Related papers: Four Wave Mixing Spectroscopy at the Interface Bet…
We present an efficient scheme for the generation and control of a degenerate four-wave mixing (FWM) signal in a N-type inhomogeneously broadened 85Rb atomic system. We observe the propagation dynamics of the generated FWM signal along with…
Nonlinear wave mixing in the X-ray range can provide valuable insights into the structural and electron dynamics of atomic and molecular systems on ultrafast time scales, with state- and site-selectivity and atomic resolution. This…
This tutorial provides a joint theoretical and experimental overview of heterodyne wave mixing spectroscopy, focusing mainly on four-wave mixing (FWM). This powerful and versatile time-resolved nonlinear optical spectroscopy technique…
Non-collinear four-wave mixing (FWM) techniques at near-infrared (NIR), visible, and ultraviolet frequencies have been widely used to map vibrational and electronic couplings, typically in complex molecules. However, correlations between…
New feasibity of coherent quantum control of four-wave mixing processes in a resonant Doppler-broadened medium are studied. We propose a technique which enables one to enhance the quantum efficiency of nonlinear optical conversion. At the…
We study nearly degenerate four-wave mixing using a two-photon-allowed vibrational transition of parahydrogen. A signal photon is generated by a trigger photon and coherence among parahydrogen, which is prepared by two counterpropagating…
We demonstrate phase super-resolution in the absence of entangled states. The key insight is to use the inherent time-reversal symmetry of quantum mechanics: our theory shows that it is possible to \emph{measure}, as opposed to prepare,…
We study theoretically the time-resolved four-wave mixing (FWM) response of an ensemble of pairs of quantum dots undergoing radiative recombination. At short (picosecond) delay times, the response signal shows beats that may be dominated by…
New experimental techniques based on non-linear ultrafast spectroscopies have been developed over the last few years, and have been demonstrated to provide powerful probes of quantum dynamics in different types of molecular aggregates,…
We describe a method for non-degenerate four-wave mixing in a cold sample of 4-level atoms. An integral part of the four-wave mixing process is a collective instability which spontaneously generates a periodic density modulation in the cold…
We theoretically investigate a N-type 87Rb atomic system for efficient generation and control of a non-degenerate Four wave mixing (FWM) signal in pulsed regime. The susceptibility of the atomic medium is customized as a gain profile by a…
A setup to frequency-convert an arbitrary image encoded in the spatial profile of a probe field onto a signal field using four-wave mixing in a thermal atom vapor is proposed. The atomic motion is exploited to cancel diffraction of both…
We present an experimental and theoretical study of photon pairs generated by spontaneous four wave mixing (SFWM), based on birefringent phasematching, in a fiber which supports more than one transverse mode. We present SFWM spectra,…
Phase imaging techniques extract the optical path-length information of a scene, whereas wavefront sensors provide the shape of an optical wavefront. Since these two applications have different technical requirements, they have developed…
The power spectrum of an optical field can be acquired without a spectrally resolving detector by means of Fourier-transform spectrometry, based on measuring the temporal autocorrelation of the optical field. Analogously, we here perform…
Phase-mismatch in nonlinear optical processes can severely limit the propagation and conversion efficiency of light fields. Here, we present an efficient optimal-control strategy to mitigate the detrimental effects of phase-mismatch in an…
We experimentally demonstrate four-wave-mixing spectroscopy using frequency combs. The experiment uses a geometry where excitation pulses and four-wave-mixing signals generated by a sample co-propagate. We separate them in the radio…
Three-color coherent anti-Stokes Raman scattering represents non-degenerate four wave mixing process that includes both a non-resonant and resonant processes, the contributions of which depend on how the molecular vibrational modes are…
This paper introduces a novel technique for reconstructing the phase of modified spectrograms of audio signals. From the analysis of mixtures of sinusoids we obtain relationships between phases of successive time frames in the…
The phase transition to mirrorless oscillation in resonantly enhanced four-wave mixing in double-$\Lambda$ systems are studied analytically for the ideal case of infinite lifetimes of ground-state coherences. The stationary susceptibilities…