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The influence of on-site (Hubbard) electron-electron interaction on disorder-induced localization is studied in order to clarify the role of electronic spin. The motivation is based on the recent experimental indications of a…

Mesoscale and Nanoscale Physics · Physics 2011-01-20 Moshe Goldstein , Richard Berkovits

We present a simple and efficient method to incorporate anharmonic effects in the vibrational \textcolor{black}{analyses} of molecules within density functional theory (DFT) calculations. This approach is closely related to the traditional…

We developed a general framework for hybrid quantum-classical computing of molecular and periodic embedding approaches based on an orbital space separation of the fragment and environment degrees of freedom. We demonstrate its potential by…

Chemical Physics · Physics 2024-12-23 Stefano Battaglia , Max Rossmannek , Vladimir V. Rybkin , Ivano Tavernelli , Jürg Hutter

Electronic structure calculation of atoms and molecules, in the past few decades has largely been dominated by density functional methods. This is primarily due to the fact that this can account for electron correlation effects in a…

Chemical Physics · Physics 2013-07-12 Amlan K. Roy

Conductivity is one of the most direct probes of electronic systems, yet its theoretical description remains challenging in the presence of strong non-local correlations. In this Letter, we analyze the conductivity of the half-filled…

Strongly Correlated Electrons · Physics 2026-03-13 Nagamalleswararao Dasari , Hugo U. R. Strand , Martin Eckstein , Alexander I. Lichtenstein , Evgeny A. Stepanov

We present a formulation of the density-functional theory + Hubbard model (DFT+U) method that is self-consistent over the choice of Hubbard projectors used to define the correlated subspaces. In order to overcome the arbitrariness in this…

Materials Science · Physics 2015-03-17 David D. O'Regan , Nicholas D. M. Hine , Mike C. Payne , Arash A. Mostofi

We perform investigation of Hubbard model with interaction between strongly correlated conducting electrons on a lattice with Debye phonons. To solve the problem generalized dynamical mean-field DMFT+\Sigma method is employed with…

Strongly Correlated Electrons · Physics 2009-10-02 E. Z. Kuchinskii , I. A. Nekrasov , M. V. Sadovskii

Despite its widespread use, the predictive accuracy of density functional theory (DFT) is hampered by delocalization errors, especially for correlated systems such as transition-metal complexes. Two complementary tuning strategies have been…

Materials Science · Physics 2022-04-11 Yael Cytter , Aditya Nandy , Akash Bajaj , Heather J. Kulik

Detailed analysis of the magnetic properties of the Hubbard model within dynamical mean-field theory (DMFT) is presented. Using a RPA-like decoupling of two-particle propagators we derive a universal form for susceptibilities, which…

Strongly Correlated Electrons · Physics 2012-01-06 Sebastian Schmitt , Norbert Grewe , Torben Jabben

The mechanism of Mott transition in the Hubbard model on the square lattice is studied without explicit introduction of magnetic and superconducting correlations, using a variational Monte Carlo method. In the trial wave functions, we…

Strongly Correlated Electrons · Physics 2015-05-27 Tomoaki Miyagawa , Hisatoshi Yokoyama

The realistic description of correlated electron systems has taken an important step forward a few years ago as the combination of density functional methods and the dynamical mean-field theory was conceived. This framework allows access to…

Strongly Correlated Electrons · Physics 2011-06-15 M. Karolak , T. O. Wehling , F. Lechermann , A. I. Lichtenstein

Electronic correlated systems are often well described by dynamical mean field theory (DMFT). While DMFT studies have mainly focused hitherto on one-particle properties, valuable information is also enclosed into local two-particle Green's…

Strongly Correlated Electrons · Physics 2012-09-25 Georg Rohringer , Angelo Valli , Alessandro Toschi

We have performed a systematic study of the emergence of meta-stable states in density functional theory plus Hubbard U (DFT+U ) simulations of NiO, CoO, FeO. Particular attention is given to the spin-polarization of the…

Materials Science · Physics 2018-10-25 Samara Keshavarz , Patrik Thunström

Hubbard-like Hamiltonians are widely used to describe on-site Coulomb interactions in magnetic and strongly-correlated solids, but there is much confusion in the literature about the form these Hamiltonians should take for shells of p and d…

Strongly Correlated Electrons · Physics 2016-02-10 M. E. A. Coury , S. L. Dudarev , W. M. C. Foulkes , A. P. Horsfield , Pui-Wai Ma , J. S. Spencer

We study the nature of spin excitations of individual transition metal atoms (Ti, V, Cr, Mn, Fe, Co and Ni) deposited on a Cu$_2$N/Cu(100) surface using both spin-polarized density functional theory (DFT) and exact diagonalization of an…

Mesoscale and Nanoscale Physics · Physics 2016-08-08 Alejandro Ferrón , Jose Luis Lado , Joaquín Fernández-Rossier

In the context of the modified Becke-Johnson (mBJ) potential, we recently underlined that $\bar{g}$, the average of $\left\vert\nabla\rho\right\vert/\rho$ in the unit cell, has markedly different values in transition-metal oxides and pure…

Materials Science · Physics 2022-01-04 Leila Kalantari , Fabien Tran , Peter Blaha

Since the preliminary work of Anisimov and co-workers, the Hubbard corrected DFT+$U$ functional has been used for predicting properties of correlated materials by applying on-site effective Coulomb interactions to specific orbitals.…

Materials Science · Physics 2022-12-20 Stefano Falletta , Alfredo Pasquarello

The dual boson approach [Ann. Phys. 327, 1320 (2012)] provides a means to construct a diagrammatic expansion around the extended dynamical mean-field theory (EDMFT). In this paper, we present the numerical implementation of the approach and…

We study the role of electron correlations in the presumed type II Weyl semimetallic candidate $\gamma$-MoTe$_2$ by employing density functional theory (DFT) where the on-site Coulomb repulsion (Hubbard U) for the Mo 4$d$ states is included…

Strongly Correlated Electrons · Physics 2019-01-16 Niraj Aryal , Efstratios Manousakis

We implement a multi-orbital cluster dynamical mean-field theory (DMFT), by improving a sample-update algorithm in the continuous-time quantum Monte Carlo method based on the interaction expansion. The proposed sampling scheme for the…

Strongly Correlated Electrons · Physics 2014-08-20 Yusuke Nomura , Shiro Sakai , Ryotaro Arita