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Raman scattering in relaxor ferroelectric PbMg1/3Ta2/3O3 (PMT) was investigated in the single crystalline form in the temperature range of 20 - 295 K. Anomalous temperature dependence of the integrated intensity and the Raman line contours…

Materials Science · Physics 2007-05-23 S. G. Lushnikov , S. N. Gvasaliya , R. S. Katiyar

We report lattice dynamical measurements, made using neutron inelastic scattering methods, of the relaxor perovskite PbMg1/3Nb2/3O3 (PMN) at momentum transfers near the edge of the Brillouin zone. Unusual"columns" of phonon scattering that…

Materials Science · Physics 2015-05-13 I. P. Swainson , C. Stock , P. M. Gehring , Guangyong Xu , K. Hirota , Y. Qiu , H. Luo , X. Zhao , J. -F. Li , D. Viehland

Neutron scattering techniques have been used to study the relaxor ferroelectric 0.68PbMg1/3Nb2/3O3-0.32PbTiO3 denoted in this paper as 0.68PMN-0.32PT. On cooling, these relaxor ferroelectrics have a long-range ordered ferroelectric phase…

Materials Science · Physics 2007-05-23 S. N. Gvasaliya , B. Roessli , R. A. Cowley , S. Kojima , S. G. Lushnikov

Neutron and x-ray diffraction techniques have been used to study the competing long and short-range polar order in the relaxor ferroelectric Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$ (PMN) under a [111] applied electric field. Despite reports of a…

Materials Science · Physics 2009-11-13 C. Stock , Guangyong Xu , P. M. Gehring , H. Luo , X. Zhao , H. Cao , J. F. Li , D. Viehland , G. Shirane

A quite unusual diffuse scattering phenomenology was observed in the single-crystal X-ray diffraction pattern of cubic perovskite BMT ($\mathrm{BaMg}_{1/3}\mathrm{Ta}_{2/3}\mathrm{O}_3$). The intensity of the scattering is parametrized as a…

Relaxor ferroelectric PbMg_1/3Ta_2/3O_3 ceramics and thin films were investigated by means of broad-band dielectric, time-domain terahertz (THz) and Fourier-transform infrared (IR) spectroscopy in the frequency range 100 Hz - 90 THz at…

Materials Science · Physics 2009-11-13 S. Kamba , D. Nuzhnyy , S. Veljko , V. Bovtun , J. Petzelt , Y. L. Wang , J. Levoska , M. Tyunina , J. Macutkevic , N. Setter , J. Banys

The relaxors Pb(Zn$_{1/3}$Nb$_{2/3}$)O$_{3}$ (PZN) and Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$ (PMN) have very similar properties based on the dielectric response around the critical temperature $T_{c}$ (defined by the structural transition under…

Materials Science · Physics 2009-11-10 C. Stock , R. J. Birgeneau , S. Wakimoto , J. S. Gardner , W. Chen , Z. -G. Ye , G. Shirane

The low-energy part of the vibration spectrum in PbMg$_{1/3}$Nb$_{2/3}$O$_3$ (PMN) relaxor ferroelectric has been studied by neutron scattering above and below the Burns temperature, T$_d$. The transverse acoustic and the lowest transverse…

Materials Science · Physics 2007-05-23 S N Gvasaliya , B Roessli , R A Cowley , P Hubert , S G Lushnikov

We have used neutron scattering techniques to characterize the diffuse scattering and lattice dynamics in single crystals of the relaxor PMN from 10K to 900K. We observed two distinct types of diffuse scattering. The first is weak,…

Materials Science · Physics 2009-06-11 P. M. Gehring , H. Hiraka , C. Stock , S. -H. Lee , W. Chen , Z. -G. Ye , S. B. Vakhrushev , Z. Chowdhuri

Using neutron elastic and inelastic scattering and high-energy x-ray diffraction, we present a comparison of 40% Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$-60% PbTiO$_{3}$ (PMN-60PT) with pure Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$ (PMN) and PbTiO$_{3}$…

