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We generalize the simplest kinetically constrained model of a glass-forming liquid by softening kinetic constraints, allowing them to be violated with a small finite rate. We demonstrate that this model supports a first-order dynamical…

Statistical Mechanics · Physics 2010-10-14 Yael S. Elmatad , Robert L. Jack , Juan P. Garrahan , David Chandler

Using simulations we identify three dynamic regimes in supersaturated isotropic fluid states of short hard rods: (i) for moderate supersaturations we observe nucleation of multi-layered crystalline clusters; (ii) at higher supersaturation,…

Soft Condensed Matter · Physics 2012-08-17 Ran Ni , Simone Belli , Rene van Roij , Marjolein Dijkstra

Liquid crystal droplets are of great interest from physics and applications. Rigorous mathematical analysis is challenging as the problem involves harmonic maps (and in general the Oseen-Frank model), free interfaces and topological defects…

Analysis of PDEs · Mathematics 2020-09-25 Fanghua Lin , Changyou Wang

We perform dynamical simulations of a two-dimensional active nematic fluid in coexistence with an isotropic fluid. Drops of active nematic become elongated, and an effective anchoring develops at the nematic-isotropic interface. The…

Soft Condensed Matter · Physics 2014-12-17 Matthew L. Blow , Sumesh P. Thampi , Julia M. Yeomans

We demonstrate how to construct dynamic phase diagrams for complex fluids that undergo transitions under flow, in which the conserved composition variable and the broken-symmetry order parameter (nematic, smectic, crystalline, etc.) are…

Soft Condensed Matter · Physics 2009-10-30 Peter D. Olmsted , C. -Y. D. Lu

We have studied, using molecular dynamics simulations, the pressure-induced melting in a monolayer of soft repulsive spherocylinders whose centers of mass are constrained to move on the surface of a sphere. We show that the orientational…

Soft Condensed Matter · Physics 2025-03-13 Jaydeep Mandal , Chandan Dasgupta , Prabal K. Maiti

The recent paper cited above claims that a molecular simulation of one specific model of supercooled water establishes a stable interface separating two metastable liquid phases, which would imply the existence of metastable two-liquid…

Statistical Mechanics · Physics 2014-08-21 David Chandler

We study a chemically active binary mixture undergoing phase separation and show that under non-equilibrium conditions, stable liquid spherical shells can form via a spinodal instability in the droplet center. A single liquid shell tends to…

Soft Condensed Matter · Physics 2023-06-21 Jonathan Bauermann , Giacomo Bartolucci , Job Boekhoven , Christoph A. Weber , Frank Jülicher

We introduce a model of water contemplating true supercooled-liquid states that, as such, are metastable with respect to the crystalline-solid ones. Its numerical solutions reproduce from Speedy-Angell's stability-limit picture to Poole et…

Statistical Mechanics · Physics 2026-05-26 Jacobo Troncoso , Claudio A. Cerdeiriña

We study the kinetics of the liquid-to-crystal transformation and of gel formation in colloidal suspensions of oppositely charged particles. We analyse, by means of both computer simulations and experiments, the evolution of a fluid…

Spontaneous onset of a low temperature topologically ordered phase in a 2-dimensional (2D) lattice model of uniaxial liquid crystal (LC) was debated extensively pointing to a suspected underlying mechanism affecting the RG flow near the…

Soft Condensed Matter · Physics 2021-06-29 B. Kamala Latha , Surajit Dhara , V. S. S. Sastry

We present a high-resolution computer simulation study of the equation of state of ST2 water, evaluating the liquid-state properties at 2718 state points, and precisely locating the liquid-liquid critical point (LLCP) occurring in this…

Statistical Mechanics · Physics 2010-10-08 Peter H. Poole , Ivan Saika-Voivod , Francesco Sciortino

A popular hypothesis that explains the anomalies of supercooled water is the existence of a metastable liquid-liquid transition hidden below the line of homogeneous nucleation. If this transition exists and if it is terminated by a critical…

Soft Condensed Matter · Physics 2014-08-25 John W. Biddle , Vincent Holten , Mikhail A. Anisimov

As typical complex liquids, ionic liquids (ILs) exhibit phases beyond the description of simple liquid theories. In particular, with an intermediate cationic side-chain length, ILs can form the nanoscale segregated liquid (NSL) phase, which…

Soft Condensed Matter · Physics 2020-04-07 Shen Li , Yanting Wang

We formulate the scaled particle theory for a general mixture of hard isosceles triangles and calculate different phase diagrams for the one-component fluid and for certain binary mixtures. The fluid of hard triangles exhibits a complex…

Soft Condensed Matter · Physics 2018-05-16 Yuri Martinez-Raton , Ariel Diaz-De Armas , Enrique Velasco

Simulations of nematic-isotropic transition of liquid crystals in two dimensions are performed using an O(2) vector model characterised by non linear nearest neighbour spin interaction governed by the fourth Legendre polynomial $P\_4$. The…

Statistical Mechanics · Physics 2007-05-23 Bertrand Berche , Ricardo Paredes

We study the zero-temperature phase diagram of two-dimensional helium-4 using neural quantum states. Our variational description allows us to address liquid and solid phases using the same functional form as well as exploring possible…

Statistical Mechanics · Physics 2025-06-19 David Linteau , Gabriel Pescia , Jannes Nys , Giuseppe Carleo , Markus Holzmann

Using event driven molecular dynamics simulations, we study a three dimensional one-component system of spherical particles interacting via a discontinuous potential combining a repulsive square soft core and an attractive square well. In…

Soft Condensed Matter · Physics 2009-11-10 A. Skibinsky , S. V. Buldyrev , G. Franzese , G. Malescio , H. E. Stanley

We numerically study a nondisordered lattice spin system with a first order liquid-crystal transition, as a model for supercooled liquids and glasses. Below the melting temperature the system can be kept in the metastable liquid phase, and…

Statistical Mechanics · Physics 2009-11-07 Andrea Cavagna , Irene Giardina , Tomas S. Grigera

"Conventional" scenario of metastable melting in ordinary substances in the limit of zero temperature assumes that the melting curve reaches the matter zero isotherm ("cold curve"). The same is true for standard variant of one-component…

Plasma Physics · Physics 2007-05-23 Igor L. Iosilevski , Alexander Yu. Chigvintsev