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We report a computer-simulation study of the equilibrium phase diagram of a three-dimensional system of particles with a repulsive step potential. The phase diagram is obtained using free-energy calculations. At low temperatures, we observe…

Soft Condensed Matter · Physics 2015-05-13 N. V. Gribova , Yu. D. Fomin , Daan Frenkel , V. N. Ryzhov

In this paper we present a simulation study of density, structural and diffusion anomalies in core-softened system introduced in our previous publications. It is well-known, that with appropriate parametrization, core-softened systems are…

Soft Condensed Matter · Physics 2015-06-12 Yu. D. Fomin , E. N. Tsiok , V. N. Ryzhov

In the present paper, using a molecular dynamics simulation, we study a nature of melting of a two-dimensional ($2D$) system of classical particles interacting through a purely repulsive isotropic core-softened potential which is used for…

Soft Condensed Matter · Physics 2015-06-22 D. E. Dudalov , Yu. D. Fomin , E. N. Tsiok , V. N. Ryzhov

A series of phase diagrams is obtained for a smooth pair-potential with an outer well and a repulsive inner shoulder. Condensed phase coexistence curves are located using free-energy calculations. Liquid-vapour equilibria are obtained with…

Statistical Mechanics · Physics 2009-11-11 D. Quigley , M. I. J. Probert

We performed extensive molecular dynamics (MD) simulations, supplemented by Mode Coupling Theory (MCT) calculations, for the Square Shoulder (SS) model, a purely repulsive potential where the hard-core is complemented by a finite shoulder.…

Soft Condensed Matter · Physics 2015-06-15 Gayatri Das , Nicoletta Gnan , Francesco Sciortino , Emanuela Zaccarelli

Using molecular dynamics simulations and integral equations (Rogers-Young, Percus-Yevick and hypernetted chain closures) we investigate the thermodynamic of particles interacting with continuous core-softened intermolecular potential.…

Soft Condensed Matter · Physics 2007-05-23 Alan B. de Oliveira , Paulo A. Netz , Thiago Colla , Marcia C. Barbosa

The behavior of colloidal particles with a hard core and a soft shell has attracted the attention for researchers in the physical-chemistry interface not only due the large number of applications, but due the unique properties of these…

Soft Condensed Matter · Physics 2021-02-23 Murilo S. Marques , José Rafael Bordin

We present molecular simulation data for viscosity, self-diffusivity, and the local structural ordering of (i) a hard-sphere fluid and (ii) a square-well fluid with short-range attractions. The latter fluid exhibits a region of dynamic…

Soft Condensed Matter · Physics 2007-09-06 William P. Krekelberg , Jeetain Mittal , Venkat Ganesan , Thomas M. Truskett

Using molecular dynamics we studied the role of the anisotropy on the phase boundary and on the anomalous behavior of 250 dimeric particles interacting by a core-softened potential. This study led us to an unexpected result: the…

We report Monte Carlo results for the fluid structure of a system of dimeric particles interacting via a core-softened potential. More specifically, dimers interact through a repulsive pair potential of inverse-power form, modified in such…

Soft Condensed Matter · Physics 2016-03-08 Gianmarco Munaò , Franz Saija

Soft-core attractive potentials can give rise to a phase diagram with three fluid phases at different densities (gas, low-density liquid and high-density liquid), separated by first order phase transition lines ending in critical points.…

Statistical Mechanics · Physics 2009-10-22 Giancarlo Franzese

The structural properties of fluids whose molecules interact via potentials with a hard core plus two piece-wise constant sections of different widths and heights are presented. These follow from the more general development previously…

Soft Condensed Matter · Physics 2013-08-27 Andrés Santos , Santos B. Yuste , Mariano López de Haro , Mariana Bárcenas , Pedro Orea

Isotropic soft-core potentials with two characteristic length scales have been used since 40 years to describe systems with polymorphism. In the recent years intense research is showing that these potentials also display polyamorphism and…

Soft Condensed Matter · Physics 2015-05-18 Pol Vilaseca , Giancarlo Franzese

2D competitive systems shows a large variety of solid and aggregate patterns, re-entrant fluid phase, a continuous melting as predicted by the KTHNY theory and, in some cases, waterlike anomalies. In this paper, we employ Langevin Dynamics…

We investigate the structural, thermodynamic and dynamic behavior of of a two dimensional core-corona system using Langevin Dynamics simulations. The particles are modeled using a core-softened potential that exhibits waterlike anomalies…

Soft Condensed Matter · Physics 2018-02-14 José Rafael Bordin , Marcia C. Barbosa

Using Monte Carlo simulation techniques, we calculate the phase diagram for a square shoulder-square well potential in two dimensions that has been previously shown to exhibit liquid anomalies consistent with a metastable liquid-liquid…

Soft Condensed Matter · Physics 2015-06-04 Ahmad M. Almudallal , Sergey V. Buldyrev , Ivan Saika-Voivod

Molecular Dynamic and Monte Carlo studies are performed in a family of core-softened (CS) potential, composed by two length scales: a repulsive shoulder at short distances and the another a variable scale, that can be repulsive or strongly…

Soft Condensed Matter · Physics 2017-01-04 L. Pinheiro , A. P. Furlan , L. B. Krott , A. Diehl , M. C. Barbosa

We investigate the slow dynamics of a colloidal model with two repulsive length scales, whose interaction potential is the sum of a hard-core and a square shoulder. Despite the simplicity of the interactions, Mode-Coupling theory predicts a…

Soft Condensed Matter · Physics 2014-07-16 Nicoletta Gnan , Gayatri Das , Matthias Sperl , Francesco Sciortino , Emanuela Zaccarelli

In the framework of the density functional theory of freezing proposed in our previous works, we calculate the phase diagram of two-dimensional system of particles interacting through the repulsive shoulder potential. This potential…

Statistical Mechanics · Physics 2015-06-23 E. S. Chumakov , Yu. D. Fomin , E. L. Shangina , E. E. Tareyeva , E. N. Tsiok , V. N. Ryzhov

We demonstrate that tunable attractive (bonding) and repulsive (anti-bonding) forces can arise in highly asymmetric structures coupled to external radiation, a consequence of the bonding/anti-bonding level repulsion of guided-wave…