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The pyrochlore lattice is associated with several potential and actual spin liquid phases as a result of its strong geometric frustration. At finite temperature, these can exhibit an unusually broad cross-over regime to a conventional…

Strongly Correlated Electrons · Physics 2020-03-09 Akshat Pandey , Roderich Moessner , Claudio Castelnovo

We argue that classical pyrochlore Heisenberg antiferromagnets with small further-neighbor couplings can order in a state where pairs of sublattices form antiparallel spirals. The spiral ordering wave vectors of the two pairs are in general…

Strongly Correlated Electrons · Physics 2023-07-18 Cecilie Glittum , Olav F. Syljuåsen

Classical spin-liquids are paramagnetic phases which feature nontrivial patterns of spin correlations within their ground-state manifold whose degeneracy scales with system size. Often they harbor fractionalized excitations, and their…

Strongly Correlated Electrons · Physics 2024-11-26 Daniel Lozano-Gómez , Yasir Iqbal , Matthias Vojta

Above 40K, the magnetic susceptibility of the heavy Fermion spinel LiV2O4 has many features in common with those of geometrically frustrated magnetic insulators, while its room temperature resistivity comfortably exceeds the Mott-Regel…

Strongly Correlated Electrons · Physics 2009-11-07 Nic Shannon

A formation of tetrahedral spin clusters is discovered by Monte Carlo simulation for a spin-ice type double-exchange model on a pyrochlore lattice. The spin-cluster phase is magnetically disordered, but breaks spatial inversion symmetry…

Strongly Correlated Electrons · Physics 2014-08-29 Hiroaki Ishizuka , Yukitoshi Motome

Pyrochlore lattices, which are found in two important classes of materials -- the $A_2B_2X_7$ pyrochlore family and the $AB_2X_4$ spinel family -- are the quintessential 3-dimensional frustrated lattice architecture. While historically…

Strongly Correlated Electrons · Physics 2021-05-05 Dalmau Reig-i-Plessis , Alannah M. Hallas

We have theoretically studied successive transitions in vanadium spinel oxides with (t_2g)^2 electron configuration. These compounds show a structural transition at ~ 50K and an antiferromagnetic transition at ~ 40K. Since threefold t_2g…

Strongly Correlated Electrons · Physics 2009-11-11 Yukitoshi Motome , Hirokazu Tsunetsugu

We study the stability of some strongly frustrated antiferromagnetic spin lattices in high magnetic fields against lattice distortions. In particular, we consider a spin-s anisotropic Heisenberg antiferromagnet on the square-kagom\'{e} and…

Strongly Correlated Electrons · Physics 2016-08-16 Oleg Derzhko , Johannes Richter , Jörg Schulenburg

Motivated by puzzling spin-glass behaviors observed in many pyrochlore-based magnets, effects of magnetoelastic coupling to local lattice distortions were recently studied by the authors for a bond-disordered antiferromagnet on a pyrochlore…

Strongly Correlated Electrons · Physics 2013-07-25 Hiroshi Shinaoka , Yusuke Tomita , Yukitoshi Motome

We present a comprehensive neutron scattering study of the breathing pyrochlore magnet LiGaCr4S8. We observe an unconventional magnetic excitation spectrum with a separation of high and low-energy spin dynamics in the correlated…

The ground-state properties of the spin-1 pyrochlore antiferromagnet are studied by applying the VBS-like tetrahedron-unit decomposition to the original spin system. The symmetrization required on every vertex is taken into account by…

Strongly Correlated Electrons · Physics 2009-11-07 Yasufumi Yamashita , Kazuo Ueda , Manfred Sigrist

Understanding spin-lattice coupling represents a key challenge in modern condensed matter physics, with crucial importance and implications for ultrafast and 2D-magnetism. The efficiency of angular momentum and energy transfer between spins…

Spin-1 antiferromagnets are abundant in nature, but few theories or results exist to understand their general properties and behavior, particularly in situations when geometric frustration is present. Here we study the $S=1$ Kagome compound…

Strongly Correlated Electrons · Physics 2020-04-29 Arpita Paul , Chia-Min Chung , Turan Birol , Hitesh J. Changlani

Spinel compounds AB$_{2}$X$_{4}$ consist of both tetrahedral (AX$_{4}$) and octahedral (BX$_{6}$) environments with the former forming a diamond lattice and the latter a geometrically frustrated pyrochlore lattice. Exploring the fascinating…

Chemical Physics · Physics 2023-03-29 Qiang Zhang , Wei Tian , Roshan K. Nepal , Ashfia Huq , Stephen Nagler , J. F. DiTusa , Rongying Jin

We investigate quantum phase transitions for the $s=1/2$ antiferromagnetic Heisenberg model on a pyrochlore lattice. By means of a series expansion starting from isolated tetrahedra, the ground-state phase diagram is determined. When the…

Strongly Correlated Electrons · Physics 2009-10-31 Akihisa Koga , Norio Kawakami

The pyrochlore lattice, a three-dimensional network of corner-sharing tetrahedra, is a promising material playground for correlated topological phases arising from the interplay between spin-orbit coupling (SOC) and electron-electron…

Magnetic ordering in the geometrically frustrated magnetic oxide spinels MgCr_2O_4 and ZnCr_2O_4 is accompanied by a structural change that helps relieve the frustration. Analysis of high-resolution synchrotron X-ray scattering reveals that…

Dielectric study on Ca3Mn2O7 features relaxor-like segmented dynamics below the antiferromagnetic ordering. Dipolar relaxations of different origin are spectrally resolved exhibiting distinct H-field alterations. This identifies their…

Materials Science · Physics 2019-09-10 Pooja Sahlot , Gaurav Sharma , Vasant Sathe , Anand Mohan Awasthi

We reveal the significance of kinetic-driven multiple-spin interactions hidden in geometrically-frustrated Kondo lattice models. Carefully examining the perturbation in terms of the spin-charge coupling up to the fourth order, we find that…

Strongly Correlated Electrons · Physics 2015-06-03 Yutaka Akagi , Masafumi Udagawa , Yukitoshi Motome

Most works on pyrochlore magnets deal with the interacting spin-1/2 local moments. We here study the spin-one local moments on the pyrochlore lattice, and propose a generic interacting spin model on a pyrochlore lattice. Our spin model…

Strongly Correlated Electrons · Physics 2018-07-11 Fei Ye Li , Gang Chen