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We report the first principles investigations on the phonons of three polytypes of BaTiO3 (BTO): paraelectric (PE) cubic Pm-3m and two ferroelectric (FE) phases, tetragonal P4mm and rhombohedral R3m. The phonon frequencies calculated using…

Materials Science · Physics 2013-12-16 Yu-Seong Seo , Jai Seok Ahn

A study of the adsorption of CO on late 4d and $5d$ transition metal (111) surfaces (Ru, Rh, Pd, Ag, Os, Ir, and Pt) considering atop and hollow site adsorption is presented. The applied functionals include the gradient corrected PBE and…

Materials Science · Physics 2011-12-30 A. Stroppa , G. Kresse

In contrast with recent claims that the Heyd-Scuseria-Ernzerhof (HSE) screened hybrid functional can provide a good description of the electronic and magnetic structure of VO2 phases [V. Eyert, Phys. Rev. Lett. 107, 016401 (2011)], we show…

Strongly Correlated Electrons · Physics 2015-06-05 Ricardo Grau-Crespo , Hao Wang , Udo Schwingenschloegl

Two-dimensional van der Waals heterostructures are potential game changers both in understanding the fundamental physics and in the realization of various devices that exploit magnetism at the nanoscale. Multiferroic heterostructures…

Materials Science · Physics 2024-12-12 Himangshu Sekhar Sarma , Subhradip Ghosh

We propose a multiconfigurational hybrid density-functional theory which rigorously combines a multiconfiguration self-consistent-field calculation with a density-functional approximation based on a linear decomposition of the…

Chemical Physics · Physics 2012-08-20 Kamal Sharkas , Andreas Savin , Hans Jørgen Aa. Jensen , Julien Toulouse

The magnetic state of UO$_2$ was determined experimentally to be anti-ferromagnetic. Starting from this experimental fact, researchers have calculated other properties within the Hubbard-corrected density-functional theory, DFT+U. Up to…

Materials Science · Physics 2024-01-03 Mahmoud Payami

Multiferroic materials, in which ferroelectric and magnetic ordering coexist, are of fundamental interest for the development of novel memory devices that allow for electrical writing and non-destructive magnetic readout operation. The…

Materials Science · Physics 2015-05-05 P. S. Wang , W. Ren , L. Bellaiche , H. J. Xiang

A detailed exploration of the $f$-atomic orbital occupancy space for UO$_2$ is performed using a first principles approach based on density functional theory (DFT), employing a full hybrid functional within a systematic basis set.…

Strongly Correlated Electrons · Physics 2022-01-05 Laura E. Ratcliff , Luigi Genovese , Hyowon Park , Peter B. Littlewood , Alejandro Lopez-Bezanilla

An atomistic effective Hamiltonian is used to compute electrocaloric (EC) effects in rare-earth substituted BiFeO$_{3}$ multiferroics. A phenomenological model is then developed to interpret these computations, with this model indicating…

The electronic energy structures and magnetic properties of iron-based compounds with group VI elements (FeTe, BiFeO$_3$, SrFe$_{12}$O$_{19}$ and SrCoTiFe$_{10}$O$_{19}$) are studied using the density functional theory (DFT) methods.…

Materials Science · Physics 2015-10-05 G. E. Grechnev , A. A. Lyogenkaya , O. V. Kotlyar , A. S. Panfilov , V. P. Gnezdilov

Novel imaging spin-filter techniques, which are based on low energy electron diffraction, are currently of high scientific interest. To improve the spin-detection efficiency a variety of new materials have been introduced in recent years. A…

Computational Physics · Physics 2015-11-18 Stephan Borek , Jürgen Braun , Hubert Ebert , Ján Minár

Multiferroics where at least two primary ferroic orders are present and coupled in a single system constitute an important class of materials. They attracted special consideration as they present both intriguing fundamental physics problems…

A comparative theoretical study is presented for the rhombohedral R3 and R3m phase HfO2, of two possible forms in its heavily Zr-doped ferroelectric thin films found recently in experiments. Their structural stability and polarization under…

Materials Science · Physics 2023-07-03 Wenbin Ouyang , Fanghao Jia , Wei Ren

We have calculated the properties of SrTiO3 (STO) using a wide array of density functionals ranging from standard semi-local functionals to modern range-separated hybrids, combined with several basis sets of varying size/quality. We show…

Computational Physics · Physics 2016-11-25 Fadwa El-Mellouhi , Edward N. Brothers , Melissa J. Lucero , Gustavo E. Scuseria

Two-dimensional (2D) semiconducting multiferroics that can effectively couple magnetic and polarization (P) orders have great interest for both fundamental research and technological applications in nanoscale, which are, however, rare in…

Materials Science · Physics 2023-03-01 Baishun Yang , Bin Shao , Jianfeng Wang , ChiYung Yam , Shengbai Zhang , Bing Huang

The hexagonal multiferroic oxide YMnO$_3$ has demonstrated applications in various fields and is widely researched due to its interesting properties. Since Mn(3d)--O(2p) interactions predominate close to the Fermi level, doping in the…

Materials Science · Physics 2025-10-22 Kazi Mazba Kamal , Alamgir Kabir

Hexagonal ferrites (h-RFeO$_3$, R=Y, Dy-Lu) have recently been identified as a new family of multiferroic complex oxides. The coexisting spontaneous electric and magnetic polarizations make h-RFeO$_3$ rare-case ferroelectric ferromagnets at…

Materials Science · Physics 2014-08-22 Xiaoshan Xu , Wenbin Wang

The design of novel cathode materials for Li-ion batteries would greatly benefit from accurate first-principles predictions of structural, electronic, and magnetic properties as well as intercalation voltages in compounds containing…

Materials Science · Physics 2022-11-03 Iurii Timrov , Francesco Aquilante , Matteo Cococcioni , Nicola Marzari

We propose a microscopic theory for magnetic switching of electric polarization (P) in the spin-spiral multiferroics by taking TbMnO3 and DyMnO3 as examples. We reproduce their phase diagrams under a magnetic field H_ex by Monte-Carlo…

Strongly Correlated Electrons · Physics 2010-10-29 Masahito Mochizuki , Nobuo Furukawa

Multiferroic (MF) devices based on simultaneous ferroelectric and ferromagnetic phenomena are considered to be promising candidates for future bi-functional micro/nano-electronics. The multiferroic phenomena in two-dimensional materials is…

Applied Physics · Physics 2022-08-30 Rabia Tahir , Sabeen Fatima , Syedah Afsheen Zahra , Deji Akinwande , Syed Rizwana