Related papers: Detection of high-power two-mode squeezing by sum-…
Sum-frequency generation (SFG) allows for coherent upconversion of an electromagnetic signal and has applications in mid-infrared vibrational spectroscopy of molecules. Recent experimental and theoretical studies have shown that plasmonic…
We propose non-phase-matched sum frequency generation (SFG) as a method for characterizing broadband multimode light. We demonstrate its advantages using high-gain parametric down conversion (PDC) as an example. By generating the sum…
We experimentally demonstrate shaping of the two-photon wavefunction of entangled photon-pairs, utilizing coherent pulse-shaping techniques. By performing spectral-phase manipulations we tailor the two-photon wavefunction exactly like a…
We report on the experimental observation of non-resonant, second-order optical Sum-Frequency Generation (SFG) in five different atomic and molecular gases. The measured signal is attributed to a SFG process by characterizing its intensity…
Triple sum-frequency (TSF) spectroscopy is a recently-developed methodology that enables collection of multidimensional spectra by resonantly exciting multiple quantum coherences of vibrational and electronic states. This work reports the…
We investigate the generation of squeezed Fock states (SFSs) via particle-number measurements in the modes of multimode Gaussian states. We identify a universal class of $N$-mode Gaussian states for which measuring $N-1$ modes results in…
We propose a computational framework to extract non-linear response functions from real-time simulations in the presence of more than one external field. We apply this approach to the calculation of sum frequency generation (SFG) and…
Sum-frequency generation (SFG) is a powerful second-order nonlinear spectroscopic technique that provides detailed insights into molecular structures and absolute orientations at surfaces and interfaces. However, conventional SFG based on…
Much work over the last 25 years has demonstrated that the interface-specific, alloptical technique, vibrational sum frequency generation (v-SFG) spectroscopy, is often uniquely capable of characterizing the structure and dynamics of…
High-harmonic generation (HHG) has recently emerged as a promising method for generating non-classical states of light with frequencies spanning from the infrared up to the extreme ultraviolet regime. In this work, we theoretically…
We present a new technique for the detection of two-mode squeezed states of light that allows for a simple characterization of these quantum states. The usual detection scheme, based on heterodyne measurements, requires the use of a local…
Sum-frequency generation (SFG) spectroscopy provides a versatile method for the investigation of non-centrosymmetric media and interfaces. Here, using tunable picosecond infrared (IR) pulses from a free-electron laser, the nonlinear optical…
Frequency-degenerate photon pairs generated using nonlinear photonic integrated devices are a crucial resource for scalable quantum information processing and metrology. However, their realization is hindered by unwanted parametric…
We propose, analyze, and evaluate a technique for the joint measurement of time-frequency entanglement between two photons. In particular, we show that the frequency sum and time difference of two photons could be simultaneously measured…
An efficient broadband sum frequency generation (SFG) technique using the two collinear optical parametric processes \omega 3=\omega 1+\omega 2 and \omega 4=\omega 1+\omega 3 is proposed. The technique uses chirped quasi-phase-matched…
Vibrational sum frequency generation (SFG) spectroscopy is a powerful technique for investigating molecular structures, orientations, and dynamics at surfaces. However, its spatial resolution is fundamentally restricted to the micrometer…
Absorption spectroscopy is a widely used technique that permits the detection and characterization of gas species at low concentrations. We propose a sensing strategy combining the advantages of frequency modulation spectroscopy with the…
High harmonic generation is a resource of extremely broad frequency combs of ultrashort light pulses. The non-classical nature of this new quantum source has been recently evidenced in semiconductors by showing that high harmonic generation…
Squeezed, nonclassical states are an integral tool of quantum metrology due to their ability to push the sensitivity of a measurement apparatus beyond the limits of classical states. While their creation in light has become a standard…
Absorption and gain processes are fundamental to any light-matter interaction and a precise measurement of these parameters is important for various scientific and technological applications. Quantum probes, specifically the squeezed states…