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One- and two-photon luminescence excitation spectroscopy showed a series of distinct excitonic states in single-walled carbon nanotubes. The energy splitting between one- and two-photon-active exciton states of different wavefunction…

Materials Science · Physics 2007-05-23 J. Maultzsch , R. Pomraenke , S. Reich , E. Chang , D. Prezzi , A. Ruini , E. Molinari , M. S. Strano , C. Thomsen , C. Lienau

The optical absorption spectrum of the carbon (4,2) nanotube is computed using an ab-initio many-body approach which takes into account excitonic effects. We develop a new method involving a local basis set which is symmetric with respect…

Materials Science · Physics 2009-11-10 Eric Chang , Giovanni Bussi , Alice Ruini , Elisa Molinari

Renormalization of quasiparticles and excitons in carbon nanotubes (CNTs) near a metallic surface has been studied within a many-body formalism using an embedding approach newly implemented in the GW and Bethe-Salpeter methods. The…

Mesoscale and Nanoscale Physics · Physics 2013-09-13 Catalin D. Spataru

Exciton effects are studied in single-wall boron-nitride nanotubes. The Coulomb interaction dependence of the band gap, the optical gap, and the binding energy of excitons are discussed. The optical gap of the (5,0) nanotube is about 6eV at…

Materials Science · Physics 2009-07-07 Kikuo Harigaya

Exciton effects are studied in single-wall boron-nitride (BN) nanotubes. Linear absorption spectra are calculated with changing the chiral index of the zigzag nanotubes. We consider the extended Hubbard model with atomic energies at the…

Materials Science · Physics 2009-07-07 Kikuo Harigaya

We present evidence that the strong electron-electron interactions in gapped carbon nanotubes lead to finite hierarchies of excitons within a given nanotube subband. We study these hierarchies by employing a field theoretic reduction of the…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Robert M. Konik

The ground-state exciton binding energy for single-walled carbon nanotubes (SWCNTs) in vacuum calculated ignoring the screening of Coulomb interaction appears to be much greater than the corresponding band gap. The most essential…

Other Condensed Matter · Physics 2010-11-18 Vadym M. Adamyan , Oleksii A. Smyrnov , Sergey V. Tishchenko

Recent fluorescence spectroscopy experiments on single wall carbon nanotubes reveal substantial deviations of observed absorption and emission energies from predictions of noninteracting models of the electronic structure. Nonetheless, the…

Materials Science · Physics 2009-11-10 C. L. Kane , E. J. Mele

We report first-principles calculations of the effects of quasiparticle self-energy and electron-hole interaction on the optical properties of single-walled BN nanotubes. Excitonic effects are shown to be even more important in BN nanotubes…

Materials Science · Physics 2007-08-23 Cheol-Hwan Park , Catalin D. Spataru , Steven G. Louie

We develop a scaling relationship between the exciton binding energy and the external dielectric function in carbon nanotubes. We show that the electron-electron and electron-hole interaction energies are strongly affected by screening yet…

Intrinsic optical transition energies for isolated and individual single wall carbon nanotubes grown over trenches are measured using tunable resonant Raman scattering. Previously measured E22_S optical transitions from nanotubes in…

Single-walled carbon nanotubes are strongly correlated systems with large Coulomb repulsion between two electrons occupying the same $p_z$ orbital. Within a molecular Hamiltonian appropriate for correlated $\pi$-electron systems, we show…

Materials Science · Physics 2009-02-15 Zhendong Wang , Demetra Psiachos , Roberto F. Badilla , Sumit Mazumdar

We calculate the exciton binding energy in single-walled carbon nanotubes with narrow band gaps, accounting for the quasi-relativistic dispersion of electrons and holes. Exact analytical solutions of the quantum relativistic two-body…

Mesoscale and Nanoscale Physics · Physics 2011-08-16 R. R. Hartmann , I. A. Shelykh , M. E. Portnoi

Carbon nanotubes are the focus of considerable research efforts due to their fascinating physical properties. They provide an excellent model system for the study of one dimensional materials and molecular electronics. The chirality of…

Light emission from carbon nanotubes is expected to be dominated by excitonic recombination. Here we calculate the properties of excitons in nanotubes embedded in a dielectric, for a wide range of tube radii and dielectric environments. We…

Materials Science · Physics 2009-11-10 Vasili Perebeinos , J. Tersoff , Phaedon Avouris

Electroabsorption spectroscopy of well-identified index-defined semiconducting carbon nanotubes is reported. The measurement of high definition electroabsorption spectra allows direct indexation with unique nanotube chirality. Results show…

We present many-body \textit{ab initio} calculations of the electronic and optical properties of semiconducting zigzag carbon nanotubes under uniaxial strain. The GW approach is utilized to obtain the quasiparticle bandgaps and is combined…

Materials Science · Physics 2015-06-16 Catalin D. Spataru , François Léonard

The recently reported experimental optical spectra of double-walled carbon nanotubes exhibit more peaks than it could be expected based on the layers alone. The appearance of excess peaks has been attributed to the interlayer interaction.…

Mesoscale and Nanoscale Physics · Physics 2020-08-12 Valentin N. Popov

Many-electron effects often dramatically modify the properties of reduced dimensional systems. We report calculations, based on an many-electron Green's function approach, of electron-hole interaction effects on the optical spectra of…

Materials Science · Physics 2009-11-10 Catalin D. Spataru , Sohrab Ismail-Beigi , Lorin X. Benedict , Steven G. Louie

The bright exciton emission of semiconducting carbon nanotubes is appealing for optoelectronic and quantum photonic devices as well as fundamental studies of light-matter interaction in one-dimensional nanostructures. The photophysics of…

Mesoscale and Nanoscale Physics · Physics 2017-05-09 Ibrahim Sarpkaya , Zhengyi Zhang , William Walden-Newman , Xuesi Wang , James Hone , Chee Wei Wong , Stefan Strauf
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