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We present a new theory that the molecular high order harmonic generation in an intense laser field is determined by molecular internal symmetry and momentum distribution of the tunneling-ionized electron. The molecular internal symmetry…

Atomic Physics · Physics 2008-01-30 J. Chen , Y. J. Chen , J. Fan , J. Liu , S. G. Chen , X. T. He

High-order harmonic generation (HHG) in gases has been studied for almost 40 years in many different conditions, varying the laser wavelength, intensity, focusing geometry, target design, gas species, etc. However, no systematic…

In strong laser-atom interactions, the Coulomb potential can affect the trajectories of rescattering electron in high-order harmonic generation (HHG). Here, by constructing a semi-analytical Coulomb-included model and comparing it with…

Atomic Physics · Physics 2025-12-16 Yigen Peng , Jiayin Che , Ruihua Xu , Shang Wang , Xuejiao Xie , Yanjun Chen

The rotational excitation of the three asymmetric-top molecular ion isotopologues H$_2$O$^+$, HDO$^+$, and D$_2$O$^+$ is studied theoretically using a combined framework of electron-molecule R-matrix scattering theory, multichannel…

Atomic Physics · Physics 2026-03-19 Joshua Forer

We describe a method of selective generation and study of polarization moments of up to the highest rank $\kappa=2F$ possible for a quantum state with total angular momentum $F$. The technique is based on nonlinear magneto-optical rotation…

Atomic Physics · Physics 2009-11-10 V. V. Yashchuk , D. Budker , W. Gawlik , D. F. Kimball , Yu. P. Malakyan , S. M. Rochester

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

Strongly Correlated Electrons · Physics 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

The selection rules of high harmonic generation (HHG) are investigated using three-dimensional time-dependent density functional theory (TDDFT). From the harmonic spectra obtained with various real molecules and different forms of laser…

Atomic Physics · Physics 2016-09-28 Xi Liu , Xiaosong Zhu , Liang Li , Yang Li , Qingbin Zhang , Pengfei Lan , Peixiang Lu

To sum up, we show in the present paper that magnetic response in Nb$_2$O$_2$F$_3$ at the high-temperatures ($T>$90 K) is related to the orbital selective regime, when part of the electrons form molecular orbitals while other electrons have…

Materials Science · Physics 2017-05-24 V. V. Gapontsev , D. I. Khomskii , S. V. Streltsov

Using the one-dimensional Hubbard model, which is commonly used for describing, e.g., high-$T_c$ superconducting cuprates, we study high-harmonic generation (HHG) from doped, correlated materials. Doping is modeled by changing the number of…

Strongly Correlated Electrons · Physics 2023-01-04 Thomas Hansen , Lars Bojer Madsen

A theoretical optimization method of high-harmonic-generation (HHG) is developed in the framework of optimal-control-theory (OCT). The target of optimization is the emission radiation of a particular frequency. The OCT formulation includes…

Quantum Physics · Physics 2020-02-19 Ido Schaefer , Ronnie Kosloff

We extend the semi-classical trajectory description for the high-order harmonic generation~(HHG) from solids by integrating the effect of electron-scattering. Comparing the extended semi-classical trajectory model with a one-dimensional…

We study the high harmonic generation with vortex beams beyond the dipole approximation. To do so we employ the full minimal coupling approach to account for multipolar coupling without truncation and describe the full spatio-temporal…

Atomic Physics · Physics 2026-01-21 Esra Ilke Albar , Valeriia P. Kosheleva , Heiko Appel , Angel Rubio , Franco P. Bonafé

We study high-order harmonic generation in aligned molecules close to the ionization threshold. Two distinct contributions to the harmonic signal are observed, which show very different responses to molecular alignment and ellipticity of…

Atomic Physics · Physics 2011-09-16 H. Soifer , P. Botheron , D. Shafir , A. Diner , O. Raz , B. D. Bruner , Y. Mairesse , B. Pons , N. Dudovich

High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

High harmonic generation (HHG) is a versatile technique for probing ultrafast electron dynamics. While HHG is sensitive to the electronic properties of the target, HHG also depends on the waveform of the laser pulse. As is well known,…

Real-space picture of electron recollision with the parent ion guides our understanding of the highly nonlinear response of atoms and molecules to intense low-frequency laser fields. It is also among several leading contestants for the…

Optics · Physics 2019-11-06 Mrudul M. S. , Adhip Pattanayak , Misha Ivanov , Gopal Dixit

High-order harmonic responses from three $C_{20}$ isomers: fullerene, ring, and bowl, are calculated within the modified Lewenstein model for molecular systems. Spectra for all three structures exhibit intense modulations of the harmonic…

Quantum Physics · Physics 2022-03-31 F. Cajiao - Vélez , A. Jaron

We employ the two-band density-matrix equations and time-dependent density functional theory to calculate high-order harmonic generation (HOHG) in graphene under a femtosecond laser irradiation. Our investigation uncovers a striking…

Atomic Physics · Physics 2023-07-25 Fulong Dong , Qinzhi Xia , Jie Liu

High order harmonic generation from clusters is a controversial topic: conflicting theories exist, with different explanations for similar experimental observations. From an experimental point of view, separating the contributions from…

Atomic and Molecular Clusters · Physics 2015-06-12 H. Ruf , C. Handschin , R. Cireasa , N. Thiré , A. Ferré , S. Petit , D. Descamps , E. Mével , E. Constant , V. Blanchet , B. Fabre , Y. Mairesse

We study numerically the Bloch electron wavepacket dynamics in periodic potentials to simulate laser-solid interactions. We introduce a new perspective in the coordinate space combined with the motion of the Bloch electron wavepackets…

Optics · Physics 2018-01-12 Tao-Yuan Du , Xiao-Huan Huang , Xue-Bin Bian
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