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Related papers: Phonons in Crystals using Inelastic X-Ray Scatteri…

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Resonant inelastic x-ray scattering (RIXS) is a well-established tool for studying electronic, nuclear and collective dynamics of excited atoms, molecules and solids. An extension of this powerful method to a time-resolved probe technique…

Chemical Physics · Physics 2015-11-03 Victor Kimberg , Nina Rohringer

Longitudinal-optical (LO) mode phonon branches of KCl and NaCl were measured using inelastic X-ray scattering (IXS) at 300 K and calculated by the first-principles phonon calculation with the stochastic self-consistent harmonic…

Materials Science · Physics 2022-07-13 Atsushi Togo , Hiroyuki Hayashi , Terumasa Tadano , Satoshi Tsutsui , Isao Tanaka

We explore the inelastic electron scattering in SrTiO3, PbTiO3, and SiC in their phonon energy range, challenging the assumption that phonon polaritons are excluded at large angles in high-resolution transmission electron energy-loss…

We report the first results of a search for real photon-photon scattering using X rays. A novel system is developed to split and collide X-ray pulses by applying interferometric techniques. A total of $6.5\times10^{5}$ pulses (each…

High Energy Physics - Experiment · Physics 2014-04-21 T. Inada , T. Yamaji , S. Adachi , T. Namba , S. Asai , T. Kobayashi , K. Tamasaku , Y. Tanaka , Y. Inubushi , K. Sawada , M. Yabashi , T. Ishikawa

The new model of phonon transmission across the interface between two crystals is proposed featured by taking into account the mismatch of crystal lattices. It has been found that the mismatch of lattices results in phonon scattering at the…

Other Condensed Matter · Physics 2016-02-22 Aleksandr Meilakhs

A technique to measure the decoherence time of optical phonons in a solid is presented. Phonons are excited with a pair of time delayed 80 fs, near infrared pulses via spontaneous, transient Raman scattering. The fringe visibility of the…

Acoustic phonons have recently been posited as playing an integral role in explaining the half-quantized thermal Hall effect in $\alpha$-RuCl$_3$. Therefore, we present much needed inelastic x-ray scattering measurements of its acoustic…

Strongly Correlated Electrons · Physics 2022-07-07 Blair W. Lebert , Subin Kim , Danil A. Prishchenko , Alexander A. Tsirlin , Ayman H. Said , Ahmet Alatas , Young-June Kim

Our objective is to study resonant tunneling of an electron in the presence of inelastic scattering by optical phonons. Using a recently developed technique, based on exact mapping of a many-body problem onto a one-body problem, we compute…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 K. Haule , J. Bonca

We study the effect of spatial dispersion of crystal modes on optical properties such as the reflectivity $R$. As an example for isotropic media, we investigate the simplest model for phonons in ionic crystals and compare with previous…

Optics · Physics 2009-11-10 I. Kaelin , Ch. Helm , G. Blatter

An application of resonant inelastic x-ray scattering technique for studying of optical scale excitations in electron-correlated materials is discussed. Examples are given including data obtained for 3d transition metal, lanthanide, and…

Strongly Correlated Electrons · Physics 2007-05-23 Sergei M. Butorin

The GALAXIES beamline at the SOLEIL synchrotron is dedicated to inelastic x-ray scattering (IXS) and photoelectron spectroscopy (HAXPES) in the 2.3-12 keV hard x-ray range. These two techniques offer powerful, complementary methods of…

Instrumentation and Detectors · Physics 2018-06-12 J. -P. Rueff , J. M. Ablett , D. Céolin , D. Prieur , Th. Moreno , V. Balédent , B. Lassalle , J. E. Rault , M. Simon , A. Shukla

We present a measurement of phonon propagation in a silicon wafer utilizing an array of frequency-multiplexed superconducting resonators coupled to a single transmission line. The electronic readout permits fully synchronous array sampling…

Instrumentation and Detectors · Physics 2015-05-18 L. J. Swenson , A. Cruciani , A. Benoit , M. Roesch , C. S. Yung , A. Bideaud , A. Monfardini

Diffuse X-ray data for mixed stack organic charge-transfer crystals approaching the neutral-ionic phase transition can be quantitatively explained as due to the softening of the optical phonon branch. The interpretation is fully consistent…

Strongly Correlated Electrons · Physics 2009-11-13 Gabriele D'Avino , Alberto Girlando , Anna Painelli , Marie-Hélène Lemée-Cailleau , Zoltán G. Soos

We measure phonon dispersion and linewidth in a single crystal of MgB_2 along the Gamma-A, Gamma-M and A-L directions using inelastic X-Ray scattering. We use Density Functional Theory to compute the effect of both electron-phonon coupling…

Polar phonons can induce electric fields in an adjacent layer, whether non-polar or polar, producing remote phonon scattering of electrons. Treatment of remote phonon scattering has been based on the dielectric continuum model which takes…

Materials Science · Physics 2020-04-15 A. Dyson , B. K. Ridley

Phonons diffraction and interference patterns are observed at the atomic scale, using molecular dynamics simulations in systems containing crystalline silicon and nanometric obstacles as voids or amorphous-inclusions. The diffraction…

Inelastic neutron-scattering experiments have been carried out on polycrystalline samples of the FeSe$_{1-x}$ superconductors. We report the phonon density of states for FeSe$_{1-x}$ with Tc$\approx$8 K. The phonon cutoff frequency is…

Superconductivity · Physics 2009-02-17 D. Phelan , J. N. Millican , E. L. Thomas , J. B. Leao , Y. Qiu , R. Paul

In the iron pnictides, the strong sensitivity of the iron magnetic moment to the arsenic position suggests a significant relationship between phonons and magnetism. We measured the phonon dispersion of several branches in the high…

The capability to probe the dispersion of elementary spin, charge, orbital, and lattice excitations has positioned resonant inelastic x-ray scattering (RIXS) at the forefront of photon science. Here we develop the scattering theory for RIXS…

Superconductivity · Physics 2015-04-10 Pasquale Marra , Steffen Sykora , Krzysztof Wohlfeld , Jeroen van den Brink

Anomalous thermal expansion behaviour of several open frame-work compounds has been extensively investigated using the techniques of inelastic neutron scattering and lattice dynamics. These compounds involve increasing level of structural…

Materials Science · Physics 2017-11-21 R. Mittal , M. K. Gupta , S. L. Chaplot