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Hexagonal HoMnO$_{3}$ is a frustrated antiferromagnet (T$_{N}$=72 K) ferroelectric (T$_{C}$=875 K) in which these two order parameters are coupled. Our neutron measurements of the spin wave dispersion for the S=2 Mn$^{3+}$ on the layered…

Strongly Correlated Electrons · Physics 2009-11-11 O. P. Vajk , M. Kenzelmann , J. W. Lynn , S. B. Kim , S. -W. Cheong

Structural and magnetic properties of a two-dimensional spin-$\frac{5}{2}$ frustrated triangular lattice antiferromagnet NH$_{4}$Fe(PO$_{3}$F)$_2$ are explored via x-ray diffraction, magnetic susceptibility, high-field magnetization, heat…

Materials Science · Physics 2025-02-11 S. Mohanty , K. M. Ranjith , C. S. Saramgi , Y. Skourski , B. Büchner , H. -J. Grafe , R. Nath

We set forth the structural and magnetic properties of the frustrated spin-$5/2$ triangle lattice antiferromagnet Na$_3$Fe(PO$_4$)$_2$ examined via x-ray diffraction, magnetization, heat capacity, and neutron diffraction measurements on the…

Materials Science · Physics 2022-01-26 Sebin J. Sebastian , A. Jain , S. M. Yusuf , M. Uhlarz , R. Nath

We report a 139La-NMR study of Ba2La2CoTe2O12, S = 1/2 equilateral triangular-lattice antiferromagnet with easy-plane anisotropy at low temperatures. This compound undergoes a magnetic phase transition at TN = 3.26 K into an ordered state…

We performed inelastic neutron scattering experiments on single crystal samples of a linear magnetoelectric material Mn$_{3}$Ta$_{2}$O$_{8}$, which exhibits a collinear antiferromagnetic order, to reveal the spin dynamics. Numerous modes…

Strongly Correlated Electrons · Physics 2025-04-08 Hodaka Kikuchi , SHunsuke Hasegawa , Shinichiro Asai , Tao Hong , Kenta Kimura , Tsuyoshi Kimura , Shinichi Itoh , Takatsugu Masuda

Using inelastic neutron scattering, we have observed a quasi-one-dimensional dispersive magnetic excitation in the frustrated triangular-lattice spin-2 chain oxide Ca3Co2O6. At the lowest temperature (T = 1.5 K), this magnon is…

Strongly Correlated Electrons · Physics 2013-12-17 Anil Jain , P. Y. Portnichenko , Hoyoung Jang , G. Jackeli , G. Friemel , A. Ivanov , A. Piovano , S. M. Yusuf , B. Keimer , D. S. Inosov

$^{75}$As NMR measurements were performed on a polycrystalline sample of spin-1/2 alternating-spin-chain Heisenberg antiferromagnet AgVOAsO$_4$. Temperature-dependent NMR shift $K(T)$, which is a direct measure of the intrinsic spin…

Materials Science · Physics 2017-12-27 N. Ahmed , P. Khuntia , H. Rosner , M. Baenitz , A. A. Tsirlin , R. Nath

Strong quantum fluctuations and unconventional spin dynamics are well established in the spin-1/2 triangular lattice Heisenberg antiferromagnet. However, their survival in the spin-1 case remains an open question. We investigate the spin…

Using elastic and inelastic neutron scattering techniques, we show that upon cooling a spatially anisotropic triangular antiferromagnet Ag$_2$MnO$_2$ freezes below $T_f ~\sim 50$ K into short range collinear state. The static spin…

Strongly Correlated Electrons · Physics 2009-07-21 S. Ji , J. -H. Kim , Y. Qiu , M. Matsuda , H. Yoshida , Z. Hiroi , M. A. Green , T. Ziman , S. -H. Lee

Elastic and inelastic neutron scattering studies reveal details of the antiferromagnetic tansition and intriguing spin-dynamics in the magneto-electric effect single crystal LiMnPO$_4$. The elastic scattering studies confirm the system is…

Strongly Correlated Electrons · Physics 2015-05-13 Jiying Li , Wei Tian , Ying Chen , Jerel L. Zarestky , Jeffrey W. Lynn , David Vaknin

