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Complex colloidal fluids, such as emulsions stabilized by complex shaped particles, play an important role in many industrial applications. However, understanding their physics requires a study at sufficiently large length scales while…

Soft Condensed Matter · Physics 2012-04-27 Florian Günther , Florian Janoschek , Stefan Frijters , Jens Harting

We present a nonlocal electrostatic formulation of nonuniform ions and water molecules with interstitial voids that uses a Fermi-like distribution to account for steric and correlation effects in electrolyte solutions. The formulation is…

Soft Condensed Matter · Physics 2017-03-27 Jinn-Liang Liu , Dexuan Xie , Bob Eisenberg

The standard model for diffuse charge phenomena in colloid science, electrokinetics and biology is the Poisson-Boltzmann mean-field theory, which breaks down for multivalent ions and large surface charge densities due to electrostatic…

Soft Condensed Matter · Physics 2020-02-14 J. Pedro de Souza , Martin Z. Bazant

We theoretically study electrostatic properties of electric double layer using a generalized Poisson-Boltzmann approach taking into account the orientational ordering of water dipoles and the excluded volume effect of water molecules as…

Soft Condensed Matter · Physics 2022-02-14 Jun-Sik Sin , Song-Jin Im , Kwang-Il Kim

The Poisson-Boltzmann mean-field description of ionic solutions has been successfully used in predicting charge distributions and interactions between charged macromolecules. While the electrostatic model of charged fluids, on which the…

Soft Condensed Matter · Physics 2014-04-22 Dan Ben-Yaakov , David Andelman , Daniel Harries , Rudi Podgornik

We investigate sedimentation of model hard sphere-like colloidal dispersions confined in horizontal capillaries using laser scanning confocal microscopy, dynamical density functional theory, and Brownian dynamics computer simulations. For…

Soft Condensed Matter · Physics 2009-11-13 C. Patrick Royall , Joachim Dzubiella , Matthias Schmidt , Alfons van Blaaderen

A theoretical model of shape-anisometric particles embedded in a cubic lattice is formulated for binary mixtures combining rod-like, plate-like and spherical particles. The model aims at providing a tool for the prediction and…

Soft Condensed Matter · Physics 2011-05-31 Stavros Peroukidis , Alexandros G. Vanakaras , Demetri J. Photinos

We present a continuation of our theoretical research into the influence of co-solvent polarizability on a differential capacitance of the electric double layer [EPL 111, 28002 (2015)]. We formulate a modified Poisson-Boltzmann theory,…

Soft Condensed Matter · Physics 2016-05-11 Yu. A. Budkov , A. L. Kolesnikov , M. G. Kiselev

We consider a nonlinear drift-diffusion system for multiple charged species in a porous medium in 2D and 3D with periodic microstructure. The system consists of a transport equation for the concentration of the species and Poisson's…

Analysis of PDEs · Mathematics 2022-06-16 Apratim Bhattacharya , Markus Gahn , Maria Neuss-Radu

We apply general variational techniques to the problem of the counterion distribution around highly charged objects where strong condensation of counterions takes place. Within a field-theoretic formulation using a fluctuating electrostatic…

Soft Condensed Matter · Physics 2009-11-07 Roland R. Netz , Henri Orland

Dense packing of particles has provided important models to study the structure of matter in various systems such as liquid, glassy and crystalline phase, etc. The simplest sphere packing models are able to represent and capture salient…

Soft Condensed Matter · Physics 2023-03-03 Weihao Wang , Zhenghong Chen , Yang Gao , Yang Jiao , Shaodong Zhang

We further study the stochastic model discussed in Ref.[2] in which positive and negative particles diffuse in an asymmetric, CP invariant way on a ring. The positive particles hop clockwise, the negative counter-clockwise and…

Statistical Mechanics · Physics 2007-05-23 Peter F. Arndt , Vladimir Rittenberg

This paper extends a recently introduced theory describing particle transport for random statistically homogeneous systems in which the distribution function p(s) for chord lengths between scattering centers is non-exponential. Here, we…

Mathematical Physics · Physics 2016-02-03 Richard Vasques , Edward W. Larsen

In this paper we present a new model for modeling the diffusion and relative dispersion of particles in homogeneous isotropic turbulence. We use an Heisenberg-like Hamiltonian to incorporate spatial correlations between fluid particles,…

Fluid Dynamics · Physics 2012-12-18 Thomas Burgener , Dirk Kadau , Hans Jürgen Herrmann

We derive a formally simple approximate analytical solution to the Poisson-Boltzmann equation for the spherical system via a geometric mapping. Its regime of applicability in the parameter space of the spherical radius and the surface…

Soft Condensed Matter · Physics 2012-02-01 Zhenwei Yao , Mark J. Bowick , Xu Ma

We derive the charge density up to second order in spatial gradient in inhomogeneous crystals using the semiclassical coarse graining procedure based on the wave packet method. It can be recast as divergence of polarization, whose…

Mesoscale and Nanoscale Physics · Physics 2021-10-15 Yiqiang Zhao , Yang Gao , Di Xiao

In this paper we study the electrostatic properties of `Janus' spheres with unequal charge densities on both hemispheres. We introduce a method to compare primitive-model Monte Carlo simulations of the ionic double layer with predictions of…

Soft Condensed Matter · Physics 2012-09-18 Joost de Graaf , Niels Boon , Marjolein Dijkstra , René van Roij

In this paper we extend the homogenization results obtained in (G. Allaire, A. Mikeli\'c, A. Piatnitski, J. Math. Phys. 51 (2010), 123103) for a system of partial differential equations describing the transport of a N-component electrolyte…

Analysis of PDEs · Mathematics 2020-09-14 Andro Mikelic , Andrey Piatnitski

The effective electrostatic interaction between a pair of colloids, both of them located close to each other at an electrolyte interface, is studied by employing the full, nonlinear Poisson-Boltzmann (PB) theory within classical density…

Soft Condensed Matter · Physics 2016-08-17 Arghya Majee , Markus Bier , S. Dietrich

The description of a conducting medium in thermal equilibrium, such as an electrolyte solution or a plasma, involves nonlinear electrostatics, a subject rarely discussed in the standard electricity and magnetism textbooks. We consider in…

Chemical Physics · Physics 2018-08-01 C. G. Gray , P. J. Stiles