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Related papers: Rotational excitation of methylidynium (CH+) by a …

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Chloronium (H$_2$Cl$^+$) is an important intermediate of Cl-chemistry in space. The accurate knowledge of its collisional properties allows a better interpretation of the corresponding observations in interstellar clouds and therefore a…

Chemical Physics · Physics 2024-12-31 Sándor Demes , Dariusz Kędziera , Alexandre Faure , François Lique

The availability of collisional rate coefficients with H$_2$ is a pre-requisite for interpretation of observations of molecules whose energy levels are populated under non local thermodynamical equilibrium conditions. In the current study,…

Astrophysics of Galaxies · Physics 2015-06-22 F. Daniel , A. Faure , L. Wiesenfeld , E. Roueff , D. C. Lis , P. Hily-Blant

Modeling of molecular emission from interstellar clouds requires the calculation of rates for excitation by collisions with the most abundant species. The present paper focuses on the calculation of rate coefficients for rotational…

Astrophysics of Galaxies · Physics 2015-05-18 E. Sarrasin , D. Ben Abdallah , M. Wernli , A. Faure , J. Cernicharo , F. Lique

Cross sections and rate coefficients for rovibronic excitation of the CH$^+$ ion by electron impact and dissociative recombination of CH$^+$ with electrons are evaluated using a theoretical approach combining an R-matrix method and…

Astrophysics of Galaxies · Physics 2025-11-25 Joshua Forer , Dávid Hvizdoš , Mehdi Ayouz , Chris H. Greene , Viatcheslav Kokoouline

Collisional excitation rate coefficients play an important role in the dynamics of energy transfer in the interstellar medium. In particular, accurate rotational excitation rates are needed to interpret microwave and infrared observations…

Solar and Stellar Astrophysics · Physics 2015-06-10 Benhui Yang , K. M. Walker , R. C. Forrey , P. C. Stancil , N. Balakrishnan

A detailed interpretation of the detected emission lines of environments in which propyne (or methyl acetylene, CH$_3$CCH) is observed requires a knowledge of its collisional rate coefficients with the most abundant species in the…

Astrophysics of Galaxies · Physics 2024-02-28 M. Ben Khalifa , B. Darna , J. Loreau

Rotational transitions in molecular hydrogen collisions are computed. The two most recently developed potential energy surfaces for the H2-H2 system are used from the following works: 1) A.I. Boothroyd, P.G. Martin, W.J. Keogh, M.J.…

Chemical Physics · Physics 2009-11-11 Renat A. Sultanov , Dennis Guster

We report rotational quenching cross sections and rate coefficients of HCl due to collisions with He. The close-coupling method and the coupled-states approximation are applied in quantum-mechanical scattering calculations of state-to-state…

Solar and Stellar Astrophysics · Physics 2015-06-18 Benhui Yang , Phillip C. Stancil

Rates for rotational excitation of HC3N by collisions with He atoms and H2 molecules are computed for kinetic temperatures in the range 5-20K and 5-100K, respectively. These rates are obtained from extensive quantum and quasi-classical…

Chemical Physics · Physics 2009-11-13 Michael Wernli , Laurent Wiesenfeld , Alexandre Faure , Pierre Valiron

Among all closed-shell species observed in molecular clouds, molecules with C$_{3v}$ symmetry play a crucial role, as their rotational spectroscopy allows them to behave as a gas thermometer. In the interstellar medium, methyl cyanide…

Astrophysics of Galaxies · Physics 2023-09-22 M. Ben Khalifa , P. J. Dagdigian , J. Loreau

Among the numerous molecular systems found in the interstellar medium (ISM), vinyl cyanide is the first identified olephinic nitrile. While it has been observed in various sources, its detection in Sgr B2 is notable as the 2$_{11}$-2$_{12}$…

Astrophysics of Galaxies · Physics 2025-06-23 Karina Sogomonyan , Malek Ben Khalifa , Jérôme Loreau

We present quantum mechanical and quasiclassical trajectory calculations of cross sections for rovibrational transitions in ortho- and para-H_2 induced by collisions with He atoms. Cross sections were obtained for kinetic energies between…

Astrophysics · Physics 2007-05-23 N. Balakrishnan , M. Vieira , J. F. Babb , R. C. Forrey , A. Dalgarno , S. Lepp

We present quantum dynamical calculations that describe the rotational excitation of H$_2$O due to collisions with H atoms. We used a recent, high accuracy potential energy surface, and solved the collisional dynamics with the…

Astrophysics of Galaxies · Physics 2015-06-23 F. Daniel , A. Faure , P. J. Dagdigian , M. -L. Dubernet , F. lique , G. Pineau des forêts

New calculations for rotational excitation of cyanoacetylene by collisions with hydrogen molecules are performed to include the lowest 38 rotational levels of HC3N and kinetic temperatures to 300 K. Calculations are based on the interaction…

Astrophysics of Galaxies · Physics 2016-06-15 A. Faure , F. Lique , L. Wiesenfeld

A theoretical method for the estimation of cross sections and rates for excitation and charge transfer processes in low-energy hydrogen atom collisions with neutral atoms, based on an asymptotic two-electron model of ionic-covalent…

Atomic Physics · Physics 2016-05-04 Paul S. Barklem

Cross sections for the rotational (de)excitation of CO by ground state para- and ortho-H_2 are obtained using quantum scattering calculations for collision energies between 1 and 520 cm^{-1}. A new CO-H_2 potential energy surface is…

Astrophysics · Physics 2008-11-26 M. Wernli , P. Valiron , A. Faure , L. Wiesenfeld , P. Jankowski , K. Szalewicz

Rate coefficient for state-to-state rotational transitions in H+ collision with CS has been obtained using accurate quantum dynamical close-coupling calculations to interpret microwave astronomical observations. Accurate three dimensional…

Chemical Physics · Physics 2016-04-19 Rajwant Kaur , T. J. Dhilip Kumar

We present a detailed theoretical study of the rotational excitation of CH$^+$ due to reactive and nonreactive collisions involving C$^+(^2P)$, H$_2$, CH$^+$, H and free electrons. Specifically, the formation of CH$^+$ proceeds through the…

We have studied the fundamental rotational relaxation and excitation collision of OH- J=0 <-> 1 with helium at different collision energies. Using state-selected photodetachment in a cryogenic ion trap, the collisional excitation of the…

We have measured the dependence of the relative integral cross section of the reaction Li+HF-->LiF+H on the collision energy using crossed molecular beams. By varying the intersection angle of the beams from 37{\deg} to 90{\deg} we covered…

Chemical Physics · Physics 2011-12-19 Rolf Bobbenkamp , Hansjurgen Loesch , Marcel Mudrich , Frank Stienkemeier
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