We derive a spin-orbital Hamiltonian for a triangular lattice of e_g orbital degenerate (Ni^{3+}) transition metal ions interacting via 90 degree superexchange involving (O^{2-}) anions, taking into account the on-site Coulomb interactions…

Strongly Correlated Electrons · Physics 2009-11-11 Albert J. W. Reitsma , Louis F. Feiner , Andrzej M. Oles'

$^{31}$P nuclear magnetic resonance (NMR) measurements have been carried out to investigate the magnetic properties and spin dynamics of Fe$^{3+}$ ($S$ = 5/2) spins in the two-dimensional triangular lattice (TL) compound…

Strongly Correlated Electrons · Physics 2022-11-23 Devi V. Ambika , Qing-Ping Ding , Sebin J. Sebastian , Ramesh Nath , Yuji Furukawa

To understand spin interactions in materials of the Cu$_2$Sb structure type, inelastic neutron scattering of Fe$_2$As single crystals was examined at different temperatures and incident neutron energies. The experimental phonon spectra…

Ag2MnO2 is studied as a possible candidate compound for an antiferromagnetic XY spin model on a triangular lattice. In spite of the large Curie-Weiss temperature of -430 K found in magnetic susceptibi-lity, Mn3+ spins with S = 2 do not…

Strongly Correlated Electrons · Physics 2009-11-13 Hiroyuki Yoshida , Sascha Ahlert , Martin Jansen , Yoshihiko Okamoto , Jun-Ichi Yamaura , Zenji Hiroi

Spin fluctuations in the triangular-lattice Heisenberg antiferromagnet NaCrO$_2$ are investigated by means of quasi-elastic neutron scattering with high energy resolution and wide energy band. Two components with the following features are…

Strongly Correlated Electrons · Physics 2022-08-17 K. Tomiyasu , Y. P. Mizuta , M. Matsuura , K. Aoyama , H. Kawamura

Elastic and inelastic neutron scattering were used to study the ordered phase of the quasi-one-dimensional spin-1/2 antiferromagnet ${\rm BaCu_{2}Si_{2}O_{7}}$. The previously proposed model for the low-temperature magnetic structure was…

Strongly Correlated Electrons · Physics 2016-08-15 M. Kenzelmann , A. Zheludev , S. Raymond , E. Ressouche , T. Masuda , P. Böni , K. Kakurai , I. Tsukada , K. Uchinokura , R. Coldea

We carried out inelastic neutron scattering experiments on a buckled honeycomb lattice antiferromagnet Ba$_{2}$NiTeO$_{6}$ exhibiting a stripe structure at a low temperature. Magnetic excitations are observed in the energy range of $\hbar…

Strongly Correlated Electrons · Physics 2017-10-11 Shinichiro Asai , Minoru Soda , Kazuhiro Kasatani , Toshio Ono , V. Ovidiu Garlea , Barry Winn , Takatsugu Masuda

We use neutron scattering to study the lattice and magnetic structure of the layered half-doped manganite Pr$_{0.5}$Ca$_{1.5}$MnO$_4$. On cooling from high temperature, the system first becomes charge- and orbital- ordered (CO/OO) near…

Strongly Correlated Electrons · Physics 2009-11-13 Songxue Chi , F. Ye , Pengcheng Dai , J. A. Fernandez-Baca , Q. Huang , J. W. Lynn , E. W. Plummer , R. Mathieu , Y. Kaneko , Y. Tokura

We use neutron scattering to study the spin excitations associated with the stripe antiferromagnetic (AFM) order in semiconducting K$_{0.85}$Fe$_{1.54}$Se$_2$ ($T_N$=$280$ K). We show that the spin wave spectra can be accurately described…

Superconductivity · Physics 2015-06-19 Jun Zhao , Yao Shen , R. J. Birgeneau , Miao Gao , Zhong-Yi Lu , D. -H. Lee , X. Z. Lu , H. J. Xiang , D. L. Abernathy , Y. Zhao

The S = 1/2 triangular lattice antiferromagnet (TLAF) is a paradigmatic example of frustrated quantum magnetism. An ongoing challenge involves understanding the influence of exchange anisotropy on the collective behavior within such…