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A precise variational solution to $N$=2--6-body problems is reported. The trial wave functions are chosen to be combinations of correlated Gaussians, which facilitate a fully analytical calculation of the matrix elements. The nonlinear…

Nuclear Theory · Physics 2016-09-08 K. Varga , Y. Suzuki

We propose a new framework of Hessian-free force-gradient integrators that do not require the analytical expression of the force-gradient term based on the Hessian of the potential. Due to that the new class of decomposition algorithms for…

Numerical Analysis · Mathematics 2025-01-13 Kevin Schäfers , Jacob Finkenrath , Michael Günther , Francesco Knechtli

In this work, the benefits of the phase fitting technique are embedded in high order discrete Lagrangian integrators. The proposed methodology creates integrators with zero phase lag in a test Lagrangian in a similar way used in phase…

Instrumentation and Methods for Astrophysics · Physics 2009-04-02 O. T. Kosmas , D. S. Vlachos

We introduce a mixed density fitting scheme that uses both a Gaussian and a plane-wave fitting basis to accurately evaluate electron repulsion integrals in crystalline systems. We use this scheme to enable efficient all-electron Gaussian…

Chemical Physics · Physics 2017-11-22 Qiming Sun , Timothy C. Berkelbach , James D. McClain , Garnet Kin-Lic Chan

The advent of nucleon-nucleon potentials derived from chiral perturbation theory, as well as the so-called V-low-k approach to the renormalization of the strong short-range repulsion contained in the potentials, have brought renewed…

Nuclear Theory · Physics 2015-05-27 L. Coraggio , A. Covello , A. Gargano , N. Itaco , T. T. S. Kuo

We present calculations of ground state properties of spherical, doubly closed-shell nuclei from $^{16}$O to $^{208}$Pb employing the techniques of many-body perturbation theory using a separable density dependent monopole interaction. The…

Nuclear Theory · Physics 2009-11-06 P. Stevenson , M. R. Strayer , J. Rikovska Stone

This paper introduces an efficient algorithm for computing the general oscillatory matrix functions. These computations are crucial for solving second-order semi-linear initial value problems. The method is exploited using the scaling and…

Numerical Analysis · Mathematics 2024-06-11 Dongping Li , Xue Wang , Xiuying Zhang

Precise variational solutions are given for problems involving diverse fermionic and bosonic $N=2-7$-body systems. The trial wave functions are chosen to be combinations of correlated Gaussians, which are constructed from products of the…

Nuclear Theory · Physics 2008-11-26 K. Varga , Y. Suzuki

A challenge in modeling time-dependent strong-field processes such as high-harmonic generation for many-body systems, is how to effectively represent the electronic continuum. We apply Rothe's method to the time-dependent Hartree-Fock…

Chemical Physics · Physics 2025-08-22 Simon Elias Schrader , Håkon Emil Kristiansen , Thomas Bondo Pedersen , Simen Kvaal

It is shown that four-component (4C), quasi-four-component (Q4C), and exact two-component (X2C) relativistic Hartree-Fock (HF) equations can be implemented in an unified manner, by making use of the atomic nature of the small components of…

Chemical Physics · Physics 2023-11-28 Wenjian Liu

We present a fully numerical framework for the optimization of molecule-specific quantum chemical basis functions within the quantics tensor train format using a finite-difference scheme. The optimization is driven by solving the…

Chemical Physics · Physics 2025-06-12 Paul Haubenwallner , Matthias Heller

We introduce a novel energy functional for ground-state electronic-structure calculations. Its fundamental variables are the natural spin-orbitals of the implied singlet many-body wave function and their joint occupation probabilities. The…

Chemical Physics · Physics 2015-06-23 Ralph Gebauer , Morrel H. Cohen , Roberto Car

Closed-form expressions for the singular-potential integrals <m| x^-alpha |n> are obtained with respect to the Gol'dman and Krivchenkov eigenfunctions for the singular potential V(x) = B x^2 + A/x^2, B > 0, A >= 0. These formulas are…

Quantum Physics · Physics 2009-10-31 Richard L. Hall , Nasser Saad , Attila B. von Keviczky

We present a new adaptive method for electronic structure calculations based on novel fast algorithms for reduction of multivariate mixtures. In our calculations, spatial orbitals are maintained as Gaussian mixtures whose terms are selected…

Numerical Analysis · Mathematics 2019-06-19 Gregory Beylkin , Lucas Monzon , Xinshuo Yang

We propose a new, alternative method for ab-initio calculations of the electronic structure of solids, which has been specifically adapted to treat many-body effects in a more rigorous way than many existing ab-initio methods. We start from…

Condensed Matter · Physics 2007-05-23 I. Schnell , G. Czycholl , R. C. Albers

We take an additional step towards the optimization of the novel finite-range pseudopotential at constrained Hartree-Fock-Bogolyubov level and implement an optimization procedure within an axial code using harmonic oscillator basis. We…

Nuclear Theory · Physics 2020-09-03 T. Haverinen , M. Kortelainen , J. Dobaczewski , K. Bennaceur

The two-body Coulomb Hamiltonian, when calculated in Coulomb-Sturmian basis, has an infinite symmetric tridiagonal form, also known as Jacobi matrix form. This Jacobi matrix structure involves a continued fraction representation for the…

Mathematical Physics · Physics 2009-11-11 F. Demir , Z. T. Hlousek , Z. Papp

We compute the ground state energy of two atoms in a one-dimensional geometry of a harmonic optical trap. We obtain a dependence of the energy on a one-dimensional scattering length, which corresponds to various strengths of the interaction…

Atomic Physics · Physics 2015-06-16 I. S. Ishmukhamedov , D. S. Valiolda , S. A. Zhaugasheva

We formulate a hyperspherical approach within standard configuration interaction calculations aiming at a description of large-scale dynamics of $N$-particle system. The channel wave function and the adiabatic channel energy are determined…

Nuclear Theory · Physics 2018-12-05 Y. Suzuki , K. Varga

By extending the concept of Euler-angle rotations to more than three dimensions, we develop the systematics under rotations in higher-dimensional space for a novel set of hyperspherical harmonics. Applying this formalism, we determine all…

Atomic and Molecular Clusters · Physics 2015-06-26 T. A. Heim , D. Green
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