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The solid diffusive phase transformation involving the nucleation and growth of one nucleus is universal and frequently employed but has not yet been fully understood at the atomic level. Here, our first-principles calculations reveal a…

Materials Science · Physics 2023-09-12 Junyuan Bai , Hongbo Xie , Xueyong Pang , Min Jiang , Gaowu Qin

The crystal structure of iron in the Earth's inner core remains debated. Most recent experiments suggest a hexagonal-close-packed (hcp) phase. In simulations, it has been generally agreed that the hcp-Fe is stable at inner core pressures…

Geophysics · Physics 2018-04-17 Rostislav Hrubiak , Yue Meng , Guoyin Shen

It has long been assumed the Earth's solid inner core started to grow when molten iron cooled to its melting point. However, the nucleation mechanism, which is a necessary step of crystallization, has not been well understood. Recent…

Geophysics · Physics 2022-01-11 Yang Sun , Feng Zhang , Mikhail I. Mendelev , Renata M. Wentzcovitch , Kai-Ming Ho

Grain growth competition during directional solidification of a polycrystal with hexagonal (hcp) symmetry (Mg-1wt%Gd alloy) is studied by phase-field modeling, exploring the effect of the temperature gradient G on the resulting grain…

Materials Science · Physics 2024-03-15 A. K. Boukellal , M. Sarebanzadeh , A. Orozco-Caballero , F. Sket , J. LLorca , D. Tourret

We have studied the high-pressure iron bcc to hcp phase transition by simultaneous X-ray Magnetic Circular Dichroism (XMCD) and X-ray Absorption Spectroscopy (XAS) with an X-ray dispersive spectrometer. The combination of the two techniques…

Other Condensed Matter · Physics 2009-11-10 O. Mathon , F. Baudelet , J. P. Itie , A. Polian , M. D'Astuto , J. C. Chervin , S. Pascarelli

The nucleation of crystals from the liquid melt is often characterized by a competition between different crystalline structures or polymorphs, and can result in nuclei with heterogeneous compositions. These mixed-phase nuclei can display…

Soft Condensed Matter · Physics 2021-08-26 Fabio Leoni , John Russo

By using a phase-field crystal (PFC) model, the liquid-crystal growth of the plastic triangular phase is simulated with emphasis on crystal shape and topological defect formation. The equilibrium shape of a plastic triangular crystal (PTC)…

Soft Condensed Matter · Physics 2017-08-07 Sai Tang , Simon Praetorius , Rainer Backofen , Axel Voigt , Yan-Mei Yu , Jincheng Wang

We report simulations on the homogeneous liquid-fcc nucleation of charged colloids for both low and high contact energy values. As a precursor for crystal formation, we observe increased local order at the position where the crystal will…

Soft Condensed Matter · Physics 2014-11-03 Kai Kratzer , Axel Arnold

We determine the full kinetic phase diagram for nucleation and growth of crystal phases in a suspension of charged colloids. We calculate nucleation barrier heights for face-centered cubic (fcc) and body-centered cubic (bcc) crystal phases…

Soft Condensed Matter · Physics 2022-08-31 Willem Gispen , Marjolein Dijkstra

We apply a simple dynamical density functional theory, the phase-field crystal (PFC) model of overdamped conservative dynamics, to address polymorphism, crystal nucleation, and crystal growth in the diffusion-controlled limit. We refine the…

Materials Science · Physics 2015-05-18 Gyula I. Tóth , György Tegze , Tamás Pusztai , László Gránásy

An electron diffraction study of nucleation and growth of the hcp phase in large pure Ar and mixed Ar-Kr clusters formed by supersonic jet expansion is carried out. The threshold cluster size corresponding to the appearance of an hcp phase…

Atomic and Molecular Clusters · Physics 2014-11-18 O. G. Danylchenko , S. I. Kovalenko , O. P. Konotop , V. N. Samovarov

Metastable phases can lead to multistep nucleation processes, influencing the liquid-to-solid transition in various systems. In this study, we investigate the homogeneous nucleation of iron's crystalline phases under Earth's inner core…

Geophysics · Physics 2025-04-04 Chen Gao , Kai-Ming Ho , Renata M. Wentzcovitch , Yang Sun

Plasticity in body-centered cubic (BCC) nanocrystals is often associated with twin nucleation phenomena under extreme loading conditions. Here, we reveal unconventional twinning pathways that operate at the intersection of crystal…

Homogeneous nucleation from aluminum (Al) melt was investigated by million-atom molecular dynamics (MD) simulations utilizing the second nearest neighbor modified embedded atom method (MEAM) potentials. The natural spontaneous homogenous…

Materials Science · Physics 2019-05-02 Avik Mahata , Mohsen Asle Zaeem , Michael I. Baskes

Nanocrystalline Ni can adopt a hexagonal close-packed (hcp) structure,which does not appear in a bulk form under any conditions.Structural studies found its $>$ 20% expansion of volume per atom compared with face-centered cubic (fcc)…

We investigate the basic thermal, mechanical and structural properties of body centred cubic iron ($\alpha$-Fe) at several temperatures and positive loading by means of Molecular Dynamics simulations in conjunction with the embedded-atom…

Materials Science · Physics 2017-02-17 Kostadin G. Gaminchev

In this paper, the effect of twin boundaries on the crack growth behaviour of single crystal BCC Fe has been investigated using molecular dynamics simulations. The growth of an atomically sharp crack with an orientation of (111)$<$110$>$…

Materials Science · Physics 2021-12-02 G. Sainath , A. Nagesha

We present an atomistic description of the {\it fcc}--to--{\it hcp} transformation mechanism in solid argon (Ar) obtained from transition path sampling molecular dynamics simulation. The phase transition pathways collected during the…

Materials Science · Physics 2017-06-28 Bingxi Li , Guangrui Qian , Artem R. Oganov , Salah Eddine Boulfelfel , Roland Faller

A full understanding of polycrystalline materials requires studying the process of nucleation, a thermally activated phase transition that typically occurs at atomistic scales. The numerical modeling of this process is problematic for…

Materials Science · Physics 2018-05-09 Paul Jreidini , Gabriel Kocher , Nikolas Provatas
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