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The four most stable structures of Ni$_N$ clusters with $N$ from 2 to 150 have been determined using a combination of the embedded-atom method in the version of Daw, Baskes and Foiles, the {\it variable metric/quasi-Newton} method, and our…

Atomic and Molecular Clusters · Physics 2016-09-08 V. G. Grigoryan , M. Springborg

C58 fullerenes were adsorbed onto room temperature Au(111) surface by low-energy (~6 eV) cluster ion beam deposition under ultrahigh vacuum conditions. The topographic and electronic properties of the deposits were monitored by means of…

Packing transitions in the lowest energy structures of Li clusters as a function of size have been identified via simulated annealing. For N>21, the large $p$ character of Li leads to unexpected ionic structures. At N~25, a packing pattern…

chem-ph · Physics 2009-10-22 Ming Wen Sung , Ryoichi Kawai , John H. Weare

Monoatomic chains of molybdenum encapsulated in single walled carbon nanotubes of different chiralities are investigated using density functional theory. We determine the optimal size of the carbon nanotube for encapsulating a single atomic…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 A. García-Fuente , V. M. García-Suárez , J. Ferrer , A. Vega

The thermochemistry of the carbon clusters C$_n$ (n=2--10) has been revisited by means of W4 theory and W3.2lite theory. Particularly the larger clusters exhibit very pronounced post-CCSD(T) correlation effects. Despite this, our best…

Chemical Physics · Physics 2010-08-26 Amir Karton , Alex Tarnopolsky , Jan M. L. Martin

Using a systematic search algorithm we identify several types of point defects in the boron fullerene with 80 atoms. All these point defect leave the cage structure intact. In addition the cage structure is also very stable with respect to…

Materials Science · Physics 2009-02-11 Kuo Bao , Stefan Goedecker , Luigi Genovese , Alexey Neelov , S. Alireza Ghasemi , Thierry Deutsch

We show that C$_{60}$ fullerene molecules can serve as promising building blocks in the construction of versatile crystal structures with unique symmetries using first-principles calculations. These phases include quasi-2D layered…

Mesoscale and Nanoscale Physics · Physics 2025-04-03 Darius Kayley , Bo Peng

The fullerene (C60) nanowires, which possess a highly unusual morphology featured by a prism-like central core and three nanobelt-like wings joined along the growth direction to give an overall Y-shaped cross section, have been studied. The…

Chemical Physics · Physics 2009-02-03 Junfeng Geng , Ilia A. Solov'yov , Wuzong Zhou , Andrey V. Solov'yov , Brian F. G. Johnson

From first-principles calculations, we predict that a single ethylene molecule can form a stable complex with two transition metals (TM) such as Ti. The resulting TM-ethylene complex then absorbs up to ten hydrogen molecules, reaching to…

Other Condensed Matter · Physics 2009-11-11 Engin Durgun , Salim Ciraci , W. Zhou , Taner Yildirim

We design antiferromagnetic spin-1/2 chains in fullerene nanoribbons by introducing extra C$_{60}$ cages at one of their edges. The resulting odd number of intermolecular bonds induces an unpaired $\pi$-electron and hence a quantised…

Materials Science · Physics 2025-09-12 Bo Peng , Michele Pizzochero

The interaction between substitutional nitrogen atoms in graphene is studied by performing first principles calculations. The nearest neighbor interaction between nitrogen dopants is highly repulsive because of the strong electrostatic…

Materials Science · Physics 2015-03-19 Hongjun Xiang , Bing Huang , Zhenyu Li , Su-Huai Wei , Jinlong Yang , Xingao Gong

How to stabilize nitrogen-rich high-energy-density molecules under conventional conditions is particularly important for the energy storage and conversion of such systems and has attracted extensive attention. In this work, our theoretical…

Chemical Physics · Physics 2023-08-10 Zhen Gong , Rui Wang , Famin Yu , Chenxi Wan , Xinrui Yang , Zhigang Wang

Strutinsky shell corrections for the Cesium-coated fullerenes were investigated. The single particle levels of electrons are obtained using the spherical mean-field potential of a shifted Wood-Saxon type. The parameters of the potential are…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 P. Mierzynski , K. Pomorski

The current paper opens a series of papers that are aimed at the determination of barriers that govern the covalent coupling between partners of C60-based composites consisting of two or more fullerenes C60 (C60 dimer and oligomers) (Part…

Materials Science · Physics 2011-06-07 E. F. Sheka , L. Kh. Shaymardanova

We review the recent theoretical treatment of fullerenes as pi-conjugated systems. Polaronic properties due to the Jahn-Teller type effects are mainly discussed. (1) A Su-Schrieffer-Heeger type electron-phonon model is applied to…

Condensed Matter · Physics 2008-11-26 Kikuo Harigaya

A systematic theoretical study of stoichiometric clusters (NaI)n up to n=15 is performed using the ab initio Perturbed-Ion (PI) model. The structures obtained are compared to previous pair potential results, and observed differences between…

Atomic and Molecular Clusters · Physics 2009-09-25 A. Aguado , A. Ayuela , J. M. Lopez , J. A. Alonso

Group 14 Zintl clusters are promising molecular building blocks for nanoscale architecture. Endohedral variants, which encapsulate d/f-block metals within p-block semimetal cages, provide insights into intermetallic bonding and compound…

Materials Science · Physics 2026-01-08 Xue Wu , Wen-Shuai Dai , Lulu Li , Fangying Hao , Hong-Guang Xu , Wei-Jun Zheng , Jijun Zhao

Sodium chloride (NaCl), a ubiquitous and chemically stable compound, has been considered inert under ambient conditions. Its typical B1 structure is highly isotropic without preferential direction, favoring the growth of a three-dimensional…

Materials Science · Physics 2025-01-24 Ping Ning , Yifan Tian , Guangtao Liu , Hongbo Wang , Qingyang Hu , Hanyu Liu , Mi Zhou , Yanming Ma

Semiconducting nanoparticles are the building blocks of optical nanodevices as their electronic states, and therefore light absorption and emission, can be controlled by modifying their size and shape. CdSe is perhaps the most studied of…

Materials Science · Physics 2015-06-25 Silvana Botti , Miguel A. L. Marques

Using first-principles methods we performed a theoretical study of carbon clusters in silicon carbide nanowires. We examined small clusters with carbon interstitials and antisites in hydrogen-passivated SiC nanowires growth along the [100]…

Materials Science · Physics 2011-07-21 J. M. Morbec , R. H. Miwa