Materials Science · Physics 2009-11-11 C. Stock , D. Ellis , I. P. Swainson , Guangyong Xu , H. Hiraka , Z. Zhong , H. Luo , X. Zhao , D. Viehland , R. J. Birgeneau , G. Shirane

Neutron inelastic scattering measurements of the polar TO phonon mode in the cubic relaxor Pb(Mg1/3Nb2/3)O3, at room temperature, reveal anomalous behavior similar to that recently observed in the Pb(Zn1/3Nb2/3)_{0.92}Ti_{0.08}O3 system in…

Materials Science · Physics 2009-10-31 P. M. Gehring , S. B. Vakhrushev , G. Shirane

We discovered a near room temperature lead-free relaxor-ferroelectric (Ba0.6Bi0.2Li0.2)TiO3 (BBLT) having A-site compositional disordered ABO3 perovskite structure. Microstructure-property relations revealed that the chemical…

Materials Science · Physics 2016-06-22 Hitesh Borkar , Vaibhav Rao , Soma Dutta , Arun Barvat , Prabir Pal , M Tomar , Vinay Gupta , J. F. Scott , Ashok Kumar

Pb(Zn$_{1/3}$Nb$_{2/3}$)O$_{3}$ is one of the simplest representatives of the lead ferroelectric relaxors. Its solid solution with PbTiO$_{3}$, at concentrations near the morphotropic phase boundary, is especially important. In this paper,…

Materials Science · Physics 2007-05-23 O. Svitelskiy , D. La-Orauttapong , J. Toulouse , W. Chen , Z. -G. Ye

Previously reported neutron scattering investigations of the canonical relaxor ferroelectric perovskite oxide with a chemical formula Pb(Mg(1/3)Nb(2/3))O3 (PMN) are revisited in order to appreciate the role of the intrinsic bulk…

Materials Science · Physics 2026-05-12 J. Hlinka

The response of polar nanoregions (PNR) in the relaxor compound Pb[(Zn$_{1/3}$Nb$_{2/3}$)$_{0.92}$Ti$_{0.08}$]O$_3$ subject to a [111]-oriented electric field has been studied by neutron diffuse scattering. Contrary to classical…

Materials Science · Physics 2009-11-11 Guangyong Xu , P. M. Gehring , G. Shirane

Local structural distortions in Na0.5Bi0.5TiO3-based solid solutions have been proved to play a crucial role in understanding and tuning their enhanced piezoelectric properties near the morphotropic phase boundary. In this work all local…

Materials Science · Physics 2017-10-06 Alexandra Neagu , Cheuk-Wai Tai

The complex interaction between transverse acoustic (TA) phonon, transverse optic (TO) phonon and polar nano-domains (PND) in the relaxor ferroelectric KTa1-xNbxO3 (KTN) is studied by means of high resolution diffuse and inelastic neutron…

Mesoscale and Nanoscale Physics · Physics 2016-09-08 J. Toulouse , E. Iolin , B. Hennion , D. Petitgrand , G. Yong , R. Erwin

Using neutron pair distribution function (PDF) analysis over the temperature range from 1000 K to 15 K, we demonstrate the existence of local polarization and the formation of medium-range, polar nanoregions (PNRs) with local rhombohedral…

Disordered Systems and Neural Networks · Physics 2009-11-10 I. -K. Jeong , T. W. Darling , J. K. Lee , Th. Proffen , R. H. Heffner , J. S. Park , K. S. Hong , W. Dmowski , T. Egami

The symmetry was examined using neutron diffraction method on Pb(Zn1/3Nb2/3)O3 -9%PbTiO3 (PZN/9PT) which has a composition at the morphotropic phase boundary (MPB) between Pb(Zn1/3Nb2/3)O3 and PbTiO3. The results were compared with those of…

We report neutron inelastic scattering measurements of the lowest-energy transverse optic (TO) phonon branch in the relaxor Pb(Mg_1/3Nb_2/3)O_3 from 400 to 1100 K. Far above the Burns temperature T_d ~ 620 K we observe well-defined…

Materials Science · Physics 2009-11-07 P. M. Gehring , S. Wakimoto , Z. -G. Ye , G. Shirane