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This study focuses on the formation of two molecules of astrobiological importance - glycolaldehyde (HC(O)CH2OH) and ethylene glycol (H2C(OH)CH2OH) - by surface hydrogenation of CO molecules. Our experiments aim at simulating the CO…

Astrophysics of Galaxies · Physics 2017-05-26 Gleb Fedoseev , Herma M. Cuppen , Sergio Ioppolo , Thanja Lamberts , Harold Linnartz

The simultaneous detection of organic molecules of the form C$_2$H$_{\text{n}}$O, such as ketene (CH$_2$CO), acetaldehyde (CH$_3$CHO), and ethanol (CH$_3$CH$_2$OH), toward early star-forming regions offers hints of shared chemical history.…

Astrophysics of Galaxies · Physics 2021-06-16 K. -J. Chuang , G. Fedoseev , C. Scirè , G. A. Baratta , C. Jäger , Th. Henning , H. Linnartz , M. E. Palumbo

The first experimental study of the low-temperature kinetics of the gas-phase reaction of NH2 with formaldehyde (CH2O) has been performed. This reaction has previously been suggested as a source of formamide (NH2CHO) in interstellar…

Astrophysics of Galaxies · Physics 2022-10-05 Kevin M. Douglas , Daniel Lucas , Catherine Walsh , Niclas A. West , Mark A. Blitz , Dwayne E. Heard

Ice chemistry in the dense, cold interstellar medium (ISM) is probably responsible for the formation of interstellar complex organic molecules (COMs). Recent laboratory experiments performed at T=4 K have shown that irradiation of CO:N2 ice…

Astrophysics of Galaxies · Physics 2024-01-09 Rafael Martín-Doménech , Alexander DelFranco , Karin I. Öberg , Mahesh Rajappan

Radical recombination has been proposed to lead to the formation of complex organic molecules (COMs) in CO-rich ices in the early stages of star formation. These COMs can then undergo hydrogen addition and abstraction reactions leading to a…

Astrophysics of Galaxies · Physics 2018-06-07 S. Álvarez-Barcia , P. Russ , J. Kästner , T. Lamberts

Context. The molecular composition of interstellar ice mantles is defined by gas-grain processes in molecular clouds, with the main components being $H_2O$, $CO$, and $CO_2$. $CH_3OH$ ice is detected towards the denser regions, where large…

Astrophysics of Galaxies · Physics 2021-08-25 B. Müller , B. M. Giuliano , M. Goto , P. Caselli

The deuterium fractionation of gas-phase molecules in hot cores is believed to reflect the composition of interstellar ices. The deuteration of methanol is a major puzzle, however, because the isotopologue ratio [CH2DOH]/[CH3OD], which is…

Solar and Stellar Astrophysics · Physics 2015-12-02 A. Faure , M. Faure , P. Theulé , E. Quirico , B. Schmitt

CO2 ice is one of the most abundant components in ice-coated interstellar ices besides H2O and CO, but the most favorable path to CO2 ice is still unclear. Molecular dynamics calculations on the ultraviolet photodissociation of different…

Chemical Physics · Physics 2015-06-17 Carina Arasa , Marc C. van Hemert , Ewine F. van Dishoeck , Geert-Jan Kroes

Complex organic molecules (COMs) have been observed not only in the hot cores surrounding low- and high- mass protostars, but also in cold dark clouds. Therefore, it is interesting to understand how such species can be formed without the…

Astrophysics of Galaxies · Physics 2016-06-06 K. -J. Chuang , G. Fedoseev , S. Ioppolo , E. F. van Dishoeck , H. Linnartz

The formation of double and triple C-C bonds from the processing of pure c-C6H12 (cyclohexane) and mixed H2O:NH3:c-C6H12 (1:0.3:0.7) ices by highly-charged, and energetic ions (219 MeV O^{7+} and 632 MeV Ni^{24+}) is studied. The…

Astrophysics of Galaxies · Physics 2015-06-04 S. Pilling , D. P. P. Andrade , E. F. da Silveira , H. Rothard , A. Domaracka , P. Boduch

The results of experiments on the formation of molecular hydrogen on low density and high density amorphous ice surfaces are analyzed using a rate equation model. The activation energy barriers for the relevant diffusion and desorption…

Methane is one of the simplest stable molecules that is both abundant and widely distributed across space. It is thought to have partial origin from interstellar molecular clouds, which are near the beginning of the star formation cycle.…

Solar and Stellar Astrophysics · Physics 2020-04-16 D. Qasim , G. Fedoseev , K. -J. Chuang , J. He , S. Ioppolo , E. F. van Dishoeck , H. Linnartz

Methoxymethanol (CH3OCH2OH, MM) has been identified through gas-phase signatures in both high- and low-mass star-forming regions. This molecule is expected to form upon hydrogen addition and abstraction reactions in CO-rich ice through…

Simple and complex organic molecules (COMs) are observed along different phases of star and planet formation and have been successfully identified in prestellar environments such as dark and translucent clouds. Yet the picture of organic…

The formation of interstellar water has been commonly accepted to occur on the surfaces of icy dust grains in dark molecular clouds at low temperatures (10-20 K), involving hydrogenation reactions of oxygen allotropes. As a result of the…

Astrophysics of Galaxies · Physics 2014-10-22 Thanja Lamberts , Herma Cuppen , Gleb Fedoseev , Sergio Ioppolo , Ko-Ju Chuang , Harold Linnartz

Interstellar formamide (NH2CHO) has recently attracted significant attention due to its potential role as a molecular building block in the formation of precursor biomolecules relevant for the origin of life. Its formation, whether on the…

Earth and Planetary Astrophysics · Physics 2018-10-09 Albert Rimola , Dimitrios Skouteris , Nadia Balucani , Cecilia Ceccarelli , Joan Enrique-Romero , Vianney Taquet , Piero Ugliengo

Even though water is the main constituent in interstellar icy mantles, its chemical origin is not well understood. Three different formation routes have been proposed following hydrogenation of O, O2, or O3, but experimental evidence is…

Astrophysics · Physics 2009-11-13 S. Ioppolo , H. M. Cuppen , C. Romanzin , E. F. van Dishoeck , H. Linnartz

[abridged] The enhanced degrees of deuterium fractionation observed in envelopes around protostars demonstrate the importance of chemistry at low temperatures, relevant in pre- and protostellar cores. formaldehyde is an important species in…

The development of molecular complexity during stellar and planetary formation owes much to the interaction of gas and dust. When the first astrochemical models including solid-state chemistry were developed more than forty years ago, data…

Ethanol (CH3CH2OH) has been detected in interstellar ices within regions associated with the early stages of star and planet formation. Its solid-phase pathways can lead to diverse conditions that can significantly influence its…

Astrophysics of Galaxies · Physics 2026-04-08 J. A. DeVine , J. Terwisscha van Scheltinga , S. Ioppolo , K. -J. Chuang , E. F. van Dishoeck , T. Lamberts