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A many-body Green's function approach to the microscopic theory of surface-enhanced Raman scattering is presented. Interaction effects between a general molecular system and a spatially anisotropic metal particle supporting plasmon…

Quantum Physics · Physics 2008-10-18 David J. Masiello , George C. Schatz

We investigate a system consisting of a single, as well as two emitters strongly coupled to surface plasmon modes of a nano-wire using a Green function approach. Explicit expressions are derived for the spontaneous decay rate into the…

Quantum Physics · Physics 2013-05-29 D. Dzsotjan , A. S. Sorensen , M. Fleischhauer

We derive expressions for the electromagnetic Green's function for a layered system using a transfer matrix technique. The expressions we arrive at makes it possible to study symmetry properties of the Green's function, such as reciprocity…

Mesoscale and Nanoscale Physics · Physics 2011-05-09 Peter Johansson

A numerical method for calculation electronic structure of a nanosystem composed of a pseudoisocyanine (PIC) molecule assembled on a silver nanoparticle is developed. The electronic structure of the silver nanoparticle containing 125 atoms…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 O. V. Farberovich , B. D. Fainberg , V. G. Maslov , V. Fleurov

The ability to manipulate plasmons is driving new developments in electronics, optics, sensing, energy, and medicine. Despite the massive momentum of experimental research in this direction, a predictive quantum-mechanical framework for…

Materials Science · Physics 2016-10-12 Fabio Caruso , Feliciano Giustino

In the framework of the many-electron s-d exchange model and Hubbard model, self-consistent equations are derived for the one-particle retarded Green's function in the many-electron Hubbard X-operator representation. We analyze the general…

Strongly Correlated Electrons · Physics 2015-06-03 A. O. Anokhin , A. V. Zarubin , V. Yu. Irkhin

Sub-wavelength arrays of quantum emitters offer an efficient free-space approach to coherent light-matter interfacing, using ultracold atoms or two-dimensional solid-state quantum materials. The combination of collectively suppressed…

Quantum Gases · Physics 2024-12-16 Simon Panyella Pedersen , Georg M. Bruun , Thomas Pohl

Effects of coupling between a molecular exciton and a surface plasmon (exciton-plasmon coupling) on the luminescence properties of the molecule and the surface plasmons are investigated using the nonequilibrium Green's function method.…

Materials Science · Physics 2013-06-12 Kuniyuki Miwa , Mamoru Sakaue , Hideaki Kasai

We investigate the dynamics of a plasmonic oscillation over a metal nanoparticle when it is strongly coupled to a quantum emitter (e.g. quantum dot, molecule). We simulate the density matrix evolution for a simple model; coupled…

Optics · Physics 2013-08-27 Mehmet Emre Tasgin

We theoretically investigate the interaction between a single molecule and a metallic nanoparticle. We develop a general quantum mechanical description for the calculation of the enhancement of radiative and non-radiative decay channels for…

Mesoscale and Nanoscale Physics · Physics 2008-01-28 Ulrich Hohenester , Andreas Truegler

Quantum many-body methods provide a systematic route to computing electronic properties of molecules and materials, but high computational costs restrict their use in large-scale applications. Due to the complexity in many-electron…

We investigate the optical response of a system consisting of periodic silver V-grooves interacting with quantum emitters. Two surface plasmon-polariton resonances are identified in the reflection spectrum of bare silver grooves, with the…

Optics · Physics 2015-08-05 Adam Blake , Maxim Sukharev

Localized surface plasmons are charge density oscillations confined to metallic nanoparticles. Excitation of localized surface plasmons by an electromagnetic field at an incident wavelength where resonance occurs results in a strong light…

Analysis of PDEs · Mathematics 2015-06-03 Habib Ammari , Pierre Millien , Matias Ruiz , Hai Zhang

We present a method to systematically study multi-photon transmission in one dimensional systems comprised of correlated quantum emitters coupled to input and output waveguides. Within the Green's function approach of the scattering matrix…

Quantum Physics · Physics 2017-05-24 Tian Feng See , Changsuk Noh , Dimitris G. Angelakis

We theoretically investigate the enhancement of surface enhanced Raman spectroscopy (SERS) using hyperbolic stratified nanostructures and compare to metal nanoresonators. The photon Green function of each nanostructure within its…

Theoretically, the presence of a metallic nanoparticle enhances the intermolecular energy transfer. We calculate this enhancement factor with a modal approach pertaining analytical results in the case of a nanosphere. We calculate the…

Mesoscale and Nanoscale Physics · Physics 2019-07-02 Titus Sandu , Catalin Tibeica , Oana Nedelcu , Mihai Gologanu

A quantum-mechanical model to calculate the electron energy-loss spectra (EELS) for the system of a closely located metallic nanoshell and a molecule has been developed. At the resonance between the molecular excitation and plasmon modes in…

Atomic Physics · Physics 2014-10-07 I. Yu. Goliney , Ye. V. Onykienko

Electron microscopy techniques such as electron energy-loss spectroscopy (EELS) facilitate the spatio-spectral characterization of plasmonic nanostructures. In this work, a time-dependent perspective is presented, which significantly…

To identify an analytical relation between the properties of polymers and their's monomer a Metal-Molecule-Metal (MMM) junction has been presented as an interesting and widely used object of research in which the molecule is a polymer which…

Mesoscale and Nanoscale Physics · Physics 2016-08-16 Mohammad Nakhaee , S Ahmad Ketabi

We develop a consistent quantum description of surface plasmons interacting with quantum emitters and external electromagnetic field. Within the framework of macroscopic electrodynamics in dispersive and absorptive medium, we derive, in the…

Mesoscale and Nanoscale Physics · Physics 2021-01-21 Tigran V. Shahbazyan
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