin-baths described by the classical Ising spin glass and the quantum random transverse Ising model which are known to have complex thermodynamic…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 E. A. Winograd , M. J. Rozenberg , R. Chitra

The dynamics of a dimer coupled to two different environments each in a spin star configuration under the influence of decoherence is studied. The exact analytical expression for the transition probability in the dimer system is obtained…

Quantum Physics · Physics 2014-01-15 I. Sinayskiy , A. Marais , F. Petruccione , A. Ekert

We consider an electrostatic qubit, interacting with a fluctuating charge of single electron transistor (SET) in the framework of exactly solvable model. The SET plays a role of the fluctuating environment affecting the qubit's parameters…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 S. A. Gurvitz , D. Mozyrsky

At low temperatures, indirect excitons formed at the in-plane electron-hole interface in a coupled quantum well structure undergo a spontaneous transition into a spatially modulated state. We report on the control of the instability…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Sen Yang , L. V. Butov , B. D. Simons , K. L. Campman , A. C. Gossard

Molecular exciton-polaritons exhibit long-range, ultrafast propagation, yet recent experiments have reported far slower propagation than expected. In this work, we implement a nonperturbative approach to quantify how static energetic…

Quantum Physics · Physics 2025-07-02 Gustavo J. R. Aroeira , Raphael F. Ribeiro

This article studies the decoherence induced on a system of two qubits by local interactions with a spin chain with nontrivial internal dynamics (governed by an XY Hamiltonian). Special attention is payed to the transition between two…

Quantum Physics · Physics 2013-05-29 Cecilia Cormick , Juan Pablo Paz
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