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We report ultrafast response of femtosecond photoexcited carriers in single layer reduced graphene oxide flakes suspended in water as well as few layer thick film deposited on indium tin oxide coated glass plate using pump-probe…

Materials Science · Physics 2011-06-30 Sunil Kumar , N. Kamaraju , K. S. Vasu , A. K. Sood

Using ultrafast optical pump-probe spectroscopy, we have measured carrier relaxation times in epitaxial graphene layers grown on SiC wafers. We find two distinct time scales associated with the relaxation of nonequilibrium photogenerated…

Materials Science · Physics 2019-06-05 Jahan M. Dawlaty , Shriram Shivaraman , Mvs Chandrashekhar , Farhan Rana , Michael G. Spencer

Femtosecond time-resolved spectroscopy using 400 nm-pump and 800 nm-probe in CVD-grown multilayer graphene provides strong evidence for isotropic distribution of photoexcited carrier after initial relaxation. Indicative of such isotropic…

Mesoscale and Nanoscale Physics · Physics 2013-12-24 Xiao-Qing Yan , Zhi-Bo Liu , Jun Yao , Xin Zhao , Xu-Dong Chen , Yongsheng Chen , Jian-Guo Tian

Third-order nonlinear absorption and refraction coefficients of a few-layer boron carbon nitride (BCN) and reduced graphene oxide (RGO) suspensions have been measured at 3.2 eV in the femtosecond regime. Optical limiting behavior is…

Mesoscale and Nanoscale Physics · Physics 2010-10-13 Sunil Kumar , N. Kamaraju , K. S. Vasu , Angshuman Nag , A. K. Sood , C. N. R. Rao

We study the carrier dynamics in epitaxially grown graphene in the range of photon energies from 10 - 250 meV. The experiments complemented by microscopic modeling reveal that the carrier relaxation is significantly slowed down as the…

Time-dependent femtosecond pump-probe spectroscopic ellipsometry studies on zincblende gallium-nitride (zb-GaN) are performed and analyzed between 2.9-3.7eV. An ultra-fast change of the absorption onset (3.23eV for zb-GaN) is observed by…

We report an optical study of charge transport in graphene. Diffusion of hot carriers in epitaxial graphene and reduced graphene oxide samples are studied using an ultrafast pump-probe technique with a high spatial resolution.…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 Brian A. Ruzicka , Shuai Wang , Lalani K. Werake , Ben Weintrub , Kian Ping Loh , Hui Zhao

We perform a femtosecond-THz optical pump-probe spectroscopy to investigate the cooling dynamics of hot carriers in quasi-free standing bilayer epitaxial graphene. We observed longer decay time constants, in the range of 2.6 to 6.4 ps,…

Mesoscale and Nanoscale Physics · Physics 2023-02-03 Sachin Sharma , Rachael L. Myers-Ward , David Kurt Gaskill , Ioannis Chatzakis

We investigate the relaxation dynamics of photogenerated carriers in silicon nanowires consisting of a crystalline core and a surrounding amorphous shell, using femtosecond time-resolved differential reflectivity and transmission…

Mesoscale and Nanoscale Physics · Physics 2012-12-24 Sunil Kumar , M. Khorasaninejad , M. M. Adachi , K. S. Karim , S. S. Saini , A. K. Sood

Exploring novel materials with enhanced optical nonlinearities at low power levels with ultrafast response and small footprints is of great interests for information processing, communication, sensing and quantum systems. Recent progress on…

Optics · Physics 2023-05-23 Md Zubair Ebne Rafique , Ali Basiri , Jing Bai , Jiawei Zuo , Yu Yao

A degenerate pump--probe technique is used to investigate the non equilibrium carrier dynamics in multi--layer graphene. Two distinctly different dynamics of the carrier relaxation are observed. A fast relaxation ($\sim 50$ fs) of the…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 P. Plochocka , P. Kossacki , A. Golnik , T. Kazimierczuk , C. Berger , W. A. de Heer , M. Potemski

We report evidence of nonequilibrium hot carriers extraction from graphene by gate-dependent photocurrent study. Scanning photocurrent excited by femtosecond pulse laser shows unusual gate dependence compared with continuous wave (CW) laser…

Mesoscale and Nanoscale Physics · Physics 2012-07-12 Chang-Hua Liu , Nanditha M. Dissanayake , Seunghyun Lee , Kyunghoon Lee , Zhaohui Zhong

Saturable absorption is a non-perturbative nonlinear optical phenomenon that plays a pivotal role in the generation of ultrafast light pulses. Here we show that this effect emerges in graphene at unprecedentedly low light intensities, thus…

Mesoscale and Nanoscale Physics · Physics 2017-03-15 A. Marini , J. D. Cox , F. J. Garcia de Abajo

The dynamics of photocarriers in reduced graphene oxide thin films is studied by using ultrafast pump-probe spectroscopy. Time dependent differential transmissions are measured with sample temperatures ranging from 9 to 300 K. At each…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Brian A. Ruzicka , Lalani K. Werake , Hui Zhao , Shuai Wang , Kian Ping Loh

Understanding the ultrafast carrier dynamics of graphene on a substrate is a fundamental step in the development of graphene based opto-electronic devices. Here, we present ultrafast pump-probe measurements of supported graphene on quartz…

Mesoscale and Nanoscale Physics · Physics 2021-02-16 Rustam Gatamov , Andrey Baydin , Halina Krzyzanowska , Norman Tolk

The nonequilibrium dynamics of carriers and phonons in graphene is investigated by solving the microscopic kinetic equations with the carrier-phonon and carrier-carrier Coulomb scatterings explicitly included. The Fermi distribution of hot…

Mesoscale and Nanoscale Physics · Physics 2012-03-15 B. Y. Sun , Y. Zhou , M. W. Wu

The energy relaxation of carriers in reduced graphene oxide thin films is studied using optical pump-probe spectroscopy with two probes of different colors. We measure the time difference between peaks of the carrier density at each probing…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Brian A. Ruzicka , Nardeep Kumar , Shuai Wang , Kian Ping Loh , Hui Zhao

The enhanced nonlinear optical response of a one-dimensional (1D) photonic crystal (PC) made from polymers and graphene composites is observed. The graphene PC was fabricated by spin-coating. It shows obvious bandgaps at two wavelengths in…

We theoretically examine the effect of carrier-carrier scattering processes (electron-hole and electron-electron) on the intraband radiation absorption and their contribution to the net dynamic conductivity in optically or electrically…

Mesoscale and Nanoscale Physics · Physics 2014-08-21 Dmitry Svintsov , Victor Ryzhii , Akira Satou , Taiichi Otsuji , Vladimir Vyurkov

Graphene is a promising material for ultrafast and broadband photodetection. Earlier studies addressed the general operation of graphene-based photo-thermoelectric devices, and the switching speed, which is limited by the charge carrier…

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