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We revisit strong-field ionization of aligned O$_2$, CO$_2$, and CS$_2$ molecules in light of recent advances in the field of strong-field physics, in particular the inclusion of multielectron polarization in the numerical solution of the…

Atomic Physics · Physics 2022-08-17 M. Abu-samha , Lars Bojer Madsen

We investigate dissociative single and double ionization of HeH+ induced by intense femtosecond laser pulses. By employing a semi-classical model with nuclear trajectories moving on field-dressed surfaces and ionization events treated as…

Atomic Physics · Physics 2018-10-24 Lun Yue , Philipp Wustelt , A. Max Sayler , Gerhard G. Paulus , Stefanie Gräfe

We develop an analytical model of correlated two-electron ionization in strong infrared laser fields. The model includes all relevant interactions between the electrons, the laser field, and the ionic core nonperturbatively. We focus on the…

Atomic Physics · Physics 2009-02-14 Denys I. Bondar , Wing-Ki Liu , Misha Yu. Ivanov

Ionization of highly charged relativistic ions by neutral atoms and ions is considered. Numerical results of recently developed computer codes based on the relativistic Born and the equivalent-photon approximations are presented. The…

Atomic Physics · Physics 2013-05-29 G. Baur , I. L. Beigman , V. P Shevelko , I. Yu. Tolstikhina , Th. Stoehlker

In this paper we study the response in time of N$_2$, O$_2$ and F$_2$ to laser pulses having a wavelength of 390nm. We find single ionization suppression in O$_2$ and its absence in F$_2$, in accordance with experimental results at $\lambda…

Quantum Physics · Physics 2009-11-10 Daniel Dundas , Jan M. Rost

Theoretical study on H$_2^+$ in an intense infrared laser field on the attosecond time-scale reveals that the molecular ion shows multiple bursts of ionization within a half-cycle of the laser field oscillation, in contrast to the widely…

Chemical Physics · Physics 2010-12-10 Norio Takemoto , Andreas Becker

The formation of an electron-hole plasma during the interaction of intense femtosecond laser pulses with transparent solids lies at the heart of femtosecond laser processing. Advanced micro- and nanomachining applications require improved…

An ultrarelativistic electron beam passing through an intense laser pulse emits radiation around its direction of propagation into a characteristic angular profile. Here we show that measurement of the variances of this profile in the…

Plasma Physics · Physics 2020-07-01 T. G. Blackburn , E. Gerstmayr , S. P. D. Mangles , M. Marklund

The two-photon decay in hydrogen-like ions is investigated within the framework of second order perturbation theory and Dirac's relativistic equation. Special attention is paid to the angular correlation of the emitted photons as well as to…

Atomic Physics · Physics 2014-10-23 P. Amaro , F. Fratini , S. Fritzsche , P. Indelicato , J. P. Santos , A. Surzhykov

The extension of coherent $\omega$-$2\omega$ control schemes, recently implemented in free-electron lasers (FELs), to molecular systems offers new opportunities to control chemical dynamics on the electronic timescale, potentially allowing…

We numerically investigate the dynamics of multiply charged hydrogenic ions in near-optical linearly polarized laser fields with intensities of order 10^16 to 10^17 W/cm^2. Depending on the charge state Z of the ion the relation of strength…

Quantum Physics · Physics 2009-11-06 S. X. Hu , C. H. Keitel

We consider the elastic scattering of electrons by hydrogen atoms in the presence of a two-color circularly polarized laser field in the domain of moderate intensities below $10^{13}$ W/cm$^2$ and high projectile energies. A hybrid approach…

Atomic Physics · Physics 2023-06-16 Gabriela Buica

The photodissociation of the HD+ molecular ion in intense short- pulsed linearly polarized laser fields is studied using a time- dependent wave-packet approach where molecular rotation is fully included. We show that applying a coherent…

chem-ph · Physics 2019-04-04 Eric Charron , Annick Giusti-Suzor , Frederick Mies

We present a combined experimental and theoretical study on strong-field ionization of a three-dimensionally oriented asymmetric top molecule, benzonitrile (C$_7$H$_5$N), by circularly polarized, nonresonant femtosecond laser pulses. Prior…

We present experimental data on the non-adiabatic strong field ionization of atomic hydrogen using elliptically polarized femtosecond laser pulses at a central wavelength of 390 nm. Our measured results are in very good agreement with a…

The motion of electrons and ions in medium-sized rare gas clusters (1000 atoms) exposed to intense laser pulses is studied microscopically by means of classical molecular dynamics using a hierarchical tree code. Pulse parameters for optimum…

Atomic and Molecular Clusters · Physics 2007-05-23 Ulf Saalmann , Jan-Michael Rost

In order to elucidate the correlated motion of atomic electrons, we investigate the attosecond-scale dynamics of their entanglement arising due to nonsequential ionization driven by a strong, linearly-polarized laser field. The calculation…

Atomic Physics · Physics 2024-03-18 Daniel Younis , Songbo Xie , Joseph H. Eberly

We present a numerical method for investigating the non-perturbative quantum mechanical interaction of light with atoms in two dimensions, without a basis expansion. This enables us to investigate intense laser-atom interactions with light…

Quantum Physics · Physics 2009-10-30 M. Protopapas , D. G. Lappas , P. L. Knight

Few-cycle pulses of intense 800 nm light are used to probe ionization and dissociation of carbon disulfide in the intensity and temporal regime where rescattering is expected to dominate the laser-molecule interaction. The wavepacket of the…

In this paper a 4-component Dirac theory of ionization of hydrogen molecular ion in a super-intense laser field is developed. Simple analytic expressions for the spin specific as well as the total ionization currents emitted from the ground…

Atomic Physics · Physics 2015-05-13 F. H. M. Faisal