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In this paper, we introduce a novel, adapted approach for computing gas adsorption properties in porous materials. We analyze the Dubinin-Polanyi's adsorption model and investigate various frameworks to estimate its required essential…

Materials Science · Physics 2023-10-25 F. Stavarache , A. Luna-Triguero , S. Calero , J. M. Vicent-Luna

Theoretical framework for the isosteric heat of adsorption is developed treating the effects of the non-ideal gas behavior and the adsorbed phase volume. Rigorous thermodynamic treatment for the adsorbed phase volume is presented for…

Chemical Physics · Physics 2017-09-07 Kyaw Thu , Sourav Mitra , Bidyut Baran Saha

Determining the adsorption isotherms is an issue of significant importance in preparative chromatography. A modern technique for estimating adsorption isotherms is to solve an inverse problem so that the simulated batch separation coincides…

Applications · Statistics 2022-11-24 Jiaji Su , Zhigang Yao , Cheng Li , Ye Zhang

In this paper, we present a new implementation of the Multicomponent Potential Theory of Adsorption model. The proposed interpretation establishes a clear cut between parameters that depends on the adsorbent from those depending on the…

Soft Condensed Matter · Physics 2020-12-01 Raphaël Gervais Lavoie , Jean Hamelin , Pierre Bénard

We introduce a new and general continuum thermodynamic framework for the mathematical analysis and computation of adsorption on dynamic interfaces. To the best of our knowledge, there is no formulation available that accounts for the…

Fluid Dynamics · Physics 2013-07-31 Markus Schmuck , Serafim Kalliadasis

We analyze here a model for an adsorbate system composed of many layers by extending a theoretical approach used to describe pattern formation on a monolayer of adsorbates with lateral interactions. The approach shows, in addition to a…

Statistical Mechanics · Physics 2009-11-07 S. B. Casal , Horacio S. Wio , S. Mangioni

Adsorption breakthrough modeling often requires complex software environments and scripting, limiting accessibility for many practitioners. We present AIM, a MATLAB-based graphical user interface (GUI) application that streamlines fixed-bed…

This work is aimed at understanding the basic principles of adsorption process in great details as adsorptive separation process has broad applications in the industry. To this end, a simple mathematical model has been used to describe…

Applied Physics · Physics 2019-07-02 Saikat Roy , Arun S. Moharir

We propose a self-consistent model taking into account variations in adsorption properties of the adsorbent surface in the process of adsorption--desorption of molecules of gas on it. We introduce a dimensionless coupling parameter that…

Materials Science · Physics 2009-11-30 A. S. Usenko

By combining different ideas, a general and efficient protocol to deal with discontinuous phase transitions at low temperatures is proposed. For small $T$'s, it is possible to derive a generic analytic expression for appropriate order…

Statistical Mechanics · Physics 2015-06-03 C. E. Fiore , M. G. E. da Luz

We investigate the competitive adsorption of a two-component gas on the surface of an adsorbent whose adsorption properties vary in adsorption due to the adsorbent deformation. The essential difference of adsorption isotherms for a…

Materials Science · Physics 2015-06-17 A. S. Usenko

Absorption imaging and spectroscopy can probe the dynamics of an ultracold neutral plasma during the first few microseconds after its creation. Quantitative analysis of the data, however, is complicated by the inhomogeneous density…

A mathematical model of the process of carbon capture in a packed column by adsorption is developed and analysed. First a detailed study is made of the governing equations. Due to the complexity of the internal geometry it is standard…

Other Condensed Matter · Physics 2020-09-15 T. G. Myers , F. Font , M. G. Hennessy

Structural materials are broadly used in applications such as nuclear vessels, high-temperature processes, and civil construction. Usually, during their placing and lifespan, they may present free or chemically bonded liquid phases in their…

Materials Science · Physics 2021-03-29 M. H. Moreira , R. F. Ausas , S. Dal Pont , P. I. Pelissari , A. P. Luz , V. C. Pandolfelli

A simple molecular thermodynamic approach is applied to the study of the adsorption of gases of chain molecules on solid surfaces. We use a model based on the Statistical Associating Fluid Theory for Variable Range (SAFT-VR) potentials [A.…

Computational Physics · Physics 2010-12-23 M. Castro , R. Martinez , A. Martinez , H. C. Rosu

Vapor adsorption experiments are widely used to assess pore size distributions, but the large hysteresis sometimes observed between sorption and desorption isotherms remains difficult to interpret. Such hysteresis is influenced pore network…

Materials Science · Physics 2018-07-03 Matthew B. Pinson , Tingtao Zhou , Hamlin M. Jennings , Martin Z. Bazant

Accounting of effective volumetric factor for the measurement at inhomogeneous temperature allows to the simplify the measurement process avoiding a pre-calibration with a noble gas. The volumetric correction in form of the volumetric…

Instrumentation and Detectors · Physics 2014-07-17 I. V. Drozdov

Integrated tempering sampling (ITS) method is an approach to enhance the sampling over a broad range of energies and temperatures in computer simulations. In this paper, a new version of integrated tempering sampling method is proposed. In…

Computational Physics · Physics 2015-06-15 Peng Zhao , Li Jiang Yang , Yi Qin Gao , Zhong-Yuan Lu

A non-equilibrium thermodynamics model able to analyze the combined effect of diffusion and adsorption in porous materials is proposed. The model considers the coupled dynamics of the diffusive phase, described by a diffusion type equation,…

Materials Science · Physics 2015-06-04 I. Santamaria-Holek , Z. J. Grzywna , J. M. Rubi

A new modeling way of describing the continuous absorption of electromagnetic (EM) radiation in dense partially ionized hydrogen plasma is tested in this work. It is shown that the obtained results give a possibility of calculating spectral…

Solar and Stellar Astrophysics · Physics 2012-08-14 A. A. Mihajlov , N M Sakan , V. A. Sreckovic , Y. Vitel
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