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Photoassociation of ultracold rubidium atoms with femtosecond laser pulses is studied theoretically. The spectrum of the pulses is cut off in order to suppress pulse amplitude at and close to the atomic resonance frequency. This leads to…

Femtosecond pulsed laser systems constitute powerful tools for the high-precision structuring of materials at micro/nano-scale resolutions. A critical parameter influencing the efficacy of ultrafast laser-material interactions is the…

Optics · Physics 2026-03-05 George D. Tsibidis

A spectroscopic application of the atom laser is suggested. The spectroscopy termed 2PACC employs the coherent properties of matter-waves from a two pulse atom laser. These waves are employed to control a gas-surface chemical recombination…

Quantum Physics · Physics 2009-11-10 Solvejg Jorgensen , Ronnie Kosloff

Recently, it was predicted theoretically and verified experimentally that a pair of delayed and cross-polarized short laser pulses can create molecular ensembles with a well defined sense of rotation (clockwise or counterclockwise). Here we…

Attosecond x-ray pulses play a crucial role in the study of ultrafast phenomena occurring within inner and valence electrons. To achieve attosecond time-resolution studies and gain control over electronic wavefunctions, it is crucial to…

Accelerator Physics · Physics 2024-01-30 Hao Sun , Xiaofan Wang , Weiqing Zhang

Light-electron interaction in empty space is the seminal ingredient for free-electron lasers and also for controlling electron beams to dynamically investigate materials and molecules. Pushing the coherent control of free electrons by light…

We introduce a protocol for dynamical dispersion engineering in an atomic chain consisting of an ordered array of multi-level atoms with subwavelength lattice constant. This chain supports dark states that are protected from dissipation in…

Quantum Physics · Physics 2022-04-15 R. Gutiérrez-Jáuregui , A. Asenjo-Garcia

We investigate the coherent control of the photo\-electron angular distribution in bichromatic atomic ionization. Neon is selected as target since it is one of the most popular systems in current gas-phase experiments with free-electron…

Atomic Physics · Physics 2018-01-31 E. V. Gryzlova , A. N. Grum-Grzhimailo , E. I. Staroselskaya , N. Douguet , K. Bartschat

A theoretical investigation on the quantum control of optical coherent four-wave mixing interactions in two-level systems driven by two intense synchronized femtosecond laser pulses of central angular frequencies $\omega$ and $3\omega$ is…

Optics · Physics 2009-11-10 Carles Serrat

High-order harmonic generation from atomic systems is considered in the crossed fields of a relativistically strong infrared laser and a weak attosecond-pulse train of soft x-rays. Due to one-photon ionization by the x-ray pulse, the…

Atomic Physics · Physics 2009-11-13 Michael Klaiber , Karen Z. Hatsagortsyan , Carsten Müller , Christoph H. Keitel

Attosecond science has been transforming our understanding of electron dynamics in atoms, molecules and solids. However, to date almost all of the attoscience experiments have been based on spectroscopic measurements because attosecond…

We develop theoretically and confirm both numerically and experimentally a comprehensive analytical model which describes the propensity rules in the emission of circularly polarized high harmonics by systems driven by two-color…

A three-dimensional semiclassical model is used to study double ionization of Ar when driven by a near-infrared and near-single-cycle laser pulse for intensities ranging from 0.85$\times$10$^{14}$ W/cm$^{2}$ to 5$\times$10$^{14}$…

Atomic Physics · Physics 2017-02-15 A. Chen , M. Kübel , B. Bergues , M. F. Kling , A. Emmanouilidou

The coherent interaction with ultrashort light pulses is a powerful strategy for monitoring and controlling the dynamics of wave packets in all states of matter. As light presents an oscillation period of a few femtoseconds ($T=2.6$~fs in…

Tracking the coupled motion of electrons and nuclei on their intrinsic timescales is essential to understanding and controlling photochemical transformations. While attosecond techniques have provided unprecedented insight into electronic…

Laser pulses with stable electric field waveforms establish the opportunity to achieve coherent control on attosecond timescales. We present experimental and theoretical results on the steering of electronic motion in a multi-electron…

Probing vibronic coherence in molecules has been a central topic in ultrafast science, as it is an essential prerequisite to monitoring electronic motion. While experiments have demonstrated that attosecond transient absorption spectroscopy…

Atomic Physics · Physics 2023-08-02 C. H. Yuen , C. D. Lin

The coherent interaction between a laser-driven single trapped atom and an optical high-finesse resonator allows to produce entangled multi-photon light pulses on demand. The mechanism is based on the mechanical effect of light. The degree…

Quantum Physics · Physics 2009-11-11 Giovanna Morigi , Juergen Eschner , Stefano Mancini , David Vitali

We theoretically investigate the generation of intense keV attosecond pulses in an orthogonally polarized multicycle midinfrared two-color laser field. It is demonstrated that multiple continuum-like humps, which have a spectral width of…

Optics · Physics 2017-11-22 Guicun Li , Yinghui Zheng , Zhinan Zeng , Ruxin Li

Here the ionization and high harmonic generation in Hydrogen and Helium by using quantum (hydrodynamic) trajectories is analyzed theoretically. The quantum trajectories allow a self-contained treatment of the electron exchange and…

Atomic Physics · Physics 2025-02-07 Ivan P. Christov