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We present measurements of magnetic field and frequency dependences of the low temperature (T = 1.8 K) AC-susceptibility, and temperature and field dependences of the longitudinal field positive muon spin relaxation ({\mu}SR) for…

Strongly Correlated Electrons · Physics 2015-06-05 R. C. Johnson , B. Z. Malkin , J. S. Lord , S. R. Giblin , A. Amato , C. Baines , A. Lascialfari , B. Barbara , M. J. Graf

We report the observation of para - antiferromagnetic transition at ~ 50 K in lithium iron phosphate, LiFePO4 through DC magnetization and M\"ossbauer spectroscopy. The Ferrous ion Fe2+ (3d6, 5D) in LiFePO4 exhibits relaxation effects with…

Materials Science · Physics 2015-06-04 Y. Sundarayya , C. Bansal , C. S. Sunandana , Ajay Kumar Mishra , Richard A. Brand , Horst Hahn

Temperature and magnetic field dependences of the 19F nuclear spin-lattice relaxation in a single crystal of LiYF4 doped with holmium are described by an approach based on a detailed consideration of the magnetic dipole-dipole interactions…

Other Condensed Matter · Physics 2011-10-04 B. Z. Malkin , M. V. Vanyunin , M. J. Graf , J. Lago , F. Borsa , A. Lascialfari , A. M. Tkachuk , B. Barbara

Strong hyperfine coupling in a 0.2% Holmium doped LiYF_4 single crystal induces staircaselike hysteresis loops of the magnetization at very low temperatures. The field sweep rate dependence of hysteresis loops allows the study of two…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 R. Giraud , W. Wernsdorfer , A. M. Tkachuk , D. Mailly , B. Barbara

Staircase hysteresis loops of the magnetization of a LiY_0.998Ho_0.002F_4 single crystal are observed at subkelvin temperatures and low field sweep rates. This behavior results from quantum dynamics at avoided level crossings of the energy…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 R. Giraud , W. Wernsdorfer , A. M. Tkachuk , D. Mailly , B. Barbara

We have carried out temperature-dependent inelastic neutron scattering measurements of YMnO3 over the temperature range 50 - 1303 K, covering both the antiferromagnetic to paramagnetic transition (70 K), as well as the ferroelectric to…

The effect of the electron-phonon interaction on magnetization relaxation is studied within the framework of first-principles scattering theory for Fe, Co, and Ni by displacing atoms in the scattering region randomly with a thermal…

Materials Science · Physics 2011-09-06 Yi Liu , Anton A. Starikov , Zhe Yuan , Paul J. Kelly

Experimental and theoretical studies of the dynamic magnetization in swept magnetic fields of the orthorhombic SrY$_2$O$_4$ single-crystals doped with the Dy$^{3+}$ Kramers ions (0.01 and 0.5 at.%) with natural abundances of even and odd Dy…

We have investigated the phonon and the magnetic excitations in LaCoO3 by inelastic neutron scattering measurements. The acoustic phonon dispersions show some characteristic features of the folded Brillouin zone (BZ) for the rhombohedrally…

Strongly Correlated Electrons · Physics 2009-11-11 Y. Kobayashi , Thant Sin Naing , M. Suzuki , M. Akimitsu , K. Asai , K. Yamada , J. Akimitsu , P. Manuel , J. M. Tranquada , G. Shirane

The crystal structure and lattice phonons of (BEDT-TTF)_2I_3 superconducting \beta-phase are computed and analyzed by the Quasi Harmonic Lattice Dynamics (QHLD) method. Whereas the crystal structure and its temperature and pressure…

Superconductivity · Physics 2024-11-26 A. Girlando , M. Masino , G. Visentini , R. G. Della Valle , A. Brillante , E. Venuti

We report on the spin waves and crystal field excitations in single crystal LiFePO$_4$ by inelastic neutron scattering over a wide range of temperatures, below and above the antiferromagnetic transition of this system. In particular, we…

Strongly Correlated Electrons · Physics 2017-03-15 Yuen Yiu , Manh Duc Le , Rasmus Toft-Peterson , Georg Ehlers , Robert McQueeney , David Vaknin

We report neutron inelastic scattering experiments on single crystal PbMg$_{1/3}$Nb$_{2/3}$O$_{3}$ doped with 32\% PbTiO$_{3}$, a relaxor ferroelectric that lies close to the morphotropic phase boundary. When cooled under an electric field…

Materials Science · Physics 2016-01-06 John A. Schneeloch , Zhijun Xu , B. Winn , C. Stock , P. M. Gehring , R. J. Birgeneau , Guangyong Xu

We present a comprehensive investigation of lattice dynamics in the double-helix antiferromagnet FeP by means of high-resolution time-of-flight neutron spectroscopy and ab-initio calculations. Phonons can hybridize with the magnetic…

Terahertz and far-infrared electric and magnetic responses of hexagonal piezomagnetic YMnO3 single crystals are investigated. Antiferromagnetic resonance is observed in the spectra of magnetic permeability mu_a [H(omega) oriented within the…

Materials Science · Physics 2012-02-13 C. Kadlec , V. Goian , K. Z. Rushchanskii , P. Kuzel , M. Lezaic , K. Kohn , R. V. Pisarev , S. Kamba

High-frequency dielectric studies of Bi_0.85Nd_0.15FeO_3 ceramics performed betweeen 100 and 900 K reveal hardening of most polar phonons on cooling below antiferroelectric phase transition, which occurs near 600 K. Moreover, a strong THz…

Materials Science · Physics 2011-10-18 V. Goian , S. Kamba , S. Greicius , D. Nuzhnyy , S. Karimi , I. M. Reaney

The interplay between different degrees of freedom such as charge, spin, orbital, and lattice has received a great deal of interest due to its potential to engineer materials properties and their functionalities for device applications. In…

Materials Science · Physics 2021-10-26 Bommareddy Poojitha , Ankit Kumar , Anjali Rathore , Devesh Negi , Surajit Saha

Density functional perturbation theory calculations of alpha-quartz using extended norm conserving pseudopotentials have been used to study the elastic properties and phonon dispersion relations along various high symmetry directions as a…

Materials Science · Physics 2007-05-23 N. Choudhury , S. L. Chaplot

Using Raman spectroscopy, we investigate the lattice phonons, magnetic excitations, and magneto-elastic coupling in the distorted triangular-lattice Heisenberg antiferromagnet alpha-SrCr2O4, which develops helical magnetic order below 43 K.…

Clear anomalies in the lattice thermal expansion (deviation from linear variation) and elastic properties (softening of the sound velocity) at the antiferromagnetic-to-paramagnetic transition are observed in the prototypical multiferroic…

We report on bifurcations effect mediated by the electron-phonon coupling in a concentrated rare-earth-containing antiferromagnet, observed in the spectra of coupled $4f$-electron-phonon modes under the influence of an external magnetic…

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