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The laser-induced fragmentation dynamics of this most fundamental polar molecule HeH$^+$ are measured using an ion beam of helium hydride and an isotopologue at various wavelengths and intensities. In contrast to the prevailing…

Chemical Physics · Physics 2018-08-21 P. Wustelt , F. Oppermann , Lun Yue , M. Möller , T. Stöhlker , S. Gräfe , M. Lein , G. G. Paulus , A. M. Sayler

We study the breakup of $\text{H}_2^+$ exposed to super-intense, femtosecond laser pulses with frequencies greater than that corresponding to the ionization potential. By solving the time-dependent Schr\"odinger equation in an extensive…

Atomic Physics · Physics 2016-04-12 Lun Yue , Lars Bojer Madsen

We address nonsequential double ionization induced by strong, linearly polarized laser fields of only a few cycles, considering a physical mechanism in which the second electron is dislodged by the inelastic collision of the first electron…

Atomic Physics · Physics 2009-11-10 C. Figueira de Morisson Faria , X. Liu , A. Sanpera , M. Lewenstein

Exact solutions describing the nonlinear electrodynamics of a thin double layer foil are presented. These solutions correspond to a broad range of problems of interest for the interaction of high intensity laser pulses with overdense…

The alignment- and internuclear-distance dependent ionization of H$_2$ exposed to intense, ultrashort laser fields is studied by solving the time-dependent two-electron Schr\"odinger equation. In the regime of perturbative few-photon…

Atomic Physics · Physics 2015-06-23 Johann Förster , Yulian V. Vanne , Alejandro Saenz

Double electron ionisation process occurs when an intense laser pulse interacts with atoms or molecules. Exact {\it ab initio} numerical simulation of such a situation is extremely computer resources demanding, thus often one is forced to…

Here, we identify a new mechanism where the early stage of electron ionization in the field of strong femtosecond laser pulse determines the final yield of non-sequential double ionization. By using simple trajectory methods we prove that…

Quantum Physics · Physics 2025-02-07 Ivan P. Christov

We investigate molecular dynamics of multiple ionization in N2 through multiple core-level photoabsorption and subsequent Auger decay processes induced by intense, short X-ray free electron laser pulses. The timing dynamics of the…

Recent advances in strong x-ray laser techniques enable the study of nonlinear multiphoton ionization in extreme high-frequency fields. Although the stabilization regime in such fields is theoretically established, its modified properties…

Atomic Physics · Physics 2026-02-17 Aleksandr V. Boitsov , Karen Z. Hatsagortsyan , Christoph H. Keitel

The frequency dependence of (nonsequential) double ionization is studied in fully quantum mechanical calculations using a (1+1)-dimensional model atom. Other time-dependent effects such as the influence of the number of field cycles are…

Quantum Physics · Physics 2025-11-10 Jan H. Thiede , Jakub S. Prauzner-Bechcicki

We report on the unambiguous observation of the sub-cycle ionization bursts in sequential strong-field double ionization of H$_2$ and their disentanglement in molecular frame photoelectron angular distributions. This observation was made…

The degree of elliptical polarization of intense short laser pulses is shown to be related to the timing of strong-field non-sequential double ionization. Higher ellipticity is predicted to force the initiation of double ionization into a…

Atomic Physics · Physics 2010-08-20 Xu Wang , J. H. Eberly

Using a three-dimensional quasiclassical technique we explore molecular double ionization by a linearly polarized, infrared (800~nm) 27~fs laser pulse. For intensities ranging from the tunneling to the over-the-barrier regime, we identify…

Atomic Physics · Physics 2011-01-27 A. Emmanouilidou , D. S. Tchitchekova

Nonsequential double ionization (NSDI) of helium in an intense few-cycle laser pulse is investigated by applying the three-dimensional semi-classical re-scattering method. It is found that the momentum distribution of He$^{2+}$ shows a…

Atomic Physics · Physics 2015-05-13 Hongyun Li , J. Chen , Hongbing Jiang , Jie Liu , Panming Fu , Qihuang Gong , Zong-Chao Yan , Bingbing Wang

We present a numerical method for investigating the non-perturbative quantum mechanical interaction of light with atoms in two dimensions, without a basis expansion. This enables us to investigate intense laser-atom interactions with light…

Quantum Physics · Physics 2009-10-30 M. Protopapas , D. G. Lappas , P. L. Knight

We present the results of the detailed experimental study of multiple ionization of Ne and Ar by 25 and 7 fs laser pulses. For Ne the highly correlated "instantaneous" emission of up to four electrons is triggered by a recollisional…

Atomic Physics · Physics 2009-11-10 A. Rudenko , K. Zrost , B. Feuerstein , V. L. B. de Jesus , C. D. Schröter , R. Moshammer , J. Ullrich

We consider the final stage of double ionization of $\rm O_2$ molecules by short linearly polarized laser pulses. The saddles of the effective adiabatic potential energy close to which simultaneous escape of electrons from a molecule takes…

Atomic Physics · Physics 2007-05-23 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt

We present three dimensional time-dependent calculations of ionization of arbitrarily spatially oriented H$_2^+$ by attosecond, intense, high-frequency laser fields. The ionization probability shows a strong dependence on both the…

Atomic Physics · Physics 2007-05-23 S. Selsto , M. Forre , J. P. Hansen , L. B. Madsen

A theoretical comparison of the electronic excitation and ionisation behaviour of molecular hydrogen oriented either parallel or perpendicular to a linear polarised laser pulse is performed. The investigation is based on a non-perturbative…

Quantum Physics · Physics 2009-11-13 Yulian V. Vanne , Alejandro Saenz

When a diatomic molecule is ionized by an intense laser field, the ionization rate depends very strongly on the inter-nuclear separation. That dependence exhibits a pronounced maximum at the inter-nuclear separation known as the critical…

Chemical Physics · Physics 2015-04-21 Han Xu , Feng He , D. Kielpinski , R. T. Sang , I. V. Litvinyuk