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Considering the photoionization of Ar@C60, we predict resonant femtosecond decays of both Ar and C60 vacancies through the continua of atom-fullerene hybrid final states. The resulting resonances emerge from the interference between…

Atomic and Molecular Clusters · Physics 2021-06-08 Mohammad H. Javani , Jacob B. Wise , Ruma De , Mohamed E. Madjet , Steven T. Manson , Himadri S. Chakraborty

We show, with an example of Na_92, that for jellium metal clusters the interference of fast electron-waves emitted from equivalent sites on the cluster edge produces monochromatic oscillations in all photoionization observables as a…

Atomic Physics · Physics 2007-05-23 Himadri S. Chakraborty , M. E. Madjet

This is an investigation on the dynamical screening of an atom confined within a fullerene of finite width. The two surfaces of the fullerene lead to the presence of two surface plasmon eigenmodes. It is shown that, in the vicinity of these…

Atomic and Molecular Clusters · Physics 2008-11-10 S. Lo , A. V. Korol , A. V. Solov'yov

The changes of dynamical behaviour of a single fullerene molecule inside an armchair carbon nanotube caused by the structural Peierls transition in the nanotube are considered. The structures of the smallest C20 and Fe@C20 fullerenes are…

We review the main aspects of multiple photoionization processes in atoms exposed to intense, short wavelength radiation. The main focus is the theoretical framework for the description of such processes as well as the conditions under…

Atomic Physics · Physics 2014-01-21 P. Lambropoulos , G. M. Nikolopoulos

We study the rotation rates and electric dipole emission of hydrogenated icosahedral fullerenes (single and multishell) in various phases of the interstellar medium. Using the formalism of Draine and Lazarian for the rotational dynamics of…

Astrophysics · Physics 2007-05-23 Susana Iglesias-Groth

Modifications of photoionization arising from resonant electron-electron correlations between neighbouring atoms in an atomic sample are studied. The sample contains atomic species A and B, with the ionization potential of A being smaller…

Atomic Physics · Physics 2015-06-04 B. Najjari , C. Müller , A. B. Voitkiv

The polarization-response spectrum of the fullerene C60 modeled as a homogeneous spherical plasma shell is calculated in the framework of the hydrodynamic approach allowing for the spatial dispersion caused by the Fermi-distributed valence…

Plasma Physics · Physics 2017-10-17 V. B. Gildenburg , I. A. Pavlichenko

In open-shell atoms and ions, processes such as photoionization, combination (Raman) scattering, electron scattering and recombination, are often mediated by many-electron compound resonances. We show that their interference (neglected in…

Atomic Physics · Physics 2015-05-14 V. V. Flambaum , M. G. Kozlov , G. F. Gribakin

We demonstrate that the structure of confinement resonances in the photoionization cross section of an endohedral atom is very sensitive to the mean displacement <a> of the atom from the cage center. The resonances are strongly suppressed…

Atomic and Molecular Clusters · Physics 2015-05-14 A. V. Korol , A. V. Solov'yov

Photoionization of the Ce$^{3+}$ - Ce$^{4+}$ process has been studied using the random phase approximation with exchange method in the energy region 100-150 eV. Comparison of our results with the recent measurement [M\"uller {\it et al},…

Atomic Physics · Physics 2015-05-13 Zhifan Chen , Alfred Z. Msezane

Effects of the interchannel coupling on the spin polarization of energetic photoelectrons emitted from atomic Ne valence subshells are examined. Like previously obtained results for cross sections and angular distributions, the…

Atomic Physics · Physics 2021-06-08 Himadri S. Chakraborty , Pranawa C. Deshmukh , Steven T. Manson

We apply time-dependent R-matrix theory to study inner-shell ionization of C atoms in ultra-short high-frequency light fields with a photon energy between 170 and 245 eV. At an intensity of 10$^{17}$ W/cm$^2$, ionization is dominated by…

Atomic Physics · Physics 2015-08-12 H. F. Rey , H. W. van der Hart

The electron-phonon and Coulomb interactions inC$_{60}$, and larger fullerene spheres are analyzed. The coupling between electrons and intramolecular vibrations give corrections $\sim 1 - 10$ meV to the electronic energies for C$_{60}$, and…

Condensed Matter · Physics 2009-10-22 F. Guinea , J. Gonzalez , M. A. H. Vozmediano

Photoionization cross section of the fullerene ion C60+ has been calculated within a single-electron approximation and also by using a consistent many-body theory accounting for many-electron correlations.

Atomic and Molecular Clusters · Physics 2016-09-20 R. G. Polozkov , V. K. Ivanov , A. V. Solov'yov

We investigate the formation of fullerene-like structures from hot Carbon gas using classical molecular dynamics, employing Brenner's potential. In particular we examine the influence of different annealing strategies on fullerene yield,…

Materials Science · Physics 2009-12-22 Klaus Lichtenegger , Wolfgang von der Linden

Considering C$_{60}$ as a model system for describing field emission from the extremity of a carbon nanotip, we explore electron emission from this fullerene excited by an intense, near-infrared, few-cycle laser pulse…

Atomic and Molecular Clusters · Physics 2016-03-23 Cong-Zhang Gao , Phuong Mai Dinh , Peter Kluepfel , Chris Meier , Paul-Gerhard Reinhard , Eric Suraud

We show that both confined atoms and electron-atom scattering can be described by a unified basis set method. The central idea behind this method is to place the atom inside a hard potential sphere, enforced by a standard Slater type basis…

Other Condensed Matter · Physics 2015-05-13 Meta van Faassen

Highly excited eigenstates of atoms and ions with open f shell are chaotic superpositions of thousands, or even millions of Hartree-Fock determinant states. The interaction between dielectronic and multielectronic configurations leads to…

Atomic Physics · Physics 2015-06-17 V. A. Dzuba , V. V. Flambaum , G. F. Gribakin , C. Harabati , M. G. Kozlov

Inter-Coulombic decay (ICD) resonances in the photoionization of Cl@C60 endofullerene molecule are calculated using a perturbative density functional theory (DFT) method. This is the first ICD study of an open shell atom in a fullerene…

Atomic and Molecular Clusters · Physics 2021-08-11 Ruma De , Esam Ali , Steven T. Manson , Himadri S. Chakraborty
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