Related papers: Arbitrary multi-site two-photon excitation in four…
Two-photon excitation is an attractive means for controlling chemistry in both space and time. Isoenergetic one- and two-photon excitations (OPE and TPE) in non-centrosymmetric molecules are often assumed to reach the same excited state…
We have formulated and experimentally demonstrated an improved algorithm for design of arbitrary two-dimensional holographic traps for ultracold atoms. Our method builds on the best previously available algorithm, MRAF, and improves on it…
Two-dimensional (2D) photonic crystals offer strong control over the propagation of light through their bands. Theoretical methods for computing the band structure in 2D are well-established and fast because 2D photonic crystals are…
A spatial quantum model of spontaneous parametric down-conversion in nonlinear layered structures is developed expanding the interacting vectorial fields into monochromatic plane waves. A two-photon spectral amplitude depending on the…
Optical dynamics in van der Waals heterobilayers is of fundamental scientific and practical interest. Based on a time-dependent adiabatic GW approach, we discover a new many-electron (excitonic) channel for converting photoexcited…
Two-dimensional (2D) material heterostructures have attracted considerable attention owing to their interesting and novel physical properties, which expand the possibilities for future optoelectronic, photovoltaic, and nanoelectronic…
We demonstrate necessary and sufficient conditions of the local convergence of the alternating projection algorithm to a unique solution up to a global phase factor. Additionally, for the ptychography imaging problem, we discuss phase…
Digital holography numerically restores three-dimensional image information using optically captured diffractive waves. The required bandwidth is larger than that of hologram pixel at a closer distance in the Fresnel diffraction regime,…
Bacteriorhodopsin (bR) is a light-driven proton pump. We use time-resolved crystallography at an X-ray free-electron laser to follow the structural changes in multiphoton-excited bR from 250 femtoseconds to 10 picoseconds. Quantum chemistry…
We demonstrate a two-dimensional time-domain spectroscopy method to extract amplitude and phase modifications of excited atomic states caused by the interaction with ultrashort laser pulses. The technique is based on Fourier analysis of the…
We report a systematic methodology to obtain supermodes with equidistant effective index distribution and to excite arbitrary target supermodes with high precision. By employing a multi-well optical potential realized by a judiciously…
Silicon photonics provides a versatile platform for large-scale integration of optical functions, but its weak intrinsic nonlinear response limits the realization of active, intensity-dependent functionalities. Hybrid integration of…
We introduce a new modality for dynamic phase imaging in confocal microscopy based on synthetic optical holography. By temporal demultiplexing of the detector signal into a series of holograms, we record time-resolved phase images directly…
High-dimensional quantum information processing has emerged as a promising avenue to transcend hardware limitations and advance the frontiers of quantum technologies. Harnessing the untapped potential of the so-called qudits necessitates…
Multimode multiphoton states are at the center of many photonic quantum technologies, from photonic quantum computing to quantum sensing. In this work, we derive a procedure to generate exactly, and with a predictable number of steps, any…
Ultrafast single-shot imaging techniques now reach frame rates of tens of tera-frame-per-second (Tfps) and long sequence depths but are often too complex for large-scale use, both in terms of image acquisition and reconstruction. We propose…
Optical solitary waves (solitons) that interact in a nonlinear system can bind and form a structure similar to a molecule. The rich dynamics of this process have created a demand for rapid spectral characterization to deepen the…
Here, by making use of medium and high resolution autocorrected off-axis electron holography, we directly probe the electrostatic potential as well as in-plane and out-of-plane charge delocalization at edges and steps in multilayer…
Two-photon excitation spectroscopy is a nonlinear technique that has gained rapidly in interest and significance for studying the complex energy-level structure and transition probabilities of materials. While the conventional spectroscopy…
Photonic lattices enable experimental exploration of transport and localization phenomena, two of the mayor goals in physics and technology. In particular, the optical excitation of some lattice sites which evanescently couple to a lattice…