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Hybrid functionals and empirical correction schemes are compared to conventional semi-local density functional theory (DFT) calculations in order to assess the predictive power of these methods concerning the formation energy and the charge…

Materials Science · Physics 2013-07-02 Sung Sakong , Johann Gutjahr , Peter Kratzer

We propose a hybrid approach which employs the dynamical mean-field theory (DMFT) self-energy for the correlated, typically rather localized orbitals and a conventional density functional theory (DFT) exchange-correlation potential for the…

Strongly Correlated Electrons · Physics 2021-06-16 Sumanta Bhandary , Karsten Held

Recently, two nonempirical hybrid functionals, dielectric-dependent range-separated hybrid functional based on the Coulomb-attenuating method (DD-RSH-CAM) and doubly screened hybrid functional (DSH), have been suggested by [Chen et al,…

Materials Science · Physics 2020-01-08 Peitao Liu , Cesare Franchini , Martijn Marsman , Georg Kresse

The Heyd-Scuseria-Ernzerhof (HSE) hybrid functional has become a widely used tool for theoretical calculations of point defects in semiconductors. It generally offers a satisfactory qualitative description of defect properties, including…

The discovery of two-dimensional (2D) materials possessing switchable spontaneous polarization with atomic thickness opens up exciting opportunities to realize ultrathin, high-density electronic devices with potential applications ranging…

Materials Science · Physics 2020-11-04 Jiawei Huang , Sang-Hoon Lee , Andrew Supka , Young-Woo Son , Shi Liu

We have performed an extensive test of the ability of density functional theory within several approximations for the exchange-correlation functional, local density approximation+Hubbard $U$ and local density approximation + dynamic mean…

Strongly Correlated Electrons · Physics 2014-10-28 Oscar Grånäs , Igor di Marco , Olle Eriksson , Lars Nordström , Corina Etz

From the physical point of view multiferroics present an extremely interesting class of systems and problems. These are essentially of two kinds. One is what are the microscopic conditions, and sometimes constrains, which determine the…

Other Condensed Matter · Physics 2009-11-13 I. Radulov , V. Lovchinov , M. Daszkiewicz

An experimental study of the in-plane azimuthal behaviour and frequency dependence of the ferromagnetic resonance field and the resonance linewidth as a function of BiFeO$_3$ thickness is carried out in a polycrystalline exchange-biased…

Materials Science · Physics 2016-09-21 J. Ben Youssef , J. Richy , N. Beaulieu , T. Hauguel , D. T. Dekadjevi , J-Ph. Jay , D. Spenato , S. P. Pogossian

We present a first-principles investigation of the structural, electronic, and magnetic properties of pyrolusite ($\beta$-MnO$_2$) using conventional and extended Hubbard-corrected density-functional theory (DFT+$U$ and DFT+$U$+$V$). The…

Materials Science · Physics 2021-10-06 Ruchika Mahajan , Iurii Timrov , Nicola Marzari , Arti Kashyap

Bismuth ferrite (BiFeO$_3$) is one of the very few known single-phase multiferroic materials. While the bulk compound is rhombohedral (R), the discovery of an epitaxial strain-induced structural transition into a so-called 'super…

Materials Science · Physics 2021-01-14 Daniel Sando , Bin Xu , Laurent Bellaiche , Valanoor Nagarajan

The dependencies on strain and oxygen vacancies of the ferroelectric polarization and the weak ferromagnetic magnetization in the multiferroic material bismuth ferrite, BiFeO_3, are investigated using first principles density functional…

Materials Science · Physics 2007-05-23 Claude Ederer , Nicola A. Spaldin

We compare the ability of four popular hybrid density functionals (B3LYP, B3PW91, HSE, and PBE0) for predicting band gaps of semiconductors and insulators over a large benchmark set using a consistent methodology. We observe no significant…

Materials Science · Physics 2016-10-07 Alejandro J. Garza , Gustavo E. Scuseria

Static electric response properties of atoms and molecules are reported within the real-space Cartesian grid implementation of pseudopotential Kohn-Sham (KS) density functional theory (DFT). A detailed systematic investigation is made for a…

Chemical Physics · Physics 2019-04-26 Tanmay Mandal , Abhisek Ghosal , Amlan K. Roy

Bismuth ferrite (BiFeO3) is one of the most promising multiferroics with a sufficiently high ferroelectric (FE) and antiferromagnetic transition temperatures, and magnetoelectric (ME) coupling coefficient at room temperature, and thus it is…

Two-dimensional (2D) magnets have broad application prospects in the spintronics, but how to effectively control them with a small electric field is still an issue. Here we propose that 2D magnets can be efficiently controlled in a…

Mesoscale and Nanoscale Physics · Physics 2022-02-01 Ping Li , Xue-Song Zhou , Zhi-Xin Guo

We analyze the coupling between the ferroelectric and magnetic order parameters in the magnetoelectric multiferroic BiFeO_3 using density functional theory within the local spin density approximation and the LSDA+U method. We show that weak…

Materials Science · Physics 2007-05-23 Claude Ederer , Nicola A. Spaldin

In three out of five cases considered in our work, DFT calculations presented by Xu and Hou in their Comment give the same ground state confirmations. On the other hand, depending on the choice of the exchange-correlation functional, the…

Materials Science · Physics 2022-11-14 A. V. Bibikov , A. V. Nikolaev , I. V. Bodrenko , P. V. Borisyuk , E. V. Tkalya

The properties of many intrinsic defects in the wide band gap semiconductor LaAlO3 are studied using the screened hybrid functional of Heyd, Scuseria, and Ernzerhof (HSE). As in pristine structures, exact exchange included in the screened…

Materials Science · Physics 2015-06-17 Fedwa El-Mellouhi , Edward N. Brothers , Melissa J. Lucero , Gustavo E. Scuseria

Halide perovskites (HPs) are widely viewed as promising photovoltaic and light-emitting materials for their suitable band gaps in the visible spectrum. Density functional theory (DFT) calculations employing (semi)local exchange-correlation…

Materials Science · Physics 2022-12-06 Jiyuan Yang , Tianyuan Zhu , Shi Liu

Searching for new functionality in next generation electronic devices is a principal driver of material physics research. Multiferroics simultaneously exhibit electric and magnetic order parameters that may be coupled through…

Materials Science · Physics 2017-06-06 Sae Hwan Chun , Kwang Woo Shin , Kee Hoon Kim , John F. Mitchell , Philip J. Ryan , Jong-Woo Kim
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