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According to the pioneering work of Nielsen and collaborators, the length of the minimal geodesic in a geometric realization of a suitable operator space provides a measure of the quantum complexity of an operation. Compared with the…

Quantum Physics · Physics 2024-10-10 Satyaki Chowdhury , Martin Bojowald , Jakub Mielczarek

The two-basis method to solve the HFB for deformed nuclei in coordinate space is examined concerning the precision of the density tail. Small cutoff energies are shown to give rise to ripples in the tail, whose wave length corresponds to…

Nuclear Theory · Physics 2007-05-23 Naoki Tajima

This chapter concerns with the recent development of a new DFT methodology for accurate, reliable prediction of many-electron systems. Background, need for such a scheme, major difficulties encountered, as well as their potential remedies…

Chemical Physics · Physics 2019-04-19 Amlan K. Roy

The most efficient known quantum circuits for preparing unitary coupled cluster states and applying Trotter steps of the arbitrary basis electronic structure Hamiltonian involve interleaved sequences of fermionic Gaussian circuits and Ising…

Quantum Physics · Physics 2021-09-13 Nicholas C. Rubin , Joonho Lee , Ryan Babbush

A self-consistent many-body approach is proposed to build a first-principles crystal field theory, where crystal field parameters are calculated ab initio. Many-body theory is used to write the energy of the interacting system as a function…

Strongly Correlated Electrons · Physics 2010-09-17 Christian Brouder

We study spectral form factor in periodically-kicked bosonic chains. We consider a family of models where a Hamiltonian with the terms diagonal in the Fock space basis, including random chemical potentials and pair-wise interactions, is…

Statistical Mechanics · Physics 2022-08-30 Dibyendu Roy , Divij Mishra , Tomaž Prosen

A two-orbital two-electron diatomic model resembling LiH is used to investigate the differences between the exact L\"owdin-Shull and approximate Hartree-Fock-Bogoliubov and Baerends-Buijse density matrix functionals in the medium- to…

Chemical Physics · Physics 2020-09-09 Robert van Meer , Jeng-Da Chai

We study meson-meson interactions using an extended $q^2\bar{q}^2(g)$ basis that allows calculating coupling of an ordinary meson-meson system to a hybrid-hybrid one. We use a potential model matrix in this extended basis which at quark…

High Energy Physics - Phenomenology · Physics 2015-03-18 Nosheen Akbar , Bilal Masud

A framework for developing new approximate electronic structure methods is presented, in which the correlation energy of a many-electron system in the ground state is computed as in the single-reference second-order many-body perturbation…

Chemical Physics · Physics 2011-06-15 Dimitri Laikov

Gausslets are one of the few basis constructions for electronic structure that combine locality, orthonormality, variable resolution, and an accurate diagonal approximation for the electron-electron interaction, but the original…

Chemical Physics · Physics 2026-05-07 Steven R. White

We propose a framework for computing the structure and dynamics for second-quantized many-nucleon Hamiltonians on quantum computers. We develop an oracle-based Hamiltonian input model that computes the many-nucleon states and nonzero…

Nuclear Theory · Physics 2024-08-14 Weijie Du , James P. Vary

In this paper we consider a generalized classical mechanics with fractional derivatives. The generalization is based on the time-clock randomization of momenta and coordinates taken from the conventional phase space. The fractional…

Classical Physics · Physics 2011-11-15 Aleksander Stanislavsky

Multicluster models consider that the nucleons can be moving around different centers in the nuclei. These models have been widely used to describe light nuclei but always considering that the mean field is composed of isotropic harmonic…

Nuclear Theory · Physics 2022-01-17 A Gijón , FJ Gálvez , F. Arias de Saavedra , E Buendía

The determination of the two-body density functional from its one-body density is achieved for Moshinsky's harmonium model, using a phase-space formulation, thereby resolving its phase dilemma. The corresponding sign rules can equivalently…

Chemical Physics · Physics 2010-11-23 José M. Gracia-Bondía , Joseph C. Várilly

A new theoretical method is developed to solve the two-body bound-state Dirac equation for positronium. Only Coulomb potential was included in the Dirac Hamiltonian. It is shown that the two-body Dirac Hamiltonian can be written in the…

High Energy Physics - Phenomenology · Physics 2024-06-11 E. M. Tursunov , Sh. G. Norbutaev , B. A. Fayzullaev

An integral scheme for the efficient evaluation of two-center integrals over contracted solid harmonic Gaussian functions is presented. Integral expressions are derived for local operators that depend on the position vector of one of the…

Chemical Physics · Physics 2017-02-07 Dorothea Golze , Niels Benedikter , Marcella Iannuzzi , Jan Wilhelm , Jürg Hutter

Few-electron systems confined in two-dimensional parabolic quantum dots at high magnetic fields are studied by the Hartree-Fock (HF) and exact diagonalization methods. A generalized multicenter Gaussian basis is proposed in the HF method. A…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 B. Szafran , S. Bednarek , J. Adamowski , M. B. Tavernier , E. Anisimovas , F. M. Peeters

A representation of polymer self-consistent field theory equivalent to quantum density functional theory is given in terms of non-orthogonal basis sets. Molecular integrals and self-consistent equations for spherically symmetric systems…

Atomic Physics · Physics 2026-02-05 Phil A. LeMaitre , Russell B. Thompson

Materials utilized by novel energy systems are often studied using weakly correlated mean-field theories. However, if these systems incorporate heavy elements, relativistic effects must be included. Therefore a Kramers unrestricted Coupled…

Materials Science · Physics 2026-05-21 Luca Murg , Christopher Lane , Roxanne M. Tutchton

A recently developed finite element approach for fully numerical atomic structure calculations [S. Lehtola, Int. J. Quantum Chem. 119, e25945 (2019)] is extended to the description of atoms with spherically symmetric densities via…

Computational Physics · Physics 2020-01-30 Susi Lehtola