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Related papers: Vibrational interference of Raman and high-harmoni…

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The influence of multiple vibrational modes on current fluctuations in electron transport through single-molecule junctions is investigated. Our analysis is based on a generic model of a molecular junction, which comprises a single…

Mesoscale and Nanoscale Physics · Physics 2014-09-26 C. Schinabeck , R. Härtle , H. B. Weber , M. Thoss

We present a combined experimental and theoretical study of resonant Raman spectroscopy in single- and triple-layer MoTe$_2$. Raman intensities are computed entirely from first principles by calculating finite differences of the dielectric…

We describe the collisional interaction between two different atoms that are trapped in a harmonic potential. The atoms are exposed to a magnetic field, which is modulated in the vicinity of an s-wave Feshbach resonance, and we study the…

Other Condensed Matter · Physics 2007-06-29 Jesper Fevre Bertelsen , Klaus Molmer

When a high power laser beam irradiates a small aperture on a solid foil target, the strong laser field drives surface plasma oscillation at the periphery of this aperture, which acts as a "relativistic oscillating window". The diffracted…

Plasma Physics · Physics 2021-04-07 Longqing Yi

High resolution low frequency Raman scattering measurements from embedded AgAu nanoparticles unveil efficient scattering by harmonics of both the quadrupolar and the spherical modes. Comparing the experimental data with theoretical…

Mesoscale and Nanoscale Physics · Physics 2009-06-02 S. Adichtchev , S. Sirotkin , G. Bachelier , L. Saviot , S. Etienne , B. Stephanidis , E. Duval , A. Mermet

Discussed is the structure of classical and quantum excitations of internal degrees of freedom of multiparticle objects like molecules, fullerens, atomic nuclei, etc. Basing on some invariance properties under the action of isometric and…

Quantum Physics · Physics 2010-12-17 J. J. Sławianowski , V. Kovalchuk , B. Gołubowska , A. Martens , E. E. Rożko

A mechanism is explored whereby intense laser radiation induces an optical force between the constituent atoms of a molecule. In the case of a diatomic molecule the effect results in a modification of the vibrational potential, and using…

Optics · Physics 2007-05-23 D. L. Andrews R. G. Crisp

We consider the nonequilibrium quantum vibrations of a molecule clamped between two macroscopic leads in a current-carrying state at finite voltages. Our approach is based on the nonequilibrium Green function technique and the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 D. A. Ryndyk , M. Hartung , G. Cuniberti

Inelastic (Raman) light scattering intensities for a 42-electron quantum dot under off-resonance conditions and in different spin and angular momentum channels are computed in order to test whether final collective states become the…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Augusto Gonzalez , Alain Delgado

The generation of harmonics by atoms interacting with two circularly polarized and frequency related laser fields is addressed through ab initio numerical simulations. A detailed charaterization of a few specific harmonics is given. In…

Atomic Physics · Physics 2009-11-10 F. Ceccherini , N. Davini , D. Bauer , F. Cornolti

Quantum coherence is highly involved in photochemical functioning of complex molecular systems. Co-existence and intermixing of electronic and/or vibrational coherences, while never unambiguously identified experimentally, has been proposed…

We establish how the intensities of the higher harmonics that arise when a photoelectron recombines with a parent ion depend functionally on the parameters of the laser wave and atomic medium, and estimate the limiting values of these…

Optics · Physics 2017-04-19 M. A. Kutlan

Existence of different types of interference in the spectrum of radiation emitted by a doubly hard scattered electron is demonstrated. The spectrum develops oscillations in two regions: the hard, where the oscillations depend on the…

Accelerator Physics · Physics 2017-04-05 M. V. Bondarenco , N. F. Shul'ga

We describe how to treat the interaction of travelling electrons with localised vibrational modes in nanojunctions. We present a multichannel scattering technique which can be applied to calculate the transport properties for realistic…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 H. Ness , A. J. Fisher

The Raman intensity can be well described by the famous Albrecht equation that consists of A and B terms. It is well known that the contribution from Albrecht's A term can be neglected without loss of accuracy for far off-resonant Raman…

Optics · Physics 2015-11-11 Zu-Yong Gong , Guangjun Tian , Sai Duan , Yi Luo

Electron-phonon and electron-electron interactions are in competition in determining the properties of molecular charge transfer conductors and superconductors. The direct influence of phonons on the electron-electron interaction was not…

Strongly Correlated Electrons · Physics 2009-10-31 M. Meneghetti

We derive the transition rates, dephasing rates, and Lamb shifts for a system consisting of many molecules collectively coupled to a resonant cavity mode. Using a variational polaron master equation, we show that strong vibrational…

Quantum Physics · Physics 2024-07-24 Dominic M Rouse , Erik M Gauger , Brendon W Lovett

This paper introduces Bohmian mechanics (BM) into the intense laser-atom physics to study high-order harmonic generation. In BM, the trajectories of atomic electrons in intense laser field can be obtained with the Bohm-Newton equation. The…

Atomic Physics · Physics 2015-05-14 X. Y. Lai , Q. Y. Cai , M. S. Zhan

When molecules interact with intense light sources of femtosecond or shorter duration the rotational degrees of freedom are frozen during the response to the strong nonperturbative interaction. We show how the frozen degrees of freedom…

Atomic Physics · Physics 2007-09-25 C. B. Madsen , A. S. Mouritzen , T. K. Kjeldsen , L. B. Madsen

We present experimental observations of interference between an atomic spin coherence and an optical field in a {\Lambda}-type gradient echo memory. The interference is mediated by a strong classical field that couples a weak probe field to…

Quantum Physics · Physics 2013-05-29 G. T. Campbell , M. Hosseini , B. M. Sparkes , P. K. Lam , B. C. Buchler