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Microphase separation in polymeric systems provides a bottom-up strategy to fabricate nanostructures. Polymers that are reported to undergo microphase separation usually include block copolymers or polyelectrolytes. Neutral homopolymers,…

Soft Condensed Matter · Physics 2022-09-26 Xian Kong , Jian Qin

We consider micro- and macro- phase separation in blends of AB and BC diblock copolymers. We show that, depending on architecture, a number of phase diagram topologies are possible. Microphase separation or macrophase separation can occur,…

Soft Condensed Matter · Physics 2009-10-31 Peter D. Olmsted , Ian W. Hamley

The ability to tune the microstructures formed by block copolymers using accessible physical approaches provides control for practical material applications. A common strategy involves the addition of homopolymers, which can induce…

Soft Condensed Matter · Physics 2025-04-11 Xiangyu Zhang , Jing Zong , Dong Meng

Given the wide range of length scales, the analysis of polymer systems often requires coarse-graining, for which various levels of description may be possible depending on the phenomenon under consideration. Here, we provide a super-coarse…

Soft Condensed Matter · Physics 2024-09-05 Naoki Iso , Yuki Norizoe , Takahiro Sakaue

A linear copolymer made of two reciprocally attracting N-monomer blocks collapses to a compact phase through a novel transition, whose exponents are determined with extensive MC simulations in two and three dimensions. In the former case,…

Soft Condensed Matter · Physics 2009-10-31 E. Orlandini , F. Seno , A. L. Stella

The Leibler theory [L. Leibler, Macromolecules, v.13, 1602 (1980)] for microphase separation in AB block copolymer melts is generalized for systems with arbitrary topology of molecules. A diagrammatic technique for calculation of the…

Soft Condensed Matter · Physics 2009-10-31 A. N. Morozov , J. G. E. M. Fraaije

The miscibility of two interacting quantum systems is an important testing ground for the understanding of complex quantum systems. Two-component Bose-Einstein condensates enable the investigation of this scenario in a particularly well…

Amphiphilic block copolymer solutions form various micellar structures including micelles and vesicles. We applied the density functional theory for block copolymers which we have proposed to amphiphilic block copolymer systems. The 3…

Soft Condensed Matter · Physics 2007-05-23 Takashi Uneyama , Masao Doi

The properties of diluted symmetric A-B diblock copolymers at the interface between A and B homopolymer phases are studied by means of Monte Carlo (MC) simulations of the bond fluctuation model. We calculate segment density profiles as well…

Chemical Physics · Physics 2015-06-26 A. Werner , F. Schmid , K. Binder , M. Mueller

Diblock copolymers by virtue of the chemical dissimilarity between the constituting blocks exhibit microphase separation in the melt state. The phase separated melt can successfully be exploited to control the morphology of the final semi…

Soft Condensed Matter · Physics 2018-02-19 Chitrita Kundu , Nikhil S. Joshi , Ashok Kumar Dasmahapatra

We study binary mixtures of small active and big passive athermal particles interacting via soft repulsive forces on a frictional substrate. Athermal self propelled particles are known to phase separate into a dense aggregate and a dilute…

Soft Condensed Matter · Physics 2018-07-05 Pritha Dolai , Aditi Simha , Shradha Mishra

We investigate the phase behavior of symmetric AB diblock copolymers confined into a thin film. The film boundaries are parallel, impenetrable and attract the A component of the diblock copolymer. Using a self-consistent field technique…

Statistical Mechanics · Physics 2009-10-31 Thorsten Geisinger , Marcus Mueller , Kurt Binder

The influence of size differences, shape, mass and persistent motion on phase separation in binary mixtures has been intensively studied. Here we focus on the exclusive role of diffusivity differences in binary mixtures of equal-sized…

Soft Condensed Matter · Physics 2016-03-04 Simon N. Weber , Christoph A. Weber , Erwin Frey

We investigate the phase behaviour of random copolymers melts via large scale Monte Carlo simulations. We observe macrophase separation into A and B--rich phases as predicted by mean field theory only for systems with a very large…

Soft Condensed Matter · Physics 2009-11-07 J. Houdayer , M. Mueller

We present a generalized theory for studying phase separation in blends of polymers containing dipoles on their backbone. The theory is used to construct co-existence curves and to study the effects of dipolar interactions on interfacial…

Soft Condensed Matter · Physics 2014-11-04 Rajeev Kumar , Bobby G. Sumpter , M. Muthukumar

A system of two self and mutual interacting ring polymers, close together in space, can display several competing equilibrium phases and phase transitions. Using Monte Carlo simulations and combinatorial arguments on a corresponding lattice…

Soft Condensed Matter · Physics 2026-04-17 EJ Janse van Rensburg , E Orlandini , MC Tesi , SG Whittington

The phase behaviour of amphiphilic multiblock copolymers with a large number of blocks in semidilute solutions is studied by lattice Monte Carlo simulations. The influence on the resulting structures of the concentration, the solvent…

Soft Condensed Matter · Physics 2016-08-18 Virginie Hugouvieux , Monique A. V. Axelos , Max Kolb

We employ cell dynamics simulation based on the CH/BD model to investigate the self-assembly behavior of a mixed system consisting of diblock copolymers (AB), homopolymers (C), and Janus nanorods. The results indicate that, at different…

Soft Condensed Matter · Physics 2025-09-24 Y. Q. Guo , J. Liu , H. R. He , N. Wu , J. J. Zhang

We consider the coupling between an external electric field and dissociated ions embedded in anisotropic polarizable media such as block copolymers. We argue that the presence of such ions can induce strong morphological changes and even…

Soft Condensed Matter · Physics 2009-11-07 Yoav Tsori , Francois Tournilhac , David Andelman , Ludwik Leibler

We study AB$_n$ miktoarm star block copolymers in the strong segregation limit, focussing on the role that the AB interface plays in determining the phase behavior. We develop an extension of the kinked-path approach which allows us to…

Soft Condensed Matter · Physics 2007-05-23 Gregory M. Grason , Randall D. Kamien