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The nonlinear response of materials, an increasingly important aspect of light-matter interaction, can be challenging to measure in highly absorbing materials. Here, we introduce an interferometric technique that enables a direct…

Optics · Physics 2024-11-25 C. D. Cruz , J. C. Stephenson , J. K. Wahlstrand

We characterize spectroscopic and coherence properties of the 1451.37 nm excited-state zero-phonon line (ZPL) between the $^{3}F_{4}$ and the $^{3}H_{4}$ manifolds of a thulium-doped yttrium aluminum perovskite (Tm$^{3+}$:YAlO$_3$) crystal…

We use a magnetometer probe based on the Zeeman shift of the rubidium resonant optical transition to explore the atomic magnetic response for a wide range of field values. We record optical spectra for fields from few tesla up to 60 tesla,…

Atomic Physics · Physics 2017-11-22 D. Ciampini , R. Battesti , C. Rizzo , E. Arimondo

Sub-wavelength graphene structures support localized plasmonic resonances in the terahertz and mid-infrared spectral regimes. The strong field confinement at the resonant frequency is predicted to significantly enhance the light-graphene…

We have searched for absorption in several common atomic species due to the atmosphere or exosphere of the transiting extrasolar planet HD 209458b, using high precision optical spectra obtained with the Subaru High Dispersion Spectrograph…

We present transient absorption spectra of an extreme ultraviolet attosecond pulse train in helium dressed by an 800 nm laser field with intensity ranging from $2\times10^{12}$ W/cm$^2$ to $2\times10^{14}$ W/cm$^2$. The energy range probed…

We calculated third order non-linear polarization to estimate the two-photon absorption of non-interacting two-level molecules in the transmission-type degenerate pump-probe geometry. The spectral intensity and the phase changes of the…

Optics · Physics 2019-05-01 Tsogvoo Khos-Ochir , Kim Myung-Whun , Purevdorj Munkhbaatar

High-resolution spectroscopy allows one to probe weak interactions and to detect subtle phenomena. While such measurements are routinely performed on atoms and molecules in the gas phase, spectroscopy of adsorbed species on surfaces is…

We describe the so-called "Lambda-Zeeman method" to investigate individual hyperfine transitions between Zeeman sublevels of atoms in an external magnetic field of 0.1 mT - 0.25 T. Atoms are confined in a nanocell with thickness L = Lambda,…

We compute the interaction of a sodium vapor with a static magnetic field ranging from 0 up to 1 Tesla, which allows to obtain the behavior of all Zeeman transitions as a function of the magnetic field for any polarization of incident laser…

Atomic Physics · Physics 2021-07-14 Rodolphe Momier , Aram V. Papoyan , Claude Leroy

A theoretical model of the influence of detection bandwidth properties on observed line shapes in laser absorption spectroscopy is described. The model predicts artificial frequency shifts, extra broadenings and line asymmetries which must…

Selective Reflection (SR) spectroscopy of the $6s$ $^2S_{1/2} \rightarrow$ $7p$ $^2P_{3/2}$ electric dipole transition of Cesium ($\lambda~=~456$ nm) is performed for the first time using a nanometric-thin cell ($L=50 - 1500$~nm). We…

Atomic Physics · Physics 2025-01-22 Armen Sargsyan , Rodolphe Momier , David Sarkisyan

An efficient $\lambda/2$-method ($\lambda$ is the resonant wavelength of laser radiation) based on nanometric-thickness cell filled with rubidium is implemented to study the splitting of hyperfine transitions of $^{85}$Rb and $^{87}$Rb…

Atomic Physics · Physics 2015-06-19 A. Sargsyan , A. Tonoyan , G. Hakhumyan , C. Leroy , Y. Pashayan-Leroy , D. Sarkisyan

We study the evolution of a V-type three-level system, whose two resonances are coherently excited and coupled by two ultrashort laser pump and probe pulses, separated by a varying time delay. We relate the quantum dynamics of the excited…

Atomic Physics · Physics 2015-04-02 Z. Liu , S. M. Cavaletto , C. Ott , K. Meyer , Y. Mi , Z. Harman , C. H. Keitel , T. Pfeifer

We study a nonlinear interferometer consisting of two consecutive parametric amplifiers, where all three optical fields (pump, signal and idler) are treated quantum mechanically, allowing for pump depletion and other quantum phenomena. The…

Quantum Physics · Physics 2018-12-27 Jefferson Flórez , Enno Giese , Davor Curic , Lambert Giner , Robert W. Boyd , Jeff S. Lundeen

We present an analysis of the absorption-line system in the Very Large Telescope/Ultraviolet and Visual Echelle Spectrograph spectrum at a redshift of $z_{\rm a}={3.1448}$ associated with the quasar SDSS J122040.23+092326.96, whose…

Astrophysics of Galaxies · Physics 2025-01-03 Qiguo Tian , Lei Hao , Yipeng Zhou , Xiheng Shi , Tuo Ji , Peng Jiang , Lin Lin , Zhenya Zheng , Hongyan Zhou

The relative population of the fine structure sublevels of an atom's ground state is affected by radiative transitions induced by an anisotropic radiation flux. This causes the alignment of atomic angular momentum. In terms of observational…

Astrophysics · Physics 2008-11-26 Huirong Yan , A. Lazarian

We present a new theoretical approach for collisional absorption of laser energy in dense plasmas which accommodates arbitrary frequencies and high intensities of the laser field. We establish a connection between laser absorption by…

Plasma Physics · Physics 2015-05-13 A. Grinenko , D. O. Gericke

Absorption profile of a four-level ladder atomic system interacting with three driving fields is studied perturbatively and analytical results are presented. Numerical results where the driving field strengths are treated upto all orders…

Quantum Physics · Physics 2015-06-26 S N Sandhya

We studied the ultrafast third-order optical nonlinearity in a single crystal of multiferroic bismuth ferrite (BiFeO3) in the near-infrared range of 0.5-1.0 eV, where the material is fundamentally transparent,at room temperature. With pump…

Strongly Correlated Electrons · Physics 2015-09-02 Eiichi Matsubara , Takeshi Mochizuki , Masaya Nagai , Toshimitsu Ito , Masaaki Ashida