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The amplitude and phase of a material's nonlinear optical response provide insight into the underlying electronic dynamics that determine its optical properties. Phase-sensitive nonlinear spectroscopy techniques are widely implemented to…

Mesoscale and Nanoscale Physics · Physics 2018-07-12 Galan Moody , Corey McDonald , Ari Feldman , Todd Harvey , Richard P. Mirin , Kevin L. Silverman

The coherent modulation of electronic and vibrational nonlinearities in atoms and molecular gases by intense few-cycle pulses has been used for high-harmonic generation in the soft X-ray and attosecond regime, as well as for Raman frequency…

Materials Science · Physics 2013-09-16 Muneaki Hase , Masayuki Katsuragawa , Anca Monia Constantinescu , Hrvoje Petek

The consistent quantum theory of self-phase modulation (SPM) and cross-phase modulation (XPM) for ultrashort light pulses (USP) in medium with electronic Kerr-nonlinearity are developed. The approach makes use of momentum operator of…

Quantum Physics · Physics 2007-05-23 A. S. Chirkin , F. Popescu

We propose a method for implementing automated state transformations on single-photon multipath qudits encoded in a one-dimensional transverse spatial domain. It relies on transferring the encoding from this domain to the orthogonal one by…

Is it possible to modulate the inherent properties of a single light beam, namely amplitude, phase and polarization, simultaneously, by merely its phase? Here, we solve this scientific problem by unifying all these three properties of a…

Narrow line-widths and the possibility of enhanced spontaneous emission via coupling to microcavities make semiconductor quantum dots ideal for harnessing coherent quantum phenomena at the single photon level. So far, however, all…

Mesoscale and Nanoscale Physics · Physics 2007-07-26 A. Muller , E. B. Flagg , P. Bianucci , D. G. Deppe , W. Ma , J. Zhang , G. J. Salamo , C. K. Shih

Single photons in Laguerre-Gaussian (LG) beams, which carry orbital angular momentum (OAM), could enable more robust and efficient photonic quantum communication and information processing, as well as enhanced sensitivity in quantum…

Coherently driven semiconductor quantum dots are one of the most promising platforms for non-classical light sources and quantum logic gates which form the foundation of photonic quantum technologies. However, to date, coherent manipulation…

We present theoretical and experimental results showing the effects of incoherent population mixing on two-dimensional (2D) coherent excitation spectra that are measured via a time-integrated population and phase-sensitive detection. The…

Orbital Angular Momentum (OAM) modes are an important resource used in various branches of quantum science and technology due to their unique helical structure and countably infinite basis. Generating light that simultaneously carries…

Quantum Physics · Physics 2025-01-29 D. Scharwald , L. Gehse , P. R. Sharapova

Large quantum photonic systems hold promise for surpassing classical computational limits, yet their state preparation remains a challenge. We propose an alternative approach to study multiparticle dynamics by mapping the excitation mode of…

We propose a framework for designing coherent optical environments that enable versatile and dynamic optical manipulation. In contrast to conventional material-based near-field platforms, our approach employs a structured coherent light…

Optics · Physics 2025-10-07 Xiaoshu Zhao , Xu Yuan , Hongxia Zheng , Huajin Chen , Zhifang Lin

We have previously demonstrated that in the context of two-dimensional (2D) coherent electronic spectroscopy measured by phase modulation and phase-sensitive detection, an \emph{incoherent} nonlinear response, due to pairs of…

Spatial modulation microscopy is a technique originally developed for quantitative spectroscopy of individual nano-objects. Here, a parallel implementation of the spatial modulation microscopy technique is demonstrated based on a line…

Colloidal quantum dots (QDs) are an attractive medium for nonlinear optics and deterministic heterogeneous integration with photonic devices. Their intrinsic nonlinearities can be strengthened further by coupling QDs to low mode-volume…

The squeezed state is important in quantum metrology and quantum information. The most effective generation tool known is the optical parametric oscillator (OPO). Currently, only the squeezed states of lower-order spatial modes can be…

Quantum Physics · Physics 2020-04-22 Long Ma , Hui Guo , Hengxin Sun , Kui Liu , Bida Su , Jiangrui Gao

An optical transmitter irradiates a target region containing a bright thermal-noise bath in which a low-reflectivity object might be embedded. The light received from this region is used to decide whether the object is present or absent.…

The development of a quantum network relies on the advances of hybrid systems which includes ground to ground communication. However, the atmospheric turbulence of the environment poses a severe challenge to the optical quantum link. In…

Light's spatial properties represent an infinite state space, making it attractive for applications requiring high dimensionality, such as quantum mechanics and classical telecommunications, but also inherently spatial applications such as…

The possibility for controlling the probe-field optical gain and absorption switching and photon conversion by a surface-plasmon-polariton near field is explored for a quantum dot above the surface of a metal. In contrast to the linear…

Mesoscale and Nanoscale Physics · Physics 2023-07-19 Danhong Huang , Michelle Easter , Godfrey Gumbs , A. A. Maradudin , Shawn-Yu Lin , Dave Cardimona , Xiang Zhang
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