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Marcus theory famously predicts that electron-transfer rates decrease once the thermodynamic driving force exceeds the reorganization energy. Yet many systems instead exhibit Rehm-Weller kinetics, in which the rate saturates rather than…

Chemical Physics · Physics 2026-04-21 Ethan Abraham

In organic field effect transistors (FETs), charges move near the surface of an organic semiconductor, at the interface with a dielectric. In the past, the nature of the microscopic motion of charge carriers -that determines the device…

Materials Science · Physics 2015-06-25 I. N. Hulea , S. Fratini , H. Xie , C. L. Mulder , N. N. Iossad , G. Rastelli , S. Ciuchi , A. F. Morpurgo

Predicting the exact many-body quantum dynamics of polarons in materials with strong carrier-phonon interactions presents a fundamental challenge, often necessitating one to adopt approximations that sacrifice the ability to predict the…

Chemical Physics · Physics 2024-11-27 Srijan Bhattacharyya , Thomas Sayer , Andrés Montoya-Castillo

We theoretically study transport in two-dimensional semimetals. Typically, electron and hole puddles emerge in the transport layer of these systems due to smooth fluctuations in the potential. We calculate the electric response of the…

Mesoscale and Nanoscale Physics · Physics 2014-10-29 Michael Knap , Jay D. Sau , Bertrand I. Halperin , Eugene Demler

Superconductors connected to normal metallic electrodes at the nanoscale provide a potential source of non-locally entangled electron pairs. Such states would arise from Cooper pairs splitting into two electrons with opposite spins…

Mesoscale and Nanoscale Physics · Physics 2007-07-16 A. Levy Yeyati , F. S. Bergeret , A. Martin-Rodero , T. M. Klapwijk

Polaron is a composite quasiparticle derived from an excess carrier trapped by local lattice distortion, and it has been studied extensively for decades both theoretically and experimentally. However, atomic-scale creation and manipulation…

Mesoscale and Nanoscale Physics · Physics 2023-07-12 Huiru Liu , Aolei Wang , Ping Zhang , Chen Ma , Caiyun Chen , Zijia Liu , Yiqi Zhang , Baojie Feng , Peng Cheng , Jin Zhao , Lan Chen , Kehui Wu

Moire superlattices of transition metal dichalcogenide (TMD) bilayers have been shown to host correlated electronic states, which arises from the interplay of emergent moire potential and long-range Coulomb interactions. Here we…

Strongly Correlated Electrons · Physics 2021-04-28 Yang Zhang , Tongtong Liu , Liang Fu

We investigate electron paring in a two-dimensional electron system mediated by vacuum fluctuations inside a nanoplasmonic terahertz cavity. We show that the structured cavity vacuum can induce long-range attractive interactions between…

Mesoscale and Nanoscale Physics · Physics 2019-04-10 Frank Schlawin , Andrea Cavalleri , Dieter Jaksch

Polarons - electrons coupled with lattice vibrations - play a key role in the transport and optical properties of many systems of reduced dimension and dimensionality. Their confinement affects drastically the phonon, polaron, bipolaron and…

Mesoscale and Nanoscale Physics · Physics 2010-05-18 A. S. Alexandrov , A. M. Bratkovsky

It can be seen by Dynamic Electrical Analysis that the electrical properties of polyetherimide at temperatures above the glass transition are strongly influenced by space charge. We have studied space charge relaxation in two commercial…

Materials Science · Physics 2021-04-01 M. Mudarra , J. Sellares , J. C. Canadas , J. A. Diego

Two-dimensional electron and hole gas systems, enabled through band structure design and epitaxial growth on planar substrates, have served as key platforms for fundamental condensed matter research and high performance devices. The…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Wei Lu , Jie Xiang , Brian P. Timko , Yue Wu , Charles M. Lieber

The concept of magnetic polaron is analysed and developed to elucidate the nature of itinerant charge carrier states in magnetic semiconductors and similar complex magnetic materials. By contrasting the scattering and bound states of…

Strongly Correlated Electrons · Physics 2007-05-23 A. L. Kuzemsky

We explore higher order dynamical effects in the transport through a two-dimensional nanoscale electron system embedded in a three-dimensional far-infrared photon cavity. The nanoscale system is considered to be a short quantum wire with a…

Mesoscale and Nanoscale Physics · Physics 2020-12-11 Vidar Gudmundsson , Nzar Rauf Abdullah , Chi-Shung Tang , Andrei Manolescu , Valeriu Moldoveanu

We consider a condensate of exciton-polaritons in a diluted magnetic semiconductor microcavity. Such system may exhibit magnetic self-trapping in the case of sufficiently strong coupling between polaritons and magnetic ions embedded in the…

Quantum Gases · Physics 2017-10-04 Paweł Miętki , Michał Matuszewski

The low-energy electronic Hamiltonian for the thinest zigzag carbon nanotube, embedded into a dielectric host, is derived and its phase diagram is discussed. The specific multi-band structure and the microscopic form of the…

Superconductivity · Physics 2007-05-23 Krzysztof Byczuk

Mutual Coulomb interactions between electrons lead to a plethora of interesting physical and chemical effects, especially if those interactions involve many fluctuating electrons over large spatial scales. Here, we identify and study in…

Charge transfer is a fundamental process that underlies a multitude of phenomena in chemistry and biology. Recent advances in observing and manipulating charge and heat transport at the nanoscale, and recently developed techniques for…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Galen T. Craven , Abraham Nitzan

The cross over from low to high carrier densities in a many-polaron system is studied in the framework of the one-dimensional spinless Holstein model, using unbiased numerical methods. Combining a novel quantum Monte Carlo approach and…

Strongly Correlated Electrons · Physics 2007-05-23 M. Hohenadler , D. Neuber , W. von der Linden , G. Wellein , J. Loos , H. Fehske

We consider transport through a vibrating molecular quantum dot contacted to macroscopic leads acting as charge reservoirs. In the equilibrium and nonequilibrium regime, we study the formation of a polaron-like transient state at the…

Strongly Correlated Electrons · Physics 2015-06-04 T. Koch , H. Fehske , J. Loos

Quasi-two-dimensional systems may exibit curvature, which adds three-dimensional influence to their internal properties. As shown by da Costa \cite{dacosta}, charged particles moving on a curved surface experience a curvature-dependent…

Mesoscale and Nanoscale Physics · Physics 2017-11-03 Fernando Santos , Sébastien Fumeron , Bertrand Berche , Fernando Moraes