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Chemical functionalization of graphene holds promise for various applications ranging from nanoelectronics to catalysis, drug delivery, and nanoassembly. In many applications it is important to be able to transport adsorbates on graphene in…

Mesoscale and Nanoscale Physics · Physics 2013-03-28 Dmitry Solenov , Kirill A. Velizhanin

The electronic and optical properties of graphene monoxide, a new type of semiconductor materials, are first theoretically studied based on density functional theory. Electronic calculations show that the band gap is 0.952 eV which indicate…

Materials Science · Physics 2012-09-05 Gui Yang , Yufeng Zhang , Xunwang Yan

The ability of atomic hydrogen to chemisorb on graphene makes the latter a promising material for hydrogen storage. Based on scanning tunneling microscopy techniques, we report on site-selective adsorption of atomic hydrogen on convexly…

The variation of the work function upon carbon adsorption on the reconstructed Au(110) surface is measured experimentally and compared to density functional calculations. The adsorption dynamics is simulated with ab-initio molecular…

Atomic Physics · Physics 2018-08-08 H. Z. Jooya , K. S. McKay , E. Kim , P. F. Weck , D. P. Pappas , D. A. Hite , H. R. Sadeghpour

The structure and dynamics of atomic oxygen adsorbed on Ag(410) and Ag(210) surfaces have been investigated using density functional theory. Our results show that the adsorption configuration in which O adatoms decorate the upper side of…

Materials Science · Physics 2009-11-10 N. Bonini , A. Kokalj , A. Dal Corso , S. de Gironcoli , S. Baroni

Currently, the fundamental factors that control the oxygen reduction reaction (ORR) activity of graphene itself, in particular the dependence of the ORR activity on the number of exposed edge sites remain elusive, mainly due to limited…

Materials Science · Physics 2014-11-18 John Benson , Qian Xu , Peng Wang , Yuting Shen , Litao Sun , Tanyuan Wang , Meixian Li , Pagona Papakonstantinou

The adsorption of volatile molecules onto dust grain surfaces fundamentally influences dust-related processes, including condensation of gas-phase molecules, dust coagulation, and planet formation in protoplanetary disks. Using advanced…

Earth and Planetary Astrophysics · Physics 2026-03-05 Lile Wang , Feng Long , Haifeng Yang , Ruobing Dong , Shenzhen Xu

In this work, we investigate the hydrogen-storage properties of Zr-decorated $\gamma$-graphyne monolayer employing Density Functional Theory (DFT) for green energy storage. We predict that each Zr atom decorated on graphyne sheet (2D) can…

Materials Science · Physics 2023-12-29 Mukesh Singh , Alok Shukla , Brahmananda Chakraborty

We use density functional theory to determine the equilibrium shape of graphene flakes, through the calculation of the edge orientation dependence of the edge energy and edge stress of graphene nanoribbons. The edge energy is a nearly…

Mesoscale and Nanoscale Physics · Physics 2011-08-08 Chee Kwan Gan , David J. Srolovitz

The adsorption of CO molecules at the Ca3Ru2O7(001) surface was studied using low-temperature scanning tunneling microscopy (STM) and density functional theory (DFT). Ca3Ru2O7 can be easily cleaved along the (001) plane, yielding a smooth,…

The main challenge to exploiting plasmons for gas vibrational mode sensing is the extremely weak infrared absorption of gas species. In this work, we explore the possibility of trapping free gas molecules via surface adsorption, optical, or…

Mesoscale and Nanoscale Physics · Physics 2020-01-29 Kaveh Khaliji , Sudipta Romen Biswas , Hai Hu , Xiaoxia Yang , Qing Dai , Sang-Hyun Oh , Phaedon Avouris , Tony Low

Surface resistivity of hydrogenated amorphous carbon films was measured as a function of the applied electrical field. The measured dependence shows a sharp ambipolar peak near zero gate voltage. Furthermore, we found that in some samples…

Materials Science · Physics 2014-09-11 Savcho Tinchev

The structure of the double-layer formed at the surface of carbon electrodes is governed by the interactions between the electrode and the electrolyte species. However, carbon is notoriously difficult to simulate accurately, even with…

We report a computational study of the adsorption of zoledronic acid molecule on hydroxyapatite (001) surface within ab initio density functional theory. The systematic study has been performed, from hydroxyapatite bulk and surface, and…

Materials Science · Physics 2017-09-20 Mun-Hyok Ri , Chol-Jun Yu , Yong-Man Jang , Song-Un Kim

We investigate the optical absorption and transmission of few-layer phosphorene in the framework of ab initio density functional simulations and many-body perturbation theory at the level of random phase approximation. In bilayer…

Mesoscale and Nanoscale Physics · Physics 2018-11-13 Zahra Torbatian , Reza Asgari

Graphene based sensor to gas molecules should be ultrasensitive and ultrafast because of the single-atomic thickness of graphene, while the response is not fast. Usually, the measured response time for many molecules, such as CO, NH3, SO2,…

Mesoscale and Nanoscale Physics · Physics 2019-07-09 Hui-Fen Zhang , Bo-Yuan Ning , Tsu-Chien Weng , Dong-Ping Wu , Xi-Jing Ning

The energy to desorb atomic oxygen from an interstellar dust grain surface, $E_{\rm des}$, is an important controlling parameter in gas-grain models; its value impacts the temperature range over which oxygen resides on a dust grain.…

Astrophysics of Galaxies · Physics 2015-06-23 Jiao He , Jianming Shi , Tyler Hopkins , Gianfranco Vidali , Michael J. Kaufman

The wetting properties of graphene have proven controversial and difficult to assess. The presence of a graphene layer on top of a substrate does not significantly change the wetting properties of the solid substrate, suggesting that a…

Soft Condensed Matter · Physics 2017-02-10 Bijoyendra Bera , Noushine Shahidzadeh , Himanshu Mishra , Daniel Bonn

Adsorption of para-Hydrogen on the surface of graphite pre-plated with a single layer of atomic krypton is studied thoretically by means of Path Integral Ground State Monte Carlo simulations. We compute energetics and density profiles of…

Statistical Mechanics · Physics 2009-11-11 Joseph Turnbull , Massimo Boninsegni

The pH dependence of emission from graphene oxide is believed to be due to the protonation of surface functional groups. In this study we use transient absorption spectroscopy to study the sub-picosecond charge dynamics in graphene oxide…

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