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Electron paramagnetic resonance (EPR) spectroscopy interrogates unpaired electron spins in solids and liquids to reveal local structure and dynamics; for example, EPR has elucidated parts of the structure of protein complexes that have…

Other Condensed Matter · Physics 2012-05-08 S. Takahashi , L. -C. Brunel , D. T. Edwards , J. van Tol , G. Ramian , S. Han , M. S. Sherwin

The development of a new era of quantum devices requires an understanding of how paramagnetic dopants or impurity spins behave in crystal hosts. Here, we describe a new spectroscopic technique which uses traditional Electron Spin Resonance…

On-chip Electron Spin Resonance (ESR) of magnetic molecules requires the ability to precisely position nanosized samples in antinodes of the electro-magnetic field for maximal magnetic interaction. A method is developed to entrap…

Mesoscale and Nanoscale Physics · Physics 2009-08-28 N. Groll , S. Bertaina , M. Pati , N. S. Dalal , I. Chiorescu

Coherent spin resonance methods such as nuclear magnetic resonance (NMR) and electron spin resonance (ESR) spectroscopy have led to spectrally highly sensitive, non-invasive quantum imaging techniques with groundbreaking applications in…

Spectroscopy is a powerful tool to probe physical, chemical, and biological systems. Recent advances in microfabrication have introduced novel, intriguing mesoscopic quantum systems including superconductor-semiconductor hybrid devices and…

Mesoscale and Nanoscale Physics · Physics 2021-11-04 J. Griesmar , R. H. Rodriguez , V. Benzoni , J. -D. Pillet , J. -L. Smirr , F. Lafont , Ç. Ö. Girit

Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…

In this paper, we present a rapidly-prototyped, costefficient, 3D-printed quasioptical sample holder for improving the signal-to-noise ratio (SNR) in modern, resonator-free, highfield electron paramagnetic resonance (EPR) spectrometers.…

Instrumentation and Detectors · Physics 2024-01-04 Antonin Sojka , Brad D. Price , Mark S. Sherwin

We report measurements of electron spin echo envelope modulation (ESEEM) performed at millikelvin temperatures in a custom-built high-sensitivity spectrometer based on superconducting micro-resonators. The high quality factor and small mode…

The successful use of picosecond-pulse free-electron-laser (FEL) radiation for the continuous-wave THz-range electron spin resonance (ESR) spectroscopy has been demonstrated. The combination of two linac-based FELs (covering the wavelength…

Millimetre-wave observations represent an important tool for Cosmology studies. The Line Intensity Mapping (LIM) technique has been proposed to map in three dimensions the specific intensity due to line (e.g. [CII], CO) emission, for…

Instrumentation and Methods for Astrophysics · Physics 2023-08-29 Usasi Chowdhury , Florence Levy-Bertrand , Martino Calvo , Johannes Goupy , Alessandro Monfardini

We present the design of a continuous-wave, highly sensitive optical spectrometer for millimeter-wave frequencies between 50 and 1000 GHz. The spectrometer uses photomixing of near-infrared light to generate radiation in a wide frequency…

Instrumentation and Detectors · Physics 2024-11-26 L. Rogić , N. Somun , S. Griffitt , A. Najev , M. Spaić , S. Hameed , Y. Shemerliuk , S. Aswartham , M. Orlita , A. Alfonsov , D. Pelc

Single-spin magnetic resonance spectroscopy promises to yield structural and chemical information at the level of individual atoms or molecules, in a non-invasive way. Here, we use an Er3+ paramagnetic center in a CaWO4 crystal, detected by…

An experimental platform of ultralow-temperature pulsed ENDOR (electron-nuclear double resonance) spectroscopy is constructed for the bulk materials. Coherent property of the coupled electron and nuclear spins of the rare-earth (RE) dopants…

Classical sensors for spectrum analysis are widely used but lack micro- or nanoscale spatial resolution. On the other hand, quantum sensors, capable of working with nanoscale precision, do not provide precise frequency resolution over a…

Quantum Physics · Physics 2022-07-12 Nicolas Staudenmaier , Simon Schmitt , Liam P. McGuinness , Fedor Jelezko

Coherent spin resonance methods, such as nuclear magnetic resonance and electron spin resonance spectroscopy, have led to spectrally highly sensitive, non-invasive quantum imaging techniques. Here, we propose a pump-probe spin resonance…

Quantum Physics · Physics 2024-12-02 Philipp Haslinger , Stefan Nimmrichter , Dennis Rätzel

High frequency electron spin resonance (ESR) spectroscopy is an invaluable tool for identification and characterization of spin systems. Nanoscale ESR using the nitrogen-vacancy (NV) center has been demonstrated down to the level of a…

Mesoscale and Nanoscale Physics · Physics 2020-05-05 Benjamin Fortman , Junior Pena , Karoly Holczer , Susumu Takahashi

Magnetic resonance spectroscopy is universally regarded as one of the most important tools in chemical and bio-medical research. However, sensitivity limitations typically restrict imaging resolution to length scales greater than 10 \mu m.…

We develop an all electrical experiment to perform the broadband phase-resolved spectroscopy of propagating spin waves in micrometer sized thin magnetic stripes. The magnetostatic surface spin waves are excited and detected by scaled down…

Mesoscale and Nanoscale Physics · Physics 2016-08-03 Florin Ciubotaru , Thibaut Devolder , Mauricio Manfrini , Christoph Adelmann , Iuliana Radu

In this study, novel use of the electromagnetic field profile of a localized spoof surface plasmonic mode to detect electron spin resonance is being reported. The mode is supported on a resonator with a complementary metallic spiral…

Applied Physics · Physics 2021-05-04 Subhadip Roy , Anuvab Nandi , Pronoy Das , Chiranjib Mitra

A combined experimental/theoretical study of the EPR in irradiated $\beta$-Ga$_2$O$_3$ is presented. Four EPR spectra, two $S=1/2$ and two $S=1$, are observed after high-energy proton or electron irradiation. One of the S=1/2 spectra (EPR1